Cargando…

Continuous manufacturing of highly stable lead halide perovskite nanocrystals via a dual-reactor strategy

Lead halide perovskite nanocrystals possess incredible potential as next generation emitters due to their stellar set of optoelectronic properties. Unfortunately, their instability towards many ambient conditions and reliance on batch processing hinder their widespread utilities. Herein, we address...

Descripción completa

Detalles Bibliográficos
Autores principales: Liang, Shuang, Biesold, Gill M., Zhuang, Mingyue, Kang, Zhitao, Wagner, Brent, Lin, Zhiqun
Formato: Online Artículo Texto
Lenguaje:English
Publicado: RSC 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10044306/
https://www.ncbi.nlm.nih.gov/pubmed/36998667
http://dx.doi.org/10.1039/d2na00744d
_version_ 1784913329310924800
author Liang, Shuang
Biesold, Gill M.
Zhuang, Mingyue
Kang, Zhitao
Wagner, Brent
Lin, Zhiqun
author_facet Liang, Shuang
Biesold, Gill M.
Zhuang, Mingyue
Kang, Zhitao
Wagner, Brent
Lin, Zhiqun
author_sort Liang, Shuang
collection PubMed
description Lead halide perovskite nanocrystals possess incredible potential as next generation emitters due to their stellar set of optoelectronic properties. Unfortunately, their instability towards many ambient conditions and reliance on batch processing hinder their widespread utilities. Herein, we address both challenges by continuously synthesizing highly stable perovskite nanocrystals via integrating star-like block copolymer nanoreactors into a house-built flow reactor. Perovskite nanocrystals manufactured in this strategy display significantly enhanced colloidal, UV, and thermal stabilities over those synthesized with conventional ligands. Such scaling up of highly stable perovskite nanocrystals represents an important step towards their eventual use in many practical applications in optoelectronic materials and devices.
format Online
Article
Text
id pubmed-10044306
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher RSC
record_format MEDLINE/PubMed
spelling pubmed-100443062023-03-29 Continuous manufacturing of highly stable lead halide perovskite nanocrystals via a dual-reactor strategy Liang, Shuang Biesold, Gill M. Zhuang, Mingyue Kang, Zhitao Wagner, Brent Lin, Zhiqun Nanoscale Adv Chemistry Lead halide perovskite nanocrystals possess incredible potential as next generation emitters due to their stellar set of optoelectronic properties. Unfortunately, their instability towards many ambient conditions and reliance on batch processing hinder their widespread utilities. Herein, we address both challenges by continuously synthesizing highly stable perovskite nanocrystals via integrating star-like block copolymer nanoreactors into a house-built flow reactor. Perovskite nanocrystals manufactured in this strategy display significantly enhanced colloidal, UV, and thermal stabilities over those synthesized with conventional ligands. Such scaling up of highly stable perovskite nanocrystals represents an important step towards their eventual use in many practical applications in optoelectronic materials and devices. RSC 2023-03-08 /pmc/articles/PMC10044306/ /pubmed/36998667 http://dx.doi.org/10.1039/d2na00744d Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Liang, Shuang
Biesold, Gill M.
Zhuang, Mingyue
Kang, Zhitao
Wagner, Brent
Lin, Zhiqun
Continuous manufacturing of highly stable lead halide perovskite nanocrystals via a dual-reactor strategy
title Continuous manufacturing of highly stable lead halide perovskite nanocrystals via a dual-reactor strategy
title_full Continuous manufacturing of highly stable lead halide perovskite nanocrystals via a dual-reactor strategy
title_fullStr Continuous manufacturing of highly stable lead halide perovskite nanocrystals via a dual-reactor strategy
title_full_unstemmed Continuous manufacturing of highly stable lead halide perovskite nanocrystals via a dual-reactor strategy
title_short Continuous manufacturing of highly stable lead halide perovskite nanocrystals via a dual-reactor strategy
title_sort continuous manufacturing of highly stable lead halide perovskite nanocrystals via a dual-reactor strategy
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10044306/
https://www.ncbi.nlm.nih.gov/pubmed/36998667
http://dx.doi.org/10.1039/d2na00744d
work_keys_str_mv AT liangshuang continuousmanufacturingofhighlystableleadhalideperovskitenanocrystalsviaadualreactorstrategy
AT biesoldgillm continuousmanufacturingofhighlystableleadhalideperovskitenanocrystalsviaadualreactorstrategy
AT zhuangmingyue continuousmanufacturingofhighlystableleadhalideperovskitenanocrystalsviaadualreactorstrategy
AT kangzhitao continuousmanufacturingofhighlystableleadhalideperovskitenanocrystalsviaadualreactorstrategy
AT wagnerbrent continuousmanufacturingofhighlystableleadhalideperovskitenanocrystalsviaadualreactorstrategy
AT linzhiqun continuousmanufacturingofhighlystableleadhalideperovskitenanocrystalsviaadualreactorstrategy