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Measurement of the $^{14}$N(n,p)$^{14}$C cross section at the CERN n_TOF facility from sub-thermal energy to 800 keV
Background: The <math><mrow><mmultiscripts><mi mathvariant="normal">N</mi><mprescripts/><none/><mn>14</mn></mmultiscripts><mo>(</mo><mi>n</mi><mo>,</mo><mi>p</mi><mo>)</mo&g...
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Lenguaje: | eng |
Publicado: |
2022
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Materias: | |
Acceso en línea: | https://dx.doi.org/10.1103/PhysRevC.107.064617 http://cds.cern.ch/record/2845228 |
_version_ | 1780976539539603456 |
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author | Torres-Sánchez, Pablo Praena, Javier Porras, Ignacio Sabaté-Gilarte, Marta Lederer-Woods, Claudia Aberle, Oliver Alcayne, Victor Amaducci, Simone Andrzejewski, Józef Audouin, Laurent Bécares, Vicente Babiano-Suarez, Victor Bacak, Michael Barbagallo, Massimo Bečvář, František Bellia, Giorgio Berthoumieux, Eric Billowes, Jon Bosnar, Damir Brown, Adam Busso, Maurizio Caamaño, Manuel Caballero, Luis Calviño, Francisco Calviani, Marco Cano-Ott, Daniel Casanovas, Adria Cerutti, Francesco Chen, Yonghao Chiaveri, Enrico Colonna, Nicola Cortés, Guillem Cortés-Giraldo, Miguel Cosentino, Luigi Cristallo, Sergio Damone, Lucia-Anna Diakaki, Maria Dietz, Mirco Domingo-Pardo, César Dressler, Rugard Dupont, Emmeric Durán, Ignacio Eleme, Zinovia Fernández-Domínguez, Beatriz Ferrari, Alfredo Ferrer, Francisco Javier Finocchiaro, Paolo Furman, Valter Göbel, Kathrin Garg, Ruchi Gawlik-Ramięga, Aleksandra Geslot, Benoit Gilardoni, Simone Glodariu, Tudor Gonçalves, Isabel González-Romero, Enrique Guerrero, Carlos Gunsing, Frank Harada, Hideo Heinitz, Stephan Heyse, Jan Jenkins, David Jericha, Erwin Käppeler, Franz Kadi, Yacine Kimura, Atsushi Kivel, Niko Kokkoris, Michael Kopatch, Yury Krtička, Milan Kurtulgil, Deniz Ladarescu, Ion Leeb, Helmut Lerendegui-Marco, Jorge Meo, Sergio Lo Lonsdale, Sarah-Jane Macina, Daniela Manna, Alice Martínez, Trinitario Masi, Alessandro Massimi, Cristian Mastinu, Pierfrancesco Mastromarco, Mario Matteucci, Francesca Maugeri, Emilio-Andrea Mazzone, Annamaria Mendoza, Emilio Mengoni, Alberto Michalopoulou, Veatriki Milazzo, Paolo Maria Mingrone, Federica Musumarra, Agatino Negret, Alexandru Nolte, Ralf Ogállar, Francisco Oprea, Andreea Patronis, Nikolas Pavlik, Andreas Perkowski, Jarosław Persanti, Luciano Quesada, José-Manuel Radeck, Désirée Ramos-Doval, Diego Rauscher, Thomas Reifarth, René Rochman, Dimitri Rubbia, Carlo Saxena, Alok Schillebeeckx, Peter Schumann, Dorothea Smith, Gavin Sosnin, Nikolay Stamatopoulos, Athanasios Tagliente, Giuseppe Tain, José Talip, T. Talip, Zeynep Tarifeño-Saldivia, Ariel Tassan-Got, Laurent Tsinganis, Andrea Ulrich, Jiri Urlass, Sebastian Valenta, Stanislav Vannini, Gianni Variale, Vincenzo Vaz, Pedro Ventura, Alberto Vlachoudis, Vasilis Vlastou, Rosa Wallner, Anton Woods, PhilipJohn Woods, Philip John Wright, Tobias Žugec, Petar |
