Cargando…

In-source and in-trap formation of molecular ions in the actinide mass range at CERN-ISOLDE

The use of radioactive molecules for fundamental physics research is a developing interdisciplinary field limited dominantly by their scarce availability. In this work, radioactive molecular ion beams containing actinide nuclei extracted from uranium carbide targets are produced via the Isotope Sepa...

Descripción completa

Detalles Bibliográficos
Autores principales: Au, M., Athanasakis-Kaklamanakis, M., Nies, L., Ballof, J., Berger, R., Chrysalidis, K., Fischer, P., Heinke, R., Johnson, J., Köster, U., Leimbach, D., Marsh, B., Mougeot, M., Reich, B., Reilly, J., Reis, E., Schlaich, M., Schweiger, Ch., Schweikhard, L., Stegemann, S., Wessolek, J., Wienholtz, F., Wilkins, S.G., Wojtaczka, W., Düllmann, Ch.E., Rothe, S.
Lenguaje:eng
Publicado: 2023
Materias:
Acceso en línea:https://dx.doi.org/10.1016/j.nimb.2023.05.015
http://cds.cern.ch/record/2855726
_version_ 1780977473261928448
author Au, M.
Athanasakis-Kaklamanakis, M.
Nies, L.
Ballof, J.
Berger, R.
Chrysalidis, K.
Fischer, P.
Heinke, R.
Johnson, J.
Köster, U.
Leimbach, D.
Marsh, B.
Mougeot, M.
Reich, B.
Reilly, J.
Reis, E.
Schlaich, M.
Schweiger, Ch.
Schweikhard, L.
Stegemann, S.
Wessolek, J.
Wienholtz, F.
Wilkins, S.G.
Wojtaczka, W.
Düllmann, Ch.E.
Rothe, S.
author_facet Au, M.
Athanasakis-Kaklamanakis, M.
Nies, L.
Ballof, J.
Berger, R.
Chrysalidis, K.
Fischer, P.
Heinke, R.
Johnson, J.
Köster, U.
Leimbach, D.
Marsh, B.
Mougeot, M.
Reich, B.
Reilly, J.
Reis, E.
Schlaich, M.
Schweiger, Ch.
Schweikhard, L.
Stegemann, S.
Wessolek, J.
Wienholtz, F.
Wilkins, S.G.
Wojtaczka, W.
Düllmann, Ch.E.
Rothe, S.
author_sort Au, M.
collection CERN
description The use of radioactive molecules for fundamental physics research is a developing interdisciplinary field limited dominantly by their scarce availability. In this work, radioactive molecular ion beams containing actinide nuclei extracted from uranium carbide targets are produced via the Isotope Separation On-Line technique at the CERN-ISOLDE facility. Two methods of molecular beam production are studied: extraction of molecular ion beams from the ion source, and formation of molecular ions from the mass-separated ion beam in a gas-filled radio-frequency quadrupole ion trap. Ion currents of U<math altimg="si66.svg" display="inline" id="d1e3016"><msup><mrow/><mrow><mo>+</mo></mrow></msup></math>, UO1−3<sup loc="post">+</sup>, UC1−3<sup loc="post">+</sup>, UF1−4<sup loc="post">+</sup>, UF1,2O1,2<sup loc="post">+</sup> are reported. Metastable tantalum and uranium fluoride molecular ions are identified. Formation of UO1−3<sup loc="post">+</sup>, U(OH)1−3<sup loc="post">+</sup>, UC1−3<sup loc="post">+</sup>, UF1,2O1,2<sup loc="post">+</sup> from mass-separated beams of U<math altimg="si66.svg" display="inline" id="d1e3073"><msup><mrow/><mrow><mo>+</mo></mrow></msup></math>, UF1,2<sup loc="post">+</sup> with residual gas is observed in the ion trap. The effect of trapping time on molecular formation is presented.
id cern-2855726
institution Organización Europea para la Investigación Nuclear
language eng
publishDate 2023
record_format invenio
spelling cern-28557262023-09-22T03:32:02Zdoi:10.1016/j.nimb.2023.05.015http://cds.cern.ch/record/2855726engAu, M.Athanasakis-Kaklamanakis, M.Nies, L.Ballof, J.Berger, R.Chrysalidis, K.Fischer, P.Heinke, R.Johnson, J.Köster, U.Leimbach, D.Marsh, B.Mougeot, M.Reich, B.Reilly, J.Reis, E.Schlaich, M.Schweiger, Ch.Schweikhard, L.Stegemann, S.Wessolek, J.Wienholtz, F.Wilkins, S.G.Wojtaczka, W.Düllmann, Ch.E.Rothe, S.In-source and in-trap formation of molecular ions in the actinide mass range at CERN-ISOLDEphysics.ins-detDetectors and Experimental TechniquesThe use of radioactive molecules for fundamental physics research is a developing interdisciplinary field limited dominantly by their scarce availability. In this work, radioactive molecular ion beams containing actinide nuclei extracted from uranium carbide targets are produced via the Isotope Separation On-Line technique at the CERN-ISOLDE facility. Two methods of molecular beam production are studied: extraction of molecular ion beams from the ion source, and formation of molecular ions from the mass-separated ion beam in a gas-filled radio-frequency quadrupole ion trap. Ion currents of U<math altimg="si66.svg" display="inline" id="d1e3016"><msup><mrow/><mrow><mo>+</mo></mrow></msup></math>, UO1−3<sup loc="post">+</sup>, UC1−3<sup loc="post">+</sup>, UF1−4<sup loc="post">+</sup>, UF1,2O1,2<sup loc="post">+</sup> are reported. Metastable