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Effect of Gas Diffusion Layer Notch Arrangement and Gradient Depth on the Performance of Proton Exchange Membrane Fuel Cells in the Serpentine Flow Field
[Image: see text] The structure of the gas diffusion layer (GDL) of a proton exchange membrane fuel cell (PEMFC) affects the transfer of the reaction gas and the water flooding phenomenon. First, the three-dimensional numerical model of the GDL was reconstructed by the stochastic reconstruction meth...
Autores principales: | , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2023
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10034774/ https://www.ncbi.nlm.nih.gov/pubmed/36969400 http://dx.doi.org/10.1021/acsomega.2c07632 |
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author | Zhang, Heng Zhang, Lili Zhang, Yongliang Hou, Zhanju Liu, Jian |
author_facet | Zhang, Heng Zhang, Lili Zhang, Yongliang Hou, Zhanju Liu, Jian |
author_sort | Zhang, Heng |
collection | PubMed |
description | [Image: see text] The structure of the gas diffusion layer (GDL) of a proton exchange membrane fuel cell (PEMFC) affects the transfer of the reaction gas and the water flooding phenomenon. First, the three-dimensional numerical model of the GDL was reconstructed by the stochastic reconstruction method, and the kinetic behaviors of liquid water in the conventional GDL, circular groove GDL, and elliptical groove GDL were compared and analyzed, based on which the liquid water penetration time, the effective diffusion rate of oxygen, and relative permeability of water in the three GDLs were analyzed, and the results of the study found that the circular groove GDL had the best drainage effect. Second, based on the PEMFC with serpentine channels, an electrochemical model of the GDL with circular grooves was arranged in the flow field, and the effects of the groove depth distribution and center spacing of circular grooves on its performance were numerically investigated. It was found that the presence of circular grooves enhanced the transfer rate of reactants from the GDL to the catalytic layer and increased the current density. Oxygen concentration uniformity and under-rib convection were enhanced when the groove depth was designed to have a power function distribution with an exponent close to 1, effectively reducing flooding. The best drainage effect was achieved when the groove spacing was 2 mm, and also the cell performance was more stable. |
format | Online Article Text |
id | pubmed-10034774 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-100347742023-03-24 Effect of Gas Diffusion Layer Notch Arrangement and Gradient Depth on the Performance of Proton Exchange Membrane Fuel Cells in the Serpentine Flow Field Zhang, Heng Zhang, Lili Zhang, Yongliang Hou, Zhanju Liu, Jian ACS Omega [Image: see text] The structure of the gas diffusion layer (GDL) of a proton exchange membrane fuel cell (PEMFC) affects the transfer of the reaction gas and the water flooding phenomenon. First, the three-dimensional numerical model of the GDL was reconstructed by the stochastic reconstruction method, and the kinetic behaviors of liquid water in the conventional GDL, circular groove GDL, and elliptical groove GDL were compared and analyzed, based on which the liquid water penetration time, the effective diffusion rate of oxygen, and relative permeability of water in the three GDLs were analyzed, and the results of the study found that the circular groove GDL had the best drainage effect. Second, based on the PEMFC with serpentine channels, an electrochemical model of the GDL with circular grooves was arranged in the flow field, and the effects of the groove depth distribution and center spacing of circular grooves on its performance were numerically investigated. It was found that the presence of circular grooves enhanced the transfer rate of reactants from the GDL to the catalytic layer and increased the current density. Oxygen concentration uniformity and under-rib convection were enhanced when the groove depth was designed to have a power function distribution with an exponent close to 1, effectively reducing flooding. The best drainage effect was achieved when the groove spacing was 2 mm, and also the cell performance was more stable. American Chemical Society 2023-03-08 /pmc/articles/PMC10034774/ /pubmed/36969400 http://dx.doi.org/10.1021/acsomega.2c07632 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/). |
spellingShingle | Zhang, Heng Zhang, Lili Zhang, Yongliang Hou, Zhanju Liu, Jian Effect of Gas Diffusion Layer Notch Arrangement and Gradient Depth on the Performance of Proton Exchange Membrane Fuel Cells in the Serpentine Flow Field |
title | Effect of Gas Diffusion Layer Notch Arrangement and
Gradient Depth on the Performance of Proton Exchange Membrane Fuel
Cells in the Serpentine Flow Field |
title_full | Effect of Gas Diffusion Layer Notch Arrangement and
Gradient Depth on the Performance of Proton Exchange Membrane Fuel
Cells in the Serpentine Flow Field |
title_fullStr | Effect of Gas Diffusion Layer Notch Arrangement and
Gradient Depth on the Performance of Proton Exchange Membrane Fuel
Cells in the Serpentine Flow Field |
title_full_unstemmed | Effect of Gas Diffusion Layer Notch Arrangement and
Gradient Depth on the Performance of Proton Exchange Membrane Fuel
Cells in the Serpentine Flow Field |
title_short | Effect of Gas Diffusion Layer Notch Arrangement and
Gradient Depth on the Performance of Proton Exchange Membrane Fuel
Cells in the Serpentine Flow Field |
title_sort | effect of gas diffusion layer notch arrangement and
gradient depth on the performance of proton exchange membrane fuel
cells in the serpentine flow field |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10034774/ https://www.ncbi.nlm.nih.gov/pubmed/36969400 http://dx.doi.org/10.1021/acsomega.2c07632 |
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