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Perovskite quantum dot one-dimensional topological laser

Various topological laser concepts have recently enabled the demonstration of robust light-emitting devices that are immune to structural deformations and tolerant to fabrication imperfections. Current realizations of photonic cavities with topological boundaries are often limited by outcoupling iss...

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Autores principales: Tian, Jingyi, Tan, Qi Ying, Wang, Yutao, Yang, Yihao, Yuan, Guanghui, Adamo, Giorgio, Soci, Cesare
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10015034/
https://www.ncbi.nlm.nih.gov/pubmed/36918559
http://dx.doi.org/10.1038/s41467-023-36963-6
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author Tian, Jingyi
Tan, Qi Ying
Wang, Yutao
Yang, Yihao
Yuan, Guanghui
Adamo, Giorgio
Soci, Cesare
author_facet Tian, Jingyi
Tan, Qi Ying
Wang, Yutao
Yang, Yihao
Yuan, Guanghui
Adamo, Giorgio
Soci, Cesare
author_sort Tian, Jingyi
collection PubMed
description Various topological laser concepts have recently enabled the demonstration of robust light-emitting devices that are immune to structural deformations and tolerant to fabrication imperfections. Current realizations of photonic cavities with topological boundaries are often limited by outcoupling issues or poor directionality and require complex design and fabrication that hinder operation at small wavelengths. Here we propose a topological cavity design based on interface states between two one-dimensional photonic crystals with distinct Zak phases. Using a few monolayers of solution-processed all-inorganic cesium lead halide perovskite quantum dots as the ultrathin gain medium, we demonstrate a lithography-free, vertical-emitting, low-threshold, and single-mode laser emitting in the green. We show that the topological laser, akin to vertical-cavity surface-emitting lasers (VCSELs), is robust against local perturbations of the multilayer structure. We argue that the design simplicity and reduction of the gain medium thickness enabled by the topological cavity make this architecture suitable for low-cost and efficient quantum dot vertical emitting lasers operating across the visible spectral region.
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spelling pubmed-100150342023-03-16 Perovskite quantum dot one-dimensional topological laser Tian, Jingyi Tan, Qi Ying Wang, Yutao Yang, Yihao Yuan, Guanghui Adamo, Giorgio Soci, Cesare Nat Commun Article Various topological laser concepts have recently enabled the demonstration of robust light-emitting devices that are immune to structural deformations and tolerant to fabrication imperfections. Current realizations of photonic cavities with topological boundaries are often limited by outcoupling issues or poor directionality and require complex design and fabrication that hinder operation at small wavelengths. Here we propose a topological cavity design based on interface states between two one-dimensional photonic crystals with distinct Zak phases. Using a few monolayers of solution-processed all-inorganic cesium lead halide perovskite quantum dots as the ultrathin gain medium, we demonstrate a lithography-free, vertical-emitting, low-threshold, and single-mode laser emitting in the green. We show that the topological laser, akin to vertical-cavity surface-emitting lasers (VCSELs), is robust against local perturbations of the multilayer structure. We argue that the design simplicity and reduction of the gain medium thickness enabled by the topological cavity make this architecture suitable for low-cost and efficient quantum dot vertical emitting lasers operating across the visible spectral region. Nature Publishing Group UK 2023-03-15 /pmc/articles/PMC10015034/ /pubmed/36918559 http://dx.doi.org/10.1038/s41467-023-36963-6 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Tian, Jingyi
Tan, Qi Ying
Wang, Yutao
Yang, Yihao
Yuan, Guanghui
Adamo, Giorgio
Soci, Cesare
Perovskite quantum dot one-dimensional topological laser
title Perovskite quantum dot one-dimensional topological laser
title_full Perovskite quantum dot one-dimensional topological laser
title_fullStr Perovskite quantum dot one-dimensional topological laser
title_full_unstemmed Perovskite quantum dot one-dimensional topological laser
title_short Perovskite quantum dot one-dimensional topological laser
title_sort perovskite quantum dot one-dimensional topological laser
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10015034/
https://www.ncbi.nlm.nih.gov/pubmed/36918559
http://dx.doi.org/10.1038/s41467-023-36963-6
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