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Absolute environmental sustainability assessment of renewable dimethyl ether fuelled heavy-duty trucks

In recent years, liquid fuels from renewable carbon that can replace fossil ones with minimal infrastructure changes have attracted increasing interest in decarbonising the heavy-duty long-haul sector. Here we focus on dimethyl ether (DME), a promising alternative to diesel due to its high cetane nu...

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Autores principales: Charalambous, Margarita A., Tulus, Victor, Ryberg, Morten W., Pérez-Ramírez, Javier, Guillén-Gosálbez, Gonzalo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10089250/
https://www.ncbi.nlm.nih.gov/pubmed/37063612
http://dx.doi.org/10.1039/d2se01409b
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author Charalambous, Margarita A.
Tulus, Victor
Ryberg, Morten W.
Pérez-Ramírez, Javier
Guillén-Gosálbez, Gonzalo
author_facet Charalambous, Margarita A.
Tulus, Victor
Ryberg, Morten W.
Pérez-Ramírez, Javier
Guillén-Gosálbez, Gonzalo
author_sort Charalambous, Margarita A.
collection PubMed
description In recent years, liquid fuels from renewable carbon that can replace fossil ones with minimal infrastructure changes have attracted increasing interest in decarbonising the heavy-duty long-haul sector. Here we focus on dimethyl ether (DME), a promising alternative to diesel due to its high cetane number, oxygen content, and more efficient and cleaner propulsion that results in low particulate matter and sulphur oxide emissions. Going well beyond previous studies that quantified the environmental impact of DME, often in terms of global warming, here we evaluate DME use in heavy-duty trucks in the context of seven planetary boundaries, all essential for maintaining the Earth's stability. Focusing on several scenarios differing in the feedstock origin, we find that routes based on fossil carbon, either in the form of coal, natural gas, or captured CO(2) from fossil plants, would increase the greenhouse gas emissions relative to the business-as-usual. Only scenarios based on renewable carbon could reduce the impacts on climate change, while hydrogen from biomass gasification coupled with carbon capture and storage (CCS) and DME from biomass gasification with CCS could enable an environmentally sustainable operation within all the planetary boundaries. Overall, our work opens up new avenues for the environmental assessment of fuels considering the finite capacity of the Earth system to guide research and policy-making more sensibly.
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spelling pubmed-100892502023-04-12 Absolute environmental sustainability assessment of renewable dimethyl ether fuelled heavy-duty trucks Charalambous, Margarita A. Tulus, Victor Ryberg, Morten W. Pérez-Ramírez, Javier Guillén-Gosálbez, Gonzalo Sustain Energy Fuels Chemistry In recent years, liquid fuels from renewable carbon that can replace fossil ones with minimal infrastructure changes have attracted increasing interest in decarbonising the heavy-duty long-haul sector. Here we focus on dimethyl ether (DME), a promising alternative to diesel due to its high cetane number, oxygen content, and more efficient and cleaner propulsion that results in low particulate matter and sulphur oxide emissions. Going well beyond previous studies that quantified the environmental impact of DME, often in terms of global warming, here we evaluate DME use in heavy-duty trucks in the context of seven planetary boundaries, all essential for maintaining the Earth's stability. Focusing on several scenarios differing in the feedstock origin, we find that routes based on fossil carbon, either in the form of coal, natural gas, or captured CO(2) from fossil plants, would increase the greenhouse gas emissions relative to the business-as-usual. Only scenarios based on renewable carbon could reduce the impacts on climate change, while hydrogen from biomass gasification coupled with carbon capture and storage (CCS) and DME from biomass gasification with CCS could enable an environmentally sustainable operation within all the planetary boundaries. Overall, our work opens up new avenues for the environmental assessment of fuels considering the finite capacity of the Earth system to guide research and policy-making more sensibly. The Royal Society of Chemistry 2023-03-07 /pmc/articles/PMC10089250/ /pubmed/37063612 http://dx.doi.org/10.1039/d2se01409b Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Charalambous, Margarita A.
Tulus, Victor
Ryberg, Morten W.
Pérez-Ramírez, Javier
Guillén-Gosálbez, Gonzalo
Absolute environmental sustainability assessment of renewable dimethyl ether fuelled heavy-duty trucks
title Absolute environmental sustainability assessment of renewable dimethyl ether fuelled heavy-duty trucks
title_full Absolute environmental sustainability assessment of renewable dimethyl ether fuelled heavy-duty trucks
title_fullStr Absolute environmental sustainability assessment of renewable dimethyl ether fuelled heavy-duty trucks
title_full_unstemmed Absolute environmental sustainability assessment of renewable dimethyl ether fuelled heavy-duty trucks
title_short Absolute environmental sustainability assessment of renewable dimethyl ether fuelled heavy-duty trucks
title_sort absolute environmental sustainability assessment of renewable dimethyl ether fuelled heavy-duty trucks
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10089250/
https://www.ncbi.nlm.nih.gov/pubmed/37063612
http://dx.doi.org/10.1039/d2se01409b
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