author_facet | Torres-Sánchez, Pablo Praena, Javier Porras, Ignacio Sabaté-Gilarte, Marta Lederer-Woods, Claudia Aberle, Oliver Alcayne, Victor Amaducci, Simone Andrzejewski, Józef Audouin, Laurent Bécares, Vicente Babiano-Suarez, Victor Bacak, Michael Barbagallo, Massimo Bečvář, František Bellia, Giorgio Berthoumieux, Eric Billowes, Jon Bosnar, Damir Brown, Adam Busso, Maurizio Caamaño, Manuel Caballero, Luis Calviño, Francisco Calviani, Marco Cano-Ott, Daniel Casanovas, Adria Cerutti, Francesco Chen, Yonghao Chiaveri, Enrico Colonna, Nicola Cortés, Guillem Cortés-Giraldo, Miguel Cosentino, Luigi Cristallo, Sergio Damone, Lucia-Anna Diakaki, Maria Dietz, Mirco Domingo-Pardo, César Dressler, Rugard Dupont, Emmeric Durán, Ignacio Eleme, Zinovia Fernández-Domínguez, Beatriz Ferrari, Alfredo Ferrer, Francisco Javier Finocchiaro, Paolo Furman, Valter Göbel, Kathrin Garg, Ruchi Gawlik-Ramięga, Aleksandra Geslot, Benoit Gilardoni, Simone Glodariu, Tudor Gonçalves, Isabel González-Romero, Enrique Guerrero, Carlos Gunsing, Frank Harada, Hideo Heinitz, Stephan Heyse, Jan Jenkins, David Jericha, Erwin Käppeler, Franz Kadi, Yacine Kimura, Atsushi Kivel, Niko Kokkoris, Michael Kopatch, Yury Krtička, Milan Kurtulgil, Deniz Ladarescu, Ion Leeb, Helmut Lerendegui-Marco, Jorge Meo, Sergio Lo Lonsdale, Sarah-Jane Macina, Daniela Manna, Alice Martínez, Trinitario Masi, Alessandro Massimi, Cristian Mastinu, Pierfrancesco Mastromarco, Mario Matteucci, Francesca Maugeri, Emilio-Andrea Mazzone, Annamaria Mendoza, Emilio Mengoni, Alberto Michalopoulou, Veatriki Milazzo, Paolo Maria Mingrone, Federica Musumarra, Agatino Negret, Alexandru Nolte, Ralf Ogállar, Francisco Oprea, Andreea Patronis, Nikolas Pavlik, Andreas Perkowski, Jarosław Persanti, Luciano Quesada, José-Manuel Radeck, Désirée Ramos-Doval, Diego Rauscher, Thomas Reifarth, René Rochman, Dimitri Rubbia, Carlo Saxena, Alok Schillebeeckx, Peter Schumann, Dorothea Smith, Gavin Sosnin, Nikolay Stamatopoulos, Athanasios Tagliente, Giuseppe Tain, José Talip, T. Talip, Zeynep Tarifeño-Saldivia, Ariel Tassan-Got, Laurent Tsinganis, Andrea Ulrich, Jiri Urlass, Sebastian Valenta, Stanislav Vannini, Gianni Variale, Vincenzo Vaz, Pedro Ventura, Alberto Vlachoudis, Vasilis Vlastou, Rosa Wallner, Anton Woods, PhilipJohn Woods, Philip John Wright, Tobias Žugec, Petar |
author_sort | Torres-Sánchez, Pablo |
collection | CERN |
description | Background: The <math><mrow><mmultiscripts><mi mathvariant="normal">N</mi><mprescripts/><none/><mn>14</mn></mmultiscripts><mo>(</mo><mi>n</mi><mo>,</mo><mi>p</mi><mo>)</mo><mmultiscripts><mi mathvariant="normal">C</mi><mprescripts/><none/><mn>14</mn></mmultiscripts></mrow></math> reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where <math><mmultiscripts><mi mathvariant="normal">N</mi><mprescripts/><none/><mn>14</mn></mmultiscripts></math> acts as a neutron poison in the <math><mi>s</mi></math> process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region, and resonance region.Purpose: We aim to measure the <math><mrow><mmultiscripts><mi mathvariant="normal">N</mi><mprescripts/><none/><mn>14</mn></mmultiscripts><mo>(</mo><mi>n</mi><mo>,</mo><mi>p</mi><mo>)</mo><mmultiscripts><mi mathvariant="normal">C</mi><mprescripts/><none/><mn>14</mn></mmultiscripts></mrow></math> cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and provide calculations of Maxwellian averaged cross sections (MACS).
