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Spontaneous hydrogen production using gadolinium telluride

Developing materials for controlled hydrogen production through water splitting is one of the most promising ways to meet current energy demand. Here, we demonstrate spontaneous and green production of hydrogen at high evolution rate using gadolinium telluride (GdTe) under ambient conditions. The sp...

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Autores principales: Kumbhakar, Partha, Parui, Arko, Dhakar, Shikha, Paliwal, Manas, Behera, Rakesh, Gautam, Abhay Raj Singh, Roy, Soumyabrata, Ajayan, Pulickel M., Sharma, Sudhanshu, Singh, Abhishek K., Tiwary, Chandra S.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Elsevier 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10130918/
https://www.ncbi.nlm.nih.gov/pubmed/37123242
http://dx.doi.org/10.1016/j.isci.2023.106510
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author Kumbhakar, Partha
Parui, Arko
Dhakar, Shikha
Paliwal, Manas
Behera, Rakesh
Gautam, Abhay Raj Singh
Roy, Soumyabrata
Ajayan, Pulickel M.
Sharma, Sudhanshu
Singh, Abhishek K.
Tiwary, Chandra S.
author_facet Kumbhakar, Partha
Parui, Arko
Dhakar, Shikha
Paliwal, Manas
Behera, Rakesh
Gautam, Abhay Raj Singh
Roy, Soumyabrata
Ajayan, Pulickel M.
Sharma, Sudhanshu
Singh, Abhishek K.
Tiwary, Chandra S.
author_sort Kumbhakar, Partha
collection PubMed
description Developing materials for controlled hydrogen production through water splitting is one of the most promising ways to meet current energy demand. Here, we demonstrate spontaneous and green production of hydrogen at high evolution rate using gadolinium telluride (GdTe) under ambient conditions. The spent materials can be reused after melting, which regain the original activity of the pristine sample. The phase formation and reusability are supported by the thermodynamics calculations. The theoretical calculation reveals ultralow activation energy for hydrogen production using GdTe caused by charge transfer from Te to Gd. Production of highly pure and instantaneous hydrogen by GdTe could accelerate green and sustainable energy conversion technologies.
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spelling pubmed-101309182023-04-27 Spontaneous hydrogen production using gadolinium telluride Kumbhakar, Partha Parui, Arko Dhakar, Shikha Paliwal, Manas Behera, Rakesh Gautam, Abhay Raj Singh Roy, Soumyabrata Ajayan, Pulickel M. Sharma, Sudhanshu Singh, Abhishek K. Tiwary, Chandra S. iScience Article Developing materials for controlled hydrogen production through water splitting is one of the most promising ways to meet current energy demand. Here, we demonstrate spontaneous and green production of hydrogen at high evolution rate using gadolinium telluride (GdTe) under ambient conditions. The spent materials can be reused after melting, which regain the original activity of the pristine sample. The phase formation and reusability are supported by the thermodynamics calculations. The theoretical calculation reveals ultralow activation energy for hydrogen production using GdTe caused by charge transfer from Te to Gd. Production of highly pure and instantaneous hydrogen by GdTe could accelerate green and sustainable energy conversion technologies. Elsevier 2023-03-30 /pmc/articles/PMC10130918/ /pubmed/37123242 http://dx.doi.org/10.1016/j.isci.2023.106510 Text en © 2023. https://creativecommons.org/licenses/by-nc-nd/4.0/This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Article
Kumbhakar, Partha
Parui, Arko
Dhakar, Shikha
Paliwal, Manas
Behera, Rakesh
Gautam, Abhay Raj Singh
Roy, Soumyabrata
Ajayan, Pulickel M.
Sharma, Sudhanshu
Singