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Temperature-Dependent Anisotropic Refractive Index in β-Ga(2)O(3): Application in Interferometric Thermometers

An accurate knowledge of the optical properties of β-Ga(2)O(3) is key to developing the full potential of this oxide for photonics applications. In particular, the dependence of these properties on temperature is still being studied. Optical micro- and nanocavities are promising for a wide range of...

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Autores principales: Carrasco, Daniel, Nieto-Pinero, Eva, Alonso-Orts, Manuel, Serna, Rosalía, San Juan, Jose M., Nó, María L., Jesenovec, Jani, McCloy, John S., Nogales, Emilio, Méndez, Bianchi
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10058191/
https://www.ncbi.nlm.nih.gov/pubmed/36986020
http://dx.doi.org/10.3390/nano13061126
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author Carrasco, Daniel
Nieto-Pinero, Eva
Alonso-Orts, Manuel
Serna, Rosalía
San Juan, Jose M.
Nó, María L.
Jesenovec, Jani
McCloy, John S.
Nogales, Emilio
Méndez, Bianchi
author_facet Carrasco, Daniel
Nieto-Pinero, Eva
Alonso-Orts, Manuel
Serna, Rosalía
San Juan, Jose M.
Nó, María L.
Jesenovec, Jani
McCloy, John S.
Nogales, Emilio
Méndez, Bianchi
author_sort Carrasco, Daniel
collection PubMed
description An accurate knowledge of the optical properties of β-Ga(2)O(3) is key to developing the full potential of this oxide for photonics applications. In particular, the dependence of these properties on temperature is still being studied. Optical micro- and nanocavities are promising for a wide range of applications. They can be created within microwires and nanowires via distributed Bragg reflectors (DBR), i.e., periodic patterns of the refractive index in dielectric materials, acting as tunable mirrors. In this work, the effect of temperature on the anisotropic refractive index of β-Ga(2)O(3) n(λ,T) was analyzed with ellipsometry in a bulk crystal, and temperature-dependent dispersion relations were obtained, with them being fitted to Sellmeier formalism in the visible range. Micro-photoluminescence (μ-PL) spectroscopy of microcavities that developed within Cr-doped β-Ga(2)O(3) nanowires shows the characteristic thermal shift of red–infrared Fabry–Perot optical resonances when excited with different laser powers. The origin of this shift is mainly related to the variation in the temperature of the refractive index. A comparison of these two experimental results was performed by finite-difference time-domain (FDTD) simulations, considering the exact morphology of the wires and the temperature-dependent, anisotropic refractive index. The shifts caused by temperature variations observed by μ-PL are similar, though slightly larger than those obtained with FDTD when implementing the n(λ,T) obtained with ellipsometry. The thermo-optic coefficient was calculated.
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spelling pubmed-100581912023-03-30 Temperature-Dependent Anisotropic Refractive Index in β-Ga(2)O(3): Application in Interferometric Thermometers Carrasco, Daniel Nieto-Pinero, Eva Alonso-Orts, Manuel Serna, Rosalía San Juan, Jose M. Nó, María L. Jesenovec, Jani McCloy, John S. Nogales, Emilio Méndez, Bianchi Nanomaterials (Basel) Article An accurate knowledge of the optical properties of β-Ga(2)O(3) is key to developing the full potential of this oxide for photonics applications. In particular, the dependence of these properties on temperature is still being studied. Optical micro- and nanocavities are promising for a wide range of applications. They can be created within microwires and nanowires via distributed Bragg reflectors (DBR), i.e., periodic patterns of the refractive index in dielectric materials, acting as tunable mirrors. In this work, the effect of temperature on the anisotropic refractive index of β-Ga(2)O(3) n(λ,T) was analyzed with ellipsometry in a bulk crystal, and temperature-dependent dispersion relations were obtained, with them being fitted to Sellmeier formalism in the visible range. Micro-photoluminescence (μ-PL) spectroscopy of microcavities that developed within Cr-doped β-Ga(2)O(3) nanowires shows the characteristic thermal shift of red–infrared Fabry–Perot optical resonances when excited with different laser powers. The origin of this shift is mainly related to the variation in the temperature of the refractive index. A comparison of these two experimental results was performed by finite-difference time-domain (FDTD) simulations, considering the exact morphology of the wires and the temperature-dependent, anisotropic refractive index. The shifts caused by temperature variations observed by μ-PL are similar, though slightly larger than those obtained with FDTD when implementing the n(λ,T) obtained with ellipsometry. The thermo-optic coefficient was calculated. MDPI 2023-03-21 /pmc/articles/PMC10058191/ /pubmed/36986020 http://dx.doi.org/10.3390/nano13061126 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Carrasco, Daniel
Nieto-Pinero, Eva
Alonso-Orts, Manuel
Serna, Rosalía
San Juan, Jose M.
Nó, María L.
Jesenovec, Jani
McCloy, John S.
Nogales, Emilio
Méndez, Bianchi
Temperature-Dependent Anisotropic Refractive Index in β-Ga(2)O(3): Application in Interferometric Thermometers
title Temperature-Dependent Anisotropic Refractive Index in β-Ga(2)O(3): Application in Interferometric Thermometers
title_full Temperature-Dependent Anisotropic Refractive Index in β-Ga(2)O(3): Application in Interferometric Thermometers
title_fullStr Temperature-Dependent Anisotropic Refractive Index in β-Ga(2)O(3): Application in Interferometric Thermometers
title_full_unstemmed Temperature-Dependent Anisotropic Refractive Index in β-Ga(2)O(3): Application in Interferometric Thermometers
title_short Temperature-Dependent Anisotropic Refractive Index in β-Ga(2)O(3): Application in Interferometric Thermometers
title_sort temperature-dependent anisotropic refractive index in β-ga(2)o(3): application in interferometric thermometers
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10058191/
https://www.ncbi.nlm.nih.gov/pubmed/36986020
http://dx.doi.org/10.3390/nano13061126
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