Method: We apply the time-of-flight technique at Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. <math><mrow><mmultiscripts><mi mathvariant="normal">B</mi><mprescripts/><none/><mn>10</mn></mmultiscripts><mo>(</mo><mi mathvariant="normal">n</mi><mo>,</mo><mi>α</mi><mo>)</mo><mmultiscripts><mi>Li</mi><mprescripts/><none/><mn>7</mn></mmultiscripts></mrow></math> and <math><mrow><mmultiscripts><mi mathvariant="normal">U</mi><mprescripts/><none/><mn>235</mn></mmultiscripts><mo>(</mo><mi>n</mi><mo>,</mo><mi>f</mi><mo>)</mo></mrow></math> reactions are used as references. Two detection systems are run simultaneously, one on beam and another off beam. Resonances are described with the <math><mi>R</mi></math>-matrix code sammy.Results: The cross section was measured from subthermal energy to 800 keV, resolving the first two resonances (at 492.7 and 644 keV). A thermal cross section was obtained (<math><mrow><mn>1.809</mn><mo>±</mo><mn>0.045</mn></mrow></math> b) that is lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations. A 1/<math><mi>v</mi></math> energy dependence of the cross section was confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations.
Conclusions: Our measurement has allowed determination of the <math><mrow><mmultiscripts><mi mathvariant="normal">N</mi><mprescripts/><none/><mn>14</mn></mmultiscripts><mo>(</mo><mi>n</mi><mo>,</mo><mi>p</mi><mo>)</mo></mrow></math> cross section over a wide energy range for the first time. We have obtained cross sections with high accuracy (2.5%) from subthermal energy to 800 keV and used these data to calculate the MACS for <math><mrow><mi>k</mi><mi>T</mi><mo>=</mo><mn>5</mn></mrow></math> to <math><mrow><mi>k</mi><mi>T</mi><mo>=</mo><mn>100</mn></mrow></math> keV. |
id | cern-2845228 |
institution | Organización Europea para la Investigación Nuclear |
language | eng |
publishDate | 2022 |
record_format | invenio |
spelling | cern-28452282023-07-27T03:49:56Zdoi:10.1103/PhysRevC.107.064617http://cds.cern.ch/record/2845228engTorres-Sánchez, PabloPraena, JavierPorras, IgnacioSabaté-Gilarte, MartaLederer-Woods, ClaudiaAberle, OliverAlcayne, VictorAmaducci, SimoneAndrzejewski, JózefAudouin, LaurentBécares, VicenteBabiano-Suarez, VictorBacak, MichaelBarbagallo, MassimoBečvář, FrantišekBellia, GiorgioBerthoumieux, EricBillowes, JonBosnar, DamirBrown, AdamBusso, MaurizioCaamaño, ManuelCaballero, LuisCalviño, FranciscoCalviani, MarcoCano-Ott, DanielCasanovas, AdriaCerutti, FrancescoChen, YonghaoChiaveri, EnricoColonna, NicolaCortés, GuillemCortés-Giraldo, MiguelCosentino, LuigiCristallo, SergioDamone, Lucia-AnnaDiakaki, MariaDietz, MircoDomingo-Pardo, CésarDressler, RugardDupont, EmmericDurán, IgnacioEleme, ZinoviaFernández-Domínguez, BeatrizFerrari, AlfredoFerrer, Francisco JavierFinocchiaro, PaoloFurman, ValterGöbel, KathrinGarg, RuchiGawlik-Ramięga, AleksandraGeslot, BenoitGilardoni, SimoneGlodariu, TudorGonçalves, IsabelGonzález-Romero, EnriqueGuerrero, CarlosGunsing, FrankHarada, HideoHeinitz, StephanHeyse, JanJenkins, DavidJericha, ErwinKäppeler, FranzKadi, YacineKimura, AtsushiKivel, NikoKokkoris, MichaelKopatch, YuryKrtička, MilanKurtulgil, DenizLadarescu, IonLeeb, HelmutLerendegui-Marco, JorgeMeo, Sergio LoLonsdale, Sarah-JaneMacina, DanielaManna, AliceMartínez, TrinitarioMasi, AlessandroMassimi, CristianMastinu, PierfrancescoMastromarco, MarioMatteucci, FrancescaMaugeri, Emilio-AndreaMazzone, AnnamariaMendoza, EmilioMengoni, AlbertoMichalopoulou, VeatrikiMilazzo, Paolo MariaMingrone, FedericaMusumarra, AgatinoNegret, AlexandruNolte, RalfOgállar, FranciscoOprea, AndreeaPatronis, NikolasPavlik, AndreasPerkowski, JarosławPersanti, LucianoQuesada, José-ManuelRadeck, DésiréeRamos-Doval, DiegoRauscher, ThomasReifarth, RenéRochman, DimitriRubbia, CarloSaxena, AlokSchillebeeckx, PeterSchumann, DorotheaSmith, GavinSosnin, NikolayStamatopoulos, AthanasiosTagliente, GiuseppeTain, JoséTalip, T.Talip, ZeynepTarifeño-Saldivia, ArielTassan-Got, LaurentTsinganis, AndreaUlrich, JiriUrlass, SebastianValenta, StanislavVannini, GianniVariale, VincenzoVaz, PedroVentura, AlbertoVlachoudis, VasilisVlastou, RosaWallner, AntonWoods, PhilipJohnWoods, Philip