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A cold electron-impact ion source driven by a photo-cathode – New opportunities for the delivery of radioactive molecular beams?

The thick-target ISOL (Isotope mass Separation OnLine) method provides beams of more than 1000 radionuclides of 74 elements. The method is well established for elements with sufficiently high volatility at ca. 2000 °C. To extract non-volatile elements the formation of a volatile molecule is required...

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Detalles Bibliográficos
Autores principales: Ballof, Jochen, Au, Mia, Barbero, Ermanno, Chrysalidis, Katerina, Düllmann, Christoph E., Fedosseev, Valentin, Granados, Eduardo, Heinke, Reinhard, Marsh, Bruce A., Owen, Michael, Rothe, Sebastian, Stora, Thierry, Yakushev, Alexander
Lenguaje:eng
Publicado: 2022
Materias:
Acceso en línea:https://dx.doi.org/10.1088/1742-6596/2244/1/012072
http://cds.cern.ch/record/2824512
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author Ballof, Jochen
Au, Mia
Barbero, Ermanno
Chrysalidis, Katerina
Düllmann, Christoph E.
Fedosseev, Valentin
Granados, Eduardo
Heinke, Reinhard
Marsh, Bruce A.
Owen, Michael
Rothe, Sebastian
Stora, Thierry
Yakushev, Alexander
author_facet Ballof, Jochen
Au, Mia
Barbero, Ermanno
Chrysalidis, Katerina
Düllmann, Christoph E.
Fedosseev, Valentin
Granados, Eduardo
Heinke, Reinhard
Marsh, Bruce A.
Owen, Michael
Rothe, Sebastian
Stora, Thierry
Yakushev, Alexander
author_sort Ballof, Jochen
collection CERN
description The thick-target ISOL (Isotope mass Separation OnLine) method provides beams of more than 1000 radionuclides of 74 elements. The method is well established for elements with sufficiently high volatility at ca. 2000 °C. To extract non-volatile elements the formation of a volatile molecule is required. While successful in some cases (e.g. carbon or boron), most of these elements are not yet available as ISOL beam. A variety of volatile carrier molecules has been proposed for all elements produced in the target material, but their probability of survival during the extraction and ionization process is often limited by the high temperatures required for isotope diffusion in the thick targets and for ion source operation. While cold target concepts have already been proposed, the normal mode of operation of the typically used Versatile Arc Discharge Ion Source (VADIS) with a hot cathode is not well suited. Here, we report about first measurements with an electron-impact ion source operated at ambient temperature using electrons that were liberated via the photo-electric effect from a copper cathode.
id cern-2824512
institution Organización Europea para la Investigación Nuclear
language eng
publishDate 2022
record_format invenio
spelling cern-28245122023-06-29T03:30:52Zdoi:10.1088/1742-6596/2244/1/012072http://cds.cern.ch/record/2824512engBallof, JochenAu, MiaBarbero, ErmannoChrysalidis, KaterinaDüllmann, Christoph E.Fedosseev, ValentinGranados, EduardoHeinke, ReinhardMarsh, Bruce A.Owen, MichaelRothe, SebastianStora, ThierryYakushev, AlexanderA cold electron-impact ion source driven by a photo-cathode – New opportunities for the delivery of radioactive molecular beams?physics.ins-detDetectors and Experimental TechniquesThe thick-target ISOL (Isotope mass Separation OnLine) method provides beams of more than 1000 radionuclides of 74 elements. The method is well established for elements with sufficiently high volatility at ca. 2000 °C. To extract non-volatile elements the formation of a volatile molecule is required. While successful in some cases (e.g. carbon or boron), most of these elements are not yet available as ISOL beam. A variety of volatile carrier molecules has been proposed for all elements produced in the target material, but their probability of survival during the extraction and ionization process is often limited by the high temperatures required for isotope diffusion in the thick targets and for ion source operation. While cold target concepts have already been proposed, the normal mode of operation of the typically used Versatile Arc Discharge Ion Source (VADIS) with a hot cathode is not well suited. Here, we report about first measurements with an electron-impact ion source operated at ambient temperature using electrons that were liberated via the photo-electric effect from a copper cathode.The thick-target ISOL (Isotope mass Separation OnLine) method provides beams of more than 1000 radionuclides of 74 elements. The method is well established for elements with sufficiently high volatility at ca. 2000 {\deg}C. To extract non-volatile elements the formation of a volatile molecule is required. While successful in some cases (e.g. carbon or boron), most of these elements are not yet available as ISOL beam. A variety of volatile carrier molecules has been proposed for all elements produced in the target material, but their probability of survival during the extraction and ionization process is often limited by the high temperatures required for isotope diffusion in the thick targets and for ion source operation. While cold target concepts have already been proposed, the normal mode of operation of the typically used Versatile Arc Discharge Ion Source (VADIS) with a hot cathode is not well suited. Here, we report about first measurements with an electron-impact ion source operated at ambient temperature using electrons that were liberated via the photo-electric effect from a copper cathode.arXiv:2110.00651oai:cds.cern.ch:28245122022
spellingShingle physics.ins-det
Detectors and Experimental Techniques
Ballof, Jochen
Au, Mia
Barbero, Ermanno
Chrysalidis, Katerina
Düllmann, Christoph E.
Fedosseev, Valentin
Granados, Eduardo
Heinke, Reinhard
Marsh, Bruce A.
Owen, Michael
Rothe, Sebastian
Stora, Thierry
Yakushev, Alexander
A cold electron-impact ion source driven by a photo-cathode – New opportunities for the delivery of radioactive molecular beams?
title A cold electron-impact ion source driven by a photo-cathode – New opportunities for the delivery of radioactive molecular beams?
title_full A cold electron-impact ion source driven by a photo-cathode – New opportunities for the delivery of radioactive molecular beams?
title_fullStr A cold electron-impact ion source driven by a photo-cathode – New opportunities for the delivery of radioactive molecular beams?
title_full_unstemmed A cold electron-impact ion source driven by a photo-cathode – New opportunities for the delivery of radioactive molecular beams?
title_short A cold electron-impact ion source driven by a photo-cathode – New opportunities for the delivery of radioactive molecular beams?
title_sort cold electron-impact ion source driven by a photo-cathode – new opportunities for the delivery of radioactive molecular beams?
topic physics.ins-det
Detectors and Experimental Techniques
url https://dx.doi.org/10.1088/1742-6596/2244/1/012072
http://cds.cern.ch/record/2824512
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