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Single-particle properties of topological Wannier excitons in bismuth chalcogenide nanosheets

We analyze the topology, dispersion, and optical selection rules of bulk Wannier excitons in nanosheets of Bi(2)Se(3), a topological insulator in the family of the bismuth chalcogenides. Our main finding is that excitons also inherit the topology of the electronic bands, quantified by the skyrmion w...

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Autores principales: Maisel Licerán, Lucas, García Flórez, Francisco, Siebbeles, Laurens D. A., Stoof, Henk T. C.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10113227/
https://www.ncbi.nlm.nih.gov/pubmed/37072513
http://dx.doi.org/10.1038/s41598-023-32740-z
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author Maisel Licerán, Lucas
García Flórez, Francisco
Siebbeles, Laurens D. A.
Stoof, Henk T. C.
author_facet Maisel Licerán, Lucas
García Flórez, Francisco
Siebbeles, Laurens D. A.
Stoof, Henk T. C.
author_sort Maisel Licerán, Lucas
collection PubMed
description We analyze the topology, dispersion, and optical selection rules of bulk Wannier excitons in nanosheets of Bi(2)Se(3), a topological insulator in the family of the bismuth chalcogenides. Our main finding is that excitons also inherit the topology of the electronic bands, quantified by the skyrmion winding numbers of the constituent electron and hole pseudospins as a function of the total exciton momentum. The excitonic bands are found to be strongly indirect due to the band inversion of the underlying single-particle model. At zero total momentum, we predict that the s-wave and d-wave states of two exciton families are selectively bright under left- or right-circularly polarized light. We furthermore show that every s-wave exciton state consists of a quartet with a degenerate and quadratically dispersing nonchiral doublet, and a chiral doublet with one linearly dispersing mode as in transition metal dichalcogenides. Finally, we discuss the potential existence of topological edge states of chiral excitons arising from the bulk-boundary correspondence.
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spelling pubmed-101132272023-04-20 Single-particle properties of topological Wannier excitons in bismuth chalcogenide nanosheets Maisel Licerán, Lucas García Flórez, Francisco Siebbeles, Laurens D. A. Stoof, Henk T. C. Sci Rep Article We analyze the topology, dispersion, and optical selection rules of bulk Wannier excitons in nanosheets of Bi(2)Se(3), a topological insulator in the family of the bismuth chalcogenides. Our main finding is that excitons also inherit the topology of the electronic bands, quantified by the skyrmion winding numbers of the constituent electron and hole pseudospins as a function of the total exciton momentum. The excitonic bands are found to be strongly indirect due to the band inversion of the underlying single-particle model. At zero total momentum, we predict that the s-wave and d-wave states of two exciton families are selectively bright under left- or right-circularly polarized light. We furthermore show that every s-wave exciton state consists of a quartet with a degenerate and quadratically dispersing nonchiral doublet, and a chiral doublet with one linearly dispersing mode as in transition metal dichalcogenides. Finally, we discuss the potential existence of topological edge states of chiral excitons arising from the bulk-boundary correspondence. Nature Publishing Group UK 2023-04-18 /pmc/articles/PMC10113227/ /pubmed/37072513 http://dx.doi.org/10.1038/s41598-023-32740-z Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Maisel Licerán, Lucas
García Flórez, Francisco
Siebbeles, Laurens D. A.
Stoof, Henk T. C.
Single-particle properties of topological Wannier excitons in bismuth chalcogenide nanosheets
title Single-particle properties of topological Wannier excitons in bismuth chalcogenide nanosheets
title_full Single-particle properties of topological Wannier excitons in bismuth chalcogenide nanosheets
title_fullStr Single-particle properties of topological Wannier excitons in bismuth chalcogenide nanosheets
title_full_unstemmed Single-particle properties of topological Wannier excitons in bismuth chalcogenide nanosheets
title_short Single-particle properties of topological Wannier excitons in bismuth chalcogenide nanosheets
title_sort single-particle properties of topological wannier excitons in bismuth chalcogenide nanosheets
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10113227/
https://www.ncbi.nlm.nih.gov/pubmed/37072513
http://dx.doi.org/10.1038/s41598-023-32740-z
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