JohnWright, TobiasŽugec, PetarMeasurement of the $^{14}$N(n,p)$^{14}$C cross section at the CERN n_TOF facility from sub-thermal energy to 800 keVnucl-exNuclear Physics - ExperimentBackground: The <math><mrow><mmultiscripts><mi mathvariant="normal">N</mi><mprescripts/><none/><mn>14</mn></mmultiscripts><mo>(</mo><mi>n</mi><mo>,</mo><mi>p</mi><mo>)</mo><mmultiscripts><mi mathvariant="normal">C</mi><mprescripts/><none/><mn>14</mn></mmultiscripts></mrow></math> reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where <math><mmultiscripts><mi mathvariant="normal">N</mi><mprescripts/><none/><mn>14</mn></mmultiscripts></math> acts as a neutron poison in the <math><mi>s</mi></math> process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region, and resonance region.Purpose: We aim to measure the <math><mrow><mmultiscripts><mi mathvariant="normal">N</mi><mprescripts/><none/><mn>14</mn></mmultiscripts><mo>(</mo><mi>n</mi><mo>,</mo><mi>p</mi><mo>)</mo><mmultiscripts><mi mathvariant="normal">C</mi><mprescripts/><none/><mn>14</mn></mmultiscripts></mrow></math> cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and provide calculations of Maxwellian averaged cross sections (MACS). Method: We apply the time-of-flight technique at Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. <math><mrow><mmultiscripts><mi mathvariant="normal">B</mi><mprescripts/><none/><mn>10</mn></mmultiscripts><mo>(</mo><mi mathvariant="normal">n</mi><mo>,</mo><mi>α</mi><mo>)</mo><mmultiscripts><mi>Li</mi><mprescripts/><none/><mn>7</mn></mmultiscripts></mrow></math> and <math><mrow><mmultiscripts><mi mathvariant="normal">U</mi><mprescripts/><none/><mn>235</mn></mmultiscripts><mo>(</mo><mi>n</mi><mo>,</mo><mi>f</mi><mo>)</mo></mrow></math> reactions are used as references. Two detection systems are run simultaneously, one on beam and another off beam. Resonances are described with the <math><mi>R</mi></math>-matrix code sammy.Results: The cross section was measured from subthermal energy to 800 keV, resolving the first two resonances (at 492.7 and 644 keV). A thermal cross section was obtained (<math><mrow><mn>1.809</mn><mo>±</mo><mn>0.045</mn></mrow></math> b) that is lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations. A 1/<math><mi>v</mi></math> energy dependence of the cross section was confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations. Conclusions: Our measurement has allowed determination of the <math><mrow><mmultiscripts><mi mathvariant="normal">N</mi><mprescripts/><none/><mn>14</mn></mmultiscripts><mo>(</mo><mi>n</mi><mo>,</mo><mi>p</mi><mo>)</mo></mrow></math> cross section over a wide energy range for the first time. We have obtained cross sections with high accuracy (2.5%) from subthermal energy to 800 keV and used these data to calculate the MACS for <math><mrow><mi>k</mi><mi>T</mi><mo>=</mo><mn>5</mn></mrow></math> to <math><mrow><mi>k</mi><mi>T</mi><mo>=</mo><mn>100</mn></mrow></math> keV.Background: The $^{14}$N(n,p)$^{14}$C reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where 14N acts as a neutron poison in the s-process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region and resonance region. Purpose: Measuring the 14N(n,p)14C cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and providing calculations of Maxwellian averaged cross sections (MACS). Method: Time-of-flight technique. Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. $^{10}$B(n,${\alpha}$)$^7$Li and $^{235}$U(n,f) reactions as references. Two detection systems running simultaneously, one on-beam and another off-beam. Description of the resonances with the R-matrix code sammy. Results: The cross section has been measured from sub-thermal energy to 800 keV resolving the two first resonances (at 492.7 and 644 keV). A thermal cross-section (1.809$\pm$0.045 b) lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations has been obtained. A 1/v energy dependence of the cross section has been confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations. Conclusions: Our measurement has allowed to determine the $^{14}$N(n,p) cross-section over a wide energy range for the first time. We have obtained cross-sections with high accuracy (2.5 %) from sub-thermal energy to 800 keV and used these data to calculate the MACS for kT = 5 to kT = 100 keV.arXiv:2212.05128oai:cds.cern.ch:28452282022-12-09 |
