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Characterization of positive clusters in the CLOUD nucleation experiments

The mechanism of new particle formation (NPF) events is still poorly understood. The CLOUD experiment is studying at which conditions this process occurs. During the CLOUD 7 campaign (fall 2012) the evolution of the nucleation rate with different reagents (sulphuric acid, ammonia, dimethylamine and...

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Detalles Bibliográficos
Autores principales: Bianchi, Federico, Tröstl, Jasmin, Schobesberger, Siegfried, Junninen, Heikki, Dommen, Josef, Worsnop, Douglas R, Baltensperger, Urs
Lenguaje:eng
Publicado: 2013
Materias:
Acceso en línea:https://dx.doi.org/10.1063/1.4803274
http://cds.cern.ch/record/2298171
Descripción
Sumario:The mechanism of new particle formation (NPF) events is still poorly understood. The CLOUD experiment is studying at which conditions this process occurs. During the CLOUD 7 campaign (fall 2012) the evolution of the nucleation rate with different reagents (sulphuric acid, ammonia, dimethylamine and α-pinene) was tested. Here we investigate the composition of freshly formed positive ions during the nucleation process, which allows us to understand the formation mechanisms of these clusters. The time evolution of the clusters is shown demonstrating the correlation between the formation of these clusters and the nucleation process.