tantalum and uranium fluoride molecular ions are identified. Formation of UO1−3<sup loc="post">+</sup>, U(OH)1−3<sup loc="post">+</sup>, UC1−3<sup loc="post">+</sup>, UF1,2O1,2<sup loc="post">+</sup> from mass-separated beams of U<math altimg="si66.svg" display="inline" id="d1e3073"><msup><mrow/><mrow><mo>+</mo></mrow></msup></math>, UF1,2<sup loc="post">+</sup> with residual gas is observed in the ion trap. The effect of trapping time on molecular formation is presented.The use of radioactive molecules for fundamental physics research is a developing interdisciplinary field limited dominantly by their scarce availability. In this work, radioactive molecular ion beams containing actinide nuclei extracted from uranium carbide targets are produced via the Isotope Separation On-Line technique at the CERN-ISOLDE facility. Two methods of molecular beam production are studied: extraction of molecular ion beams from the ion source, and formation of molecular ions from the mass-separated ion beam in a gas-filled radio-frequency quadrupole ion trap. Ion currents of U$^+$, UO$_{1-3}^+$, UC$_{1-3}^+$, UF$_{1-4}^+$, UF$_{1,2}$O$_{1,2}^+$ are reported. Metastable tantalum and uranium fluoride molecular ions are identified. Formation of UO$_{1-3}^+$, U(OH)$_{1-3}^+$, UC$_{1-3}^+$, UF$_{1,2}$O$_{1,2}^+$ from mass-separated beams of U$^+$, UF$_{1,2}^+$ with residual gas is observed in the ion trap. The effect of trapping time on molecular formation is presented.arXiv:2303.12215oai:cds.cern.ch:28557262023-03-21
spellingShingle physics.ins-det
Detectors and Experimental Techniques
Au, M.
Athanasakis-Kaklamanakis, M.
Nies, L.
Ballof, J.
Berger, R.
Chrysalidis, K.
Fischer, P.
Heinke, R.
Johnson, J.
Köster, U.
Leimbach, D.
Marsh, B.
Mougeot, M.
Reich, B.
Reilly, J.
Reis, E.
Schlaich, M.
Schweiger, Ch.
Schweikhard, L.
Stegemann, S.
Wessolek, J.
Wienholtz, F.
Wilkins, S.G.
Wojtaczka, W.
Düllmann, Ch.E.
Rothe, S.
In-source and in-trap formation of molecular ions in the actinide mass range at CERN-ISOLDE
title In-source and in-trap formation of molecular ions in the actinide mass range at CERN-ISOLDE
title_full In-source and in-trap formation of molecular ions in the actinide mass range at CERN-ISOLDE
title_fullStr In-source and in-trap formation of molecular ions in the actinide mass range at CERN-ISOLDE
title_full_unstemmed In-source and in-trap formation of molecular ions in the actinide mass range at CERN-ISOLDE
title_short In-source and in-trap formation of molecular ions in the actinide mass range at CERN-ISOLDE
title_sort in-source and in-trap formation of molecular ions in the actinide mass range at cern-isolde
topic physics.ins-det
Detectors and Experimental Techniques
url https://dx.doi.org/10.1016/j.nimb.2023.05.015
http://cds.cern.ch/record/2855726
work_keys_str_mv AT aum insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT athanasakiskaklamanakism insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT niesl insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT ballofj insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT bergerr insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT chrysalidisk insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT fischerp insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT heinker insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT johnsonj insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT kosteru insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT leimbachd insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT marshb insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT mougeotm insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT reichb insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT reillyj insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT reise insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT schlaichm insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT schweigerch insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT schweikhardl insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT stegemanns insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT wessolekj insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT wienholtzf insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT wilkinssg insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT wojtaczkaw insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT dullmannche insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde
AT rothes insourceandintrapformationofmolecularionsintheactinidemassrangeatcernisolde