spellingShingle | nucl-ex Nuclear Physics - Experiment Torres-Sánchez, Pablo Praena, Javier Porras, Ignacio Sabaté-Gilarte, Marta Lederer-Woods, Claudia Aberle, Oliver Alcayne, Victor Amaducci, Simone Andrzejewski, Józef Audouin, Laurent Bécares, Vicente Babiano-Suarez, Victor Bacak, Michael Barbagallo, Massimo Bečvář, František Bellia, Giorgio Berthoumieux, Eric Billowes, Jon Bosnar, Damir Brown, Adam Busso, Maurizio Caamaño, Manuel Caballero, Luis Calviño, Francisco Calviani, Marco Cano-Ott, Daniel Casanovas, Adria Cerutti, Francesco Chen, Yonghao Chiaveri, Enrico Colonna, Nicola Cortés, Guillem Cortés-Giraldo, Miguel Cosentino, Luigi Cristallo, Sergio Damone, Lucia-Anna Diakaki, Maria Dietz, Mirco Domingo-Pardo, César Dressler, Rugard Dupont, Emmeric Durán, Ignacio Eleme, Zinovia Fernández-Domínguez, Beatriz Ferrari, Alfredo Ferrer, Francisco Javier Finocchiaro, Paolo Furman, Valter Göbel, Kathrin Garg, Ruchi Gawlik-Ramięga, Aleksandra Geslot, Benoit Gilardoni, Simone Glodariu, Tudor Gonçalves, Isabel González-Romero, Enrique Guerrero, Carlos Gunsing, Frank Harada, Hideo Heinitz, Stephan Heyse, Jan Jenkins, David Jericha, Erwin Käppeler, Franz Kadi, Yacine Kimura, Atsushi Kivel, Niko Kokkoris, Michael Kopatch, Yury Krtička, Milan Kurtulgil, Deniz Ladarescu, Ion Leeb, Helmut Lerendegui-Marco, Jorge Meo, Sergio Lo Lonsdale, Sarah-Jane Macina, Daniela Manna, Alice Martínez, Trinitario Masi, Alessandro Massimi, Cristian Mastinu, Pierfrancesco Mastromarco, Mario Matteucci, Francesca Maugeri, Emilio-Andrea Mazzone, Annamaria Mendoza, Emilio Mengoni, Alberto Michalopoulou, Veatriki Milazzo, Paolo Maria Mingrone, Federica Musumarra, Agatino Negret, Alexandru Nolte, Ralf Ogállar, Francisco Oprea, Andreea Patronis, Nikolas Pavlik, Andreas Perkowski, Jarosław Persanti, Luciano Quesada, José-Manuel Radeck, Désirée Ramos-Doval, Diego Rauscher, Thomas Reifarth, René Rochman, Dimitri Rubbia, Carlo Saxena, Alok Schillebeeckx, Peter Schumann, Dorothea Smith, Gavin Sosnin, Nikolay Stamatopoulos, Athanasios Tagliente, Giuseppe Tain, José Talip, T. Talip, Zeynep Tarifeño-Saldivia, Ariel Tassan-Got, Laurent Tsinganis, Andrea Ulrich, Jiri Urlass, Sebastian Valenta, Stanislav Vannini, Gianni Variale, Vincenzo Vaz, Pedro Ventura, Alberto Vlachoudis, Vasilis Vlastou, Rosa Wallner, Anton Woods, PhilipJohn Woods, Philip John Wright, Tobias Žugec, Petar Measurement of the $^{14}$N(n,p)$^{14}$C cross section at the CERN n_TOF facility from sub-thermal energy to 800 keV |
title | Measurement of the $^{14}$N(n,p)$^{14}$C cross section at the CERN n_TOF facility from sub-thermal energy to 800 keV |
title_full | Measurement of the $^{14}$N(n,p)$^{14}$C cross section at the CERN n_TOF facility from sub-thermal energy to 800 keV |
title_fullStr | Measurement of the $^{14}$N(n,p)$^{14}$C cross section at the CERN n_TOF facility from sub-thermal energy to 800 keV |
title_full_unstemmed | Measurement of the $^{14}$N(n,p)$^{14}$C cross section at the CERN n_TOF facility from sub-thermal energy to 800 keV |
title_short | Measurement of the $^{14}$N(n,p)$^{14}$C cross section at the CERN n_TOF facility from sub-thermal energy to 800 keV |
title_sort | measurement of the $^{14}$n(n,p)$^{14}$c cross section at the cern n_tof facility from sub-thermal energy to 800 kev |
topic | nucl-ex Nuclear Physics - Experiment |
url | https://dx.doi.org/10.1103/PhysRevC.107.064617 http://cds.cern.ch/record/2845228 |
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