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Free carrier absorption in self-activated PbWO_4 and Ce-doped Y_3(Al_0.25Ga_0.75)_3O_12 and Gd_3Al_2Ga_3O_12 garnet scintillators

Nonequilibrium carrier dynamics in the scintillators prospective for fast timing in high energy physics and medical imaging applications was studied. The time-resolved free carrier absorption investigation was carried out to study the dynamics of nonequilibrium carriers in wide-band-gap scintillatio...

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Autores principales: Auffray, E., Korjik, M., M.T. Lucchini, S. Nargelas, O. Sidletskiy, G. Tamulaitis, Y. Tratsiak, A. Vaitkevičius
Formato: info:eu-repo/semantics/article
Lenguaje:eng
Publicado: Opt. Mater. 2016
Materias:
Acceso en línea:https://dx.doi.org/10.1016/j.optmat.2016.06.040
http://cds.cern.ch/record/2239269
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author Auffray, E.
Korjik, M.
M.T. Lucchini
S. Nargelas
O. Sidletskiy
G. Tamulaitis
Y. Tratsiak
A. Vaitkevičius
author_facet Auffray, E.
Korjik, M.
M.T. Lucchini
S. Nargelas
O. Sidletskiy
G. Tamulaitis
Y. Tratsiak
A. Vaitkevičius
author_sort Auffray, E.
collection CERN
description Nonequilibrium carrier dynamics in the scintillators prospective for fast timing in high energy physics and medical imaging applications was studied. The time-resolved free carrier absorption investigation was carried out to study the dynamics of nonequilibrium carriers in wide-band-gap scintillation materials: self-activated led tungstate (PbWO_4, PWO) ant two garnet crystals, GAGG:Ce and YAGG:Ce. It was shown that free electrons appear in the conduction band of PWO and YAGG:Ce crystals within a sub-picosecond time scale, while the free holes in GAGG:Ce appear due to delocalization from Gd^3+ ground states to the valence band within a few picoseconds after short-pulse excitation. The influence of Gd ions on the nonequilibrium carrier dynamics is discussed on the base of comparison the results of the free carrier absorption in GAGG:Ce containing gadolinium and in YAGG without Gd in the host lattice.
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spelling cern-22392692019-09-30T06:29:59Z doi:10.1016/j.optmat.2016.06.040 http://cds.cern.ch/record/2239269 eng Auffray, E. Korjik, M. M.T. Lucchini S. Nargelas O. Sidletskiy G. Tamulaitis Y. Tratsiak A. Vaitkevičius Free carrier absorption in self-activated PbWO_4 and Ce-doped Y_3(Al_0.25Ga_0.75)_3O_12 and Gd_3Al_2Ga_3O_12 garnet scintillators Detectors and Experimental Techniques 14: Infrastructure for advanced calorimeters Nonequilibrium carrier dynamics in the scintillators prospective for fast timing in high energy physics and medical imaging applications was studied. The time-resolved free carrier absorption investigation was carried out to study the dynamics of nonequilibrium carriers in wide-band-gap scintillation materials: self-activated led tungstate (PbWO_4, PWO) ant two garnet crystals, GAGG:Ce and YAGG:Ce. It was shown that free electrons appear in the conduction band of PWO and YAGG:Ce crystals within a sub-picosecond time scale, while the free holes in GAGG:Ce appear due to delocalization from Gd^3+ ground states to the valence band within a few picoseconds after short-pulse excitation. The influence of Gd ions on the nonequilibrium carrier dynamics is discussed on the base of comparison the results of the free carrier absorption in GAGG:Ce containing gadolinium and in YAGG without Gd in the host lattice. info:eu-repo/grantAgreement/EC/FP7/654168 info:eu-repo/semantics/openAccess Education Level info:eu-repo/semantics/article http://cds.cern.ch/record/2239269 Opt. Mater. Opt. Mater., (2016) pp. 461-465 2016
spellingShingle Detectors and Experimental Techniques
14: Infrastructure for advanced calorimeters
Auffray, E.
Korjik, M.
M.T. Lucchini
S. Nargelas
O. Sidletskiy
G. Tamulaitis
Y. Tratsiak
A. Vaitkevičius
Free carrier absorption in self-activated PbWO_4 and Ce-doped Y_3(Al_0.25Ga_0.75)_3O_12 and Gd_3Al_2Ga_3O_12 garnet scintillators
title Free carrier absorption in self-activated PbWO_4 and Ce-doped Y_3(Al_0.25Ga_0.75)_3O_12 and Gd_3Al_2Ga_3O_12 garnet scintillators
title_full Free carrier absorption in self-activated PbWO_4 and Ce-doped Y_3(Al_0.25Ga_0.75)_3O_12 and Gd_3Al_2Ga_3O_12 garnet scintillators
title_fullStr Free carrier absorption in self-activated PbWO_4 and Ce-doped Y_3(Al_0.25Ga_0.75)_3O_12 and Gd_3Al_2Ga_3O_12 garnet scintillators
title_full_unstemmed Free carrier absorption in self-activated PbWO_4 and Ce-doped Y_3(Al_0.25Ga_0.75)_3O_12 and Gd_3Al_2Ga_3O_12 garnet scintillators
title_short Free carrier absorption in self-activated PbWO_4 and Ce-doped Y_3(Al_0.25Ga_0.75)_3O_12 and Gd_3Al_2Ga_3O_12 garnet scintillators
title_sort free carrier absorption in self-activated pbwo_4 and ce-doped y_3(al_0.25ga_0.75)_3o_12 and gd_3al_2ga_3o_12 garnet scintillators
topic Detectors and Experimental Techniques
14: Infrastructure for advanced calorimeters
url https://dx.doi.org/10.1016/j.optmat.2016.06.040
http://cds.cern.ch/record/2239269
http://cds.cern.ch/record/2239269
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