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Pressure-induced transition from a Mott insulator to a ferromagnetic Weyl metal in La(2)O(3)Fe(2)Se(2)

The insulator-metal transition in Mott insulators, known as the Mott transition, is usually accompanied with various novel quantum phenomena, such as unconventional superconductivity, non-Fermi liquid behavior and colossal magnetoresistance. Here, based on high-pressure electrical transport and XRD...

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Autores principales: Yang, Ye, Yu, Fanghang, Wen, Xikai, Gui, Zhigang, Zhang, Yuqing, Zhan, Fangyang, Wang, Rui, Ying, Jianjun, Chen, Xianhui
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10119149/
https://www.ncbi.nlm.nih.gov/pubmed/37081003
http://dx.doi.org/10.1038/s41467-023-37971-2
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author Yang, Ye
Yu, Fanghang
Wen, Xikai
Gui, Zhigang
Zhang, Yuqing
Zhan, Fangyang
Wang, Rui
Ying, Jianjun
Chen, Xianhui
author_facet Yang, Ye
Yu, Fanghang
Wen, Xikai
Gui, Zhigang
Zhang, Yuqing
Zhan, Fangyang
Wang, Rui
Ying, Jianjun
Chen, Xianhui
author_sort Yang, Ye
collection PubMed
description The insulator-metal transition in Mott insulators, known as the Mott transition, is usually accompanied with various novel quantum phenomena, such as unconventional superconductivity, non-Fermi liquid behavior and colossal magnetoresistance. Here, based on high-pressure electrical transport and XRD measurements, and first-principles calculations, we find that a unique pressure-induced Mott transition from an antiferromagnetic Mott insulator to a ferromagnetic Weyl metal in the iron oxychalcogenide La(2)O(3)Fe(2)Se(2) occurs around 37 GPa without structural phase transition. Our theoretical calculations reveal that such an insulator-metal transition is mainly due to the enlarged bandwidth and diminishing of electron correlation at high pressure, fitting well with the experimental data. Moreover, the high-pressure ferromagnetic Weyl metallic phase possesses attractive electronic band structures with six pairs of Weyl points close to the Fermi level, and its topological property can be easily manipulated by the magnetic field. The emergence of Weyl fermions in La(2)O(3)Fe(2)Se(2) at high pressure may bridge the gap between nontrivial band topology and Mott insulating states. Our findings not only realize ferromagnetic Weyl fermions associated with the Mott transition, but also suggest pressure as an effective controlling parameter to tune the emergent phenomena in correlated electron systems.
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spelling pubmed-101191492023-04-22 Pressure-induced transition from a Mott insulator to a ferromagnetic Weyl metal in La(2)O(3)Fe(2)Se(2) Yang, Ye Yu, Fanghang Wen, Xikai Gui, Zhigang Zhang, Yuqing Zhan, Fangyang Wang, Rui Ying, Jianjun Chen, Xianhui Nat Commun Article The insulator-metal transition in Mott insulators, known as the Mott transition, is usually accompanied with various novel quantum phenomena, such as unconventional superconductivity, non-Fermi liquid behavior and colossal magnetoresistance. Here, based on high-pressure electrical transport and XRD measurements, and first-principles calculations, we find that a unique pressure-induced Mott transition from an antiferromagnetic Mott insulator to a ferromagnetic Weyl metal in the iron oxychalcogenide La(2)O(3)Fe(2)Se(2) occurs around 37 GPa without structural phase transition. Our theoretical calculations reveal that such an insulator-metal transition is mainly due to the enlarged bandwidth and diminishing of electron correlation at high pressure, fitting well with the experimental data. Moreover, the high-pressure ferromagnetic Weyl metallic phase possesses attractive electronic band structures with six pairs of Weyl points close to the Fermi level, and its topological property can be easily manipulated by the magnetic field. The emergence of Weyl fermions in La(2)O(3)Fe(2)Se(2) at high pressure may bridge the gap between nontrivial band topology and Mott insulating states. Our findings not only realize ferromagnetic Weyl fermions associated with the Mott transition, but also suggest pressure as an effective controlling parameter to tune the emergent phenomena in correlated electron systems. Nature Publishing Group UK 2023-04-20 /pmc/articles/PMC10119149/ /pubmed/37081003 http://dx.doi.org/10.1038/s41467-023-37971-2 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Yang, Ye
Yu, Fanghang
Wen, Xikai
Gui, Zhigang
Zhang, Yuqing
Zhan, Fangyang
Wang, Rui
Ying, Jianjun
Chen, Xianhui
Pressure-induced transition from a Mott insulator to a ferromagnetic Weyl metal in La(2)O(3)Fe(2)Se(2)
title Pressure-induced transition from a Mott insulator to a ferromagnetic Weyl metal in La(2)O(3)Fe(2)Se(2)
title_full Pressure-induced transition from a Mott insulator to a ferromagnetic Weyl metal in La(2)O(3)Fe(2)Se(2)
title_fullStr Pressure-induced transition from a Mott insulator to a ferromagnetic Weyl metal in La(2)O(3)Fe(2)Se(2)
title_full_unstemmed Pressure-induced transition from a Mott insulator to a ferromagnetic Weyl metal in La(2)O(3)Fe(2)Se(2)
title_short Pressure-induced transition from a Mott insulator to a ferromagnetic Weyl metal in La(2)O(3)Fe(2)Se(2)
title_sort pressure-induced transition from a mott insulator to a ferromagnetic weyl metal in la(2)o(3)fe(2)se(2)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10119149/
https://www.ncbi.nlm.nih.gov/pubmed/37081003
http://dx.doi.org/10.1038/s41467-023-37971-2
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