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Electronical Conductivity Improvement of Carbon-Based Slurry Electrodes Using Carbon Foams for Enhanced Performance in Advanced Electrochemical Energy Storage Systems

[Image: see text] In this work, the novel idea of using a carbon foam to improve slurry electrode systems’ electronic and ionic conductivities is introduced and experimentally investigated. Slurries with different mass loadings of 5, 10, and 15 wt % are prepared using steam-activated Norit (from pea...

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Autores principales: Mourshed, Monjur, Rezaei Niya, Seyed Mohammad, Shabani, Bahman
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10034989/
https://www.ncbi.nlm.nih.gov/pubmed/36969409
http://dx.doi.org/10.1021/acsomega.3c00278
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author Mourshed, Monjur
Rezaei Niya, Seyed Mohammad
Shabani, Bahman
author_facet Mourshed, Monjur
Rezaei Niya, Seyed Mohammad
Shabani, Bahman
author_sort Mourshed, Monjur
collection PubMed
description [Image: see text] In this work, the novel idea of using a carbon foam to improve slurry electrode systems’ electronic and ionic conductivities is introduced and experimentally investigated. Slurries with different mass loadings of 5, 10, and 15 wt % are prepared using steam-activated Norit (from peat) as an active charge carrier with 1 M H(2)SO(4) and distilled water for specifically analyzing the electronic conductivity. A single-pass rectangular flow channel is used in this slurry system, where the channel width is varied from 4.1 to 2.6 cm by changing the current collectors’ position and slurry flowing from zero (static) to a maximum of 240 mL·min(–1). Carbon foams with two different thicknesses of 10 and 6.5 mm and two different pore sizes of 10 pores per inch (PPI) and 5 PPI are used for this investigation. It is observed that application of the carbon foam improves slurry conductivity; with a 10 mm thick, 10 PPI carbon foam, maximum increases of 204% in electronic conductivity and 23% in ionic conductivity are observed for water-based and acid-based slurries, respectively.
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spelling pubmed-100349892023-03-24 Electronical Conductivity Improvement of Carbon-Based Slurry Electrodes Using Carbon Foams for Enhanced Performance in Advanced Electrochemical Energy Storage Systems Mourshed, Monjur Rezaei Niya, Seyed Mohammad Shabani, Bahman ACS Omega [Image: see text] In this work, the novel idea of using a carbon foam to improve slurry electrode systems’ electronic and ionic conductivities is introduced and experimentally investigated. Slurries with different mass loadings of 5, 10, and 15 wt % are prepared using steam-activated Norit (from peat) as an active charge carrier with 1 M H(2)SO(4) and distilled water for specifically analyzing the electronic conductivity. A single-pass rectangular flow channel is used in this slurry system, where the channel width is varied from 4.1 to 2.6 cm by changing the current collectors’ position and slurry flowing from zero (static) to a maximum of 240 mL·min(–1). Carbon foams with two different thicknesses of 10 and 6.5 mm and two different pore sizes of 10 pores per inch (PPI) and 5 PPI are used for this investigation. It is observed that application of the carbon foam improves slurry conductivity; with a 10 mm thick, 10 PPI carbon foam, maximum increases of 204% in electronic conductivity and 23% in ionic conductivity are observed for water-based and acid-based slurries, respectively. American Chemical Society 2023-03-09 /pmc/articles/PMC10034989/ /pubmed/36969409 http://dx.doi.org/10.1021/acsomega.3c00278 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Mourshed, Monjur
Rezaei Niya, Seyed Mohammad
Shabani, Bahman
Electronical Conductivity Improvement of Carbon-Based Slurry Electrodes Using Carbon Foams for Enhanced Performance in Advanced Electrochemical Energy Storage Systems
title Electronical Conductivity Improvement of Carbon-Based Slurry Electrodes Using Carbon Foams for Enhanced Performance in Advanced Electrochemical Energy Storage Systems
title_full Electronical Conductivity Improvement of Carbon-Based Slurry Electrodes Using Carbon Foams for Enhanced Performance in Advanced Electrochemical Energy Storage Systems
title_fullStr Electronical Conductivity Improvement of Carbon-Based Slurry Electrodes Using Carbon Foams for Enhanced Performance in Advanced Electrochemical Energy Storage Systems
title_full_unstemmed Electronical Conductivity Improvement of Carbon-Based Slurry Electrodes Using Carbon Foams for Enhanced Performance in Advanced Electrochemical Energy Storage Systems
title_short Electronical Conductivity Improvement of Carbon-Based Slurry Electrodes Using Carbon Foams for Enhanced Performance in Advanced Electrochemical Energy Storage Systems
title_sort electronical conductivity improvement of carbon-based slurry electrodes using carbon foams for enhanced performance in advanced electrochemical energy storage systems
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10034989/
https://www.ncbi.nlm.nih.gov/pubmed/36969409
http://dx.doi.org/10.1021/acsomega.3c00278
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