Cargando…

Effect of Gas Diffusion Layer Notch Arrangement and Gradient Depth on the Performance of Proton Exchange Membrane Fuel Cells in the Serpentine Flow Field

[Image: see text] The structure of the gas diffusion layer (GDL) of a proton exchange membrane fuel cell (PEMFC) affects the transfer of the reaction gas and the water flooding phenomenon. First, the three-dimensional numerical model of the GDL was reconstructed by the stochastic reconstruction meth...

Descripción completa

Detalles Bibliográficos
Autores principales: Zhang, Heng, Zhang, Lili, Zhang, Yongliang, Hou, Zhanju, Liu, Jian
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10034774/
https://www.ncbi.nlm.nih.gov/pubmed/36969400
http://dx.doi.org/10.1021/acsomega.2c07632
_version_ 1784911279591260160
author Zhang, Heng
Zhang, Lili
Zhang, Yongliang
Hou, Zhanju
Liu, Jian
author_facet Zhang, Heng
Zhang, Lili
Zhang, Yongliang
Hou, Zhanju
Liu, Jian
author_sort Zhang, Heng
collection PubMed
description [Image: see text] The structure of the gas diffusion layer (GDL) of a proton exchange membrane fuel cell (PEMFC) affects the transfer of the reaction gas and the water flooding phenomenon. First, the three-dimensional numerical model of the GDL was reconstructed by the stochastic reconstruction method, and the kinetic behaviors of liquid water in the conventional GDL, circular groove GDL, and elliptical groove GDL were compared and analyzed, based on which the liquid water penetration time, the effective diffusion rate of oxygen, and relative permeability of water in the three GDLs were analyzed, and the results of the study found that the circular groove GDL had the best drainage effect. Second, based on the PEMFC with serpentine channels, an electrochemical model of the GDL with circular grooves was arranged in the flow field, and the effects of the groove depth distribution and center spacing of circular grooves on its performance were numerically investigated. It was found that the presence of circular grooves enhanced the transfer rate of reactants from the GDL to the catalytic layer and increased the current density. Oxygen concentration uniformity and under-rib convection were enhanced when the groove depth was designed to have a power function distribution with an exponent close to 1, effectively reducing flooding. The best drainage effect was achieved when the groove spacing was 2 mm, and also the cell performance was more stable.
format Online
Article
Text
id pubmed-10034774
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher American Chemical Society
record_format MEDLINE/PubMed
spelling pubmed-100347742023-03-24 Effect of Gas Diffusion Layer Notch Arrangement and Gradient Depth on the Performance of Proton Exchange Membrane Fuel Cells in the Serpentine Flow Field Zhang, Heng Zhang, Lili Zhang, Yongliang Hou, Zhanju Liu, Jian ACS Omega [Image: see text] The structure of the gas diffusion layer (GDL) of a proton exchange membrane fuel cell (PEMFC) affects the transfer of the reaction gas and the water flooding phenomenon. First, the three-dimensional numerical model of the GDL was reconstructed by the stochastic reconstruction method, and the kinetic behaviors of liquid water in the conventional GDL, circular groove GDL, and elliptical groove GDL were compared and analyzed, based on which the liquid water penetration time, the effective diffusion rate of oxygen, and relative permeability of water in the three GDLs were analyzed, and the results of the study found that the circular groove GDL had the best drainage effect. Second, based on the PEMFC with serpentine channels, an electrochemical model of the GDL with circular grooves was arranged in the flow field, and the effects of the groove depth distribution and center spacing of circular grooves on its performance were numerically investigated. It was found that the presence of circular grooves enhanced the transfer rate of reactants from the GDL to the catalytic layer and increased the current density. Oxygen concentration uniformity and under-rib convection were enhanced when the groove depth was designed to have a power function distribution with an exponent close to 1, effectively reducing flooding. The best drainage effect was achieved when the groove spacing was 2 mm, and also the cell performance was more stable. American Chemical Society 2023-03-08 /pmc/articles/PMC10034774/ /pubmed/36969400 http://dx.doi.org/10.1021/acsomega.2c07632 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Zhang, Heng
Zhang, Lili
Zhang, Yongliang
Hou, Zhanju
Liu, Jian
Effect of Gas Diffusion Layer Notch Arrangement and Gradient Depth on the Performance of Proton Exchange Membrane Fuel Cells in the Serpentine Flow Field
title Effect of Gas Diffusion Layer Notch Arrangement and Gradient Depth on the Performance of Proton Exchange Membrane Fuel Cells in the Serpentine Flow Field
title_full Effect of Gas Diffusion Layer Notch Arrangement and Gradient Depth on the Performance of Proton Exchange Membrane Fuel Cells in the Serpentine Flow Field
title_fullStr Effect of Gas Diffusion Layer Notch Arrangement and Gradient Depth on the Performance of Proton Exchange Membrane Fuel Cells in the Serpentine Flow Field
title_full_unstemmed Effect of Gas Diffusion Layer Notch Arrangement and Gradient Depth on the Performance of Proton Exchange Membrane Fuel Cells in the Serpentine Flow Field
title_short Effect of Gas Diffusion Layer Notch Arrangement and Gradient Depth on the Performance of Proton Exchange Membrane Fuel Cells in the Serpentine Flow Field
title_sort effect of gas diffusion layer notch arrangement and gradient depth on the performance of proton exchange membrane fuel cells in the serpentine flow field
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10034774/
https://www.ncbi.nlm.nih.gov/pubmed/36969400
http://dx.doi.org/10.1021/acsomega.2c07632
work_keys_str_mv AT zhangheng effectofgasdiffusionlayernotcharrangementandgradientdepthontheperformanceofprotonexchangemembranefuelcellsintheserpentineflowfield
AT zhanglili effectofgasdiffusionlayernotcharrangementandgradientdepthontheperformanceofprotonexchangemembranefuelcellsintheserpentineflowfield
AT zhangyongliang effectofgasdiffusionlayernotcharrangementandgradientdepthontheperformanceofprotonexchangemembranefuelcellsintheserpentineflowfield
AT houzhanju effectofgasdiffusionlayernotcharrangementandgradientdepthontheperformanceofprotonexchangemembranefuelcellsintheserpentineflowfield
AT liujian effectofgasdiffusionlayernotcharrangementandgradientdepthontheperformanceofprotonexchangemembranefuelcellsintheserpentineflowfield