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Estimates of Future New Particle Formation under Different Emission Scenarios in Beijing

[Image: see text] New particle formation (NPF) is a leading source of particulate matter by number and a contributor to particle mass during haze events. Reductions in emissions of air pollutants, many of which are NPF precursors, are expected in the move toward carbon neutrality or net-zero. Expect...

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Autores principales: Brean, James, Rowell, Alex, Beddows, David C. S., Shi, Zongbo, Harrison, Roy M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10061929/
https://www.ncbi.nlm.nih.gov/pubmed/36930743
http://dx.doi.org/10.1021/acs.est.2c08348
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author Brean, James
Rowell, Alex
Beddows, David C. S.
Shi, Zongbo
Harrison, Roy M.
author_facet Brean, James
Rowell, Alex
Beddows, David C. S.
Shi, Zongbo
Harrison, Roy M.
author_sort Brean, James
collection PubMed
description [Image: see text] New particle formation (NPF) is a leading source of particulate matter by number and a contributor to particle mass during haze events. Reductions in emissions of air pollutants, many of which are NPF precursors, are expected in the move toward carbon neutrality or net-zero. Expected changes to pollutant emissions are used to investigate future changes to NPF processes, in comparison to a simulation of current conditions. The projected changes to SO(2) emissions are key in changing future NPF number, with different scenarios producing either a doubling or near total reduction in sulfuric acid-amine particle formation rates. Particle growth rates are projected to change little in all but the strictest emission control scenarios. These changes will reduce the particle mass arising by NPF substantially, thus showing a further cobenefit of net-zero policies. Major uncertainties remain in future NPF including the volatility of oxygenated organic molecules resulting from changes to NO(x) and amine emissions.
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spelling pubmed-100619292023-03-31 Estimates of Future New Particle Formation under Different Emission Scenarios in Beijing Brean, James Rowell, Alex Beddows, David C. S. Shi, Zongbo Harrison, Roy M. Environ Sci Technol [Image: see text] New particle formation (NPF) is a leading source of particulate matter by number and a contributor to particle mass during haze events. Reductions in emissions of air pollutants, many of which are NPF precursors, are expected in the move toward carbon neutrality or net-zero. Expected changes to pollutant emissions are used to investigate future changes to NPF processes, in comparison to a simulation of current conditions. The projected changes to SO(2) emissions are key in changing future NPF number, with different scenarios producing either a doubling or near total reduction in sulfuric acid-amine particle formation rates. Particle growth rates are projected to change little in all but the strictest emission control scenarios. These changes will reduce the particle mass arising by NPF substantially, thus showing a further cobenefit of net-zero policies. Major uncertainties remain in future NPF including the volatility of oxygenated organic molecules resulting from changes to NO(x) and amine emissions. American Chemical Society 2023-03-17 /pmc/articles/PMC10061929/ /pubmed/36930743 http://dx.doi.org/10.1021/acs.est.2c08348 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Brean, James
Rowell, Alex
Beddows, David C. S.
Shi, Zongbo
Harrison, Roy M.
Estimates of Future New Particle Formation under Different Emission Scenarios in Beijing
title Estimates of Future New Particle Formation under Different Emission Scenarios in Beijing
title_full Estimates of Future New Particle Formation under Different Emission Scenarios in Beijing
title_fullStr Estimates of Future New Particle Formation under Different Emission Scenarios in Beijing
title_full_unstemmed Estimates of Future New Particle Formation under Different Emission Scenarios in Beijing
title_short Estimates of Future New Particle Formation under Different Emission Scenarios in Beijing
title_sort estimates of future new particle formation under different emission scenarios in beijing
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10061929/
https://www.ncbi.nlm.nih.gov/pubmed/36930743
http://dx.doi.org/10.1021/acs.est.2c08348
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