Cargando…

Study on Preparation and Performance of CO(2) Foamed Concrete for Heat Insulation and Carbon Storage

Environmental problems caused by large amounts of CO(2) generated by coal–electricity integration bases have raised concerns. To solve these problems, this study develops a CO(2) foam concrete (CFC) material with both heat insulation and carbon fixation characteristics to realize CO(2) in situ stora...

Descripción completa

Detalles Bibliográficos
Autores principales: Ta, Xupeng, Zhang, Yuan, Wan, Zhijun, Shi, Peng, Zhou, Jiale
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10095924/
https://www.ncbi.nlm.nih.gov/pubmed/37049022
http://dx.doi.org/10.3390/ma16072725
Descripción
Sumario:Environmental problems caused by large amounts of CO(2) generated by coal–electricity integration bases have raised concerns. To solve these problems, this study develops a CO(2) foam concrete (CFC) material with both heat insulation and carbon fixation characteristics to realize CO(2) in situ storage and utilization. In this study, a Portland-cement-based CO(2) foam concrete (PC-CFC) with good thermal insulation performance and carbon fixation ability is prepared using carbonation pretreatment cement and a physical foaming method. The effects of CO(2) on the compressive strength, thermal insulation, and carbon fixation properties of PC-CFC are studied. The internal relationship between the compressive strength, thermal insulation, and carbon fixation performance of PC-CFC is analyzed, and the feasibility of PC-CFC as a filling material to realize the in situ mineralization and storage of CO(2) in the coal–electricity integration base is discussed. The experimental results show that the compressive strength of PC-CFC is significantly improved by CO(2) curing. However, CO(2) in the PC-CFC pores may weaken the strength of the pore structure, and the compressive strength decreases by 3.62% for each 1% increase in PC-CFC porosity. Using CO(2) as a foaming gas and the physical foaming method to prepare CFC can achieve improved thermal insulation performance. The thermal conductivity of PC-CFC is 0.0512–0.0905 W/(m·K). In addition, the compressive strength of PC-CFC increases by 19.08% when the thermal conductivity of PC-CFC increases by 1%. On the premise of meeting the thermal insulation requirements, PC-CFC can achieve improved compressive strength. The carbon sequestration rate of the PC-CFC skeleton is 6.1–8.57%, and the carbon storage capacity of PC-CFC pores is 1.36–2.60 kg/ton, which has obvious carbon sequestration potential; however, the preparation process and parameters of PC-CFC still require further improvement. The research results show that PC-CFC has great potential for engineering applications and is of great significance for realizing carbon reduction at the coal–electricity integration base.