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Recent Advances in Manganese-Based Materials for Electrolytic Water Splitting

Developing earth-abundant and highly effective electrocatalysts for electrocatalytic water splitting is a prerequisite for the upcoming hydrogen energy society. Recently, manganese-based materials have been one of the most promising candidates to replace noble metal catalysts due to their natural ab...

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Detalles Bibliográficos
Autores principales: Hu, Jing, Zhou, Yuru, Liu, Yinan, Xu, Zhichao, Li, Haijin
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10095233/
https://www.ncbi.nlm.nih.gov/pubmed/37047832
http://dx.doi.org/10.3390/ijms24076861
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author Hu, Jing
Zhou, Yuru
Liu, Yinan
Xu, Zhichao
Li, Haijin
author_facet Hu, Jing
Zhou, Yuru
Liu, Yinan
Xu, Zhichao
Li, Haijin
author_sort Hu, Jing
collection PubMed
description Developing earth-abundant and highly effective electrocatalysts for electrocatalytic water splitting is a prerequisite for the upcoming hydrogen energy society. Recently, manganese-based materials have been one of the most promising candidates to replace noble metal catalysts due to their natural abundance, low cost, adjustable electronic properties, and excellent chemical stability. Although some achievements have been made in the past decades, their performance is still far lower than that of Pt. Therefore, further research is needed to improve the performance of manganese-based catalytic materials. In this review, we summarize the research progress on the application of manganese-based materials as catalysts for electrolytic water splitting. We first introduce the mechanism of electrocatalytic water decomposition using a manganese-based electrocatalyst. We then thoroughly discuss the optimization strategy used to enhance the catalytic activity of manganese-based electrocatalysts, including doping and defect engineering, interface engineering, and phase engineering. Finally, we present several future design opportunities for highly efficient manganese-based electrocatalysts.
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spelling pubmed-100952332023-04-13 Recent Advances in Manganese-Based Materials for Electrolytic Water Splitting Hu, Jing Zhou, Yuru Liu, Yinan Xu, Zhichao Li, Haijin Int J Mol Sci Review Developing earth-abundant and highly effective electrocatalysts for electrocatalytic water splitting is a prerequisite for the upcoming hydrogen energy society. Recently, manganese-based materials have been one of the most promising candidates to replace noble metal catalysts due to their natural abundance, low cost, adjustable electronic properties, and excellent chemical stability. Although some achievements have been made in the past decades, their performance is still far lower than that of Pt. Therefore, further research is needed to improve the performance of manganese-based catalytic materials. In this review, we summarize the research progress on the application of manganese-based materials as catalysts for electrolytic water splitting. We first introduce the mechanism of electrocatalytic water decomposition using a manganese-based electrocatalyst. We then thoroughly discuss the optimization strategy used to enhance the catalytic activity of manganese-based electrocatalysts, including doping and defect engineering, interface engineering, and phase engineering. Finally, we present several future design opportunities for highly efficient manganese-based electrocatalysts. MDPI 2023-04-06 /pmc/articles/PMC10095233/ /pubmed/37047832 http://dx.doi.org/10.3390/ijms24076861 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Review
Hu, Jing
Zhou, Yuru
Liu, Yinan
Xu, Zhichao
Li, Haijin
Recent Advances in Manganese-Based Materials for Electrolytic Water Splitting
title Recent Advances in Manganese-Based Materials for Electrolytic Water Splitting
title_full Recent Advances in Manganese-Based Materials for Electrolytic Water Splitting
title_fullStr Recent Advances in Manganese-Based Materials for Electrolytic Water Splitting
title_full_unstemmed Recent Advances in Manganese-Based Materials for Electrolytic Water Splitting
title_short Recent Advances in Manganese-Based Materials for Electrolytic Water Splitting
title_sort recent advances in manganese-based materials for electrolytic water splitting
topic Review
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10095233/
https://www.ncbi.nlm.nih.gov/pubmed/37047832
http://dx.doi.org/10.3390/ijms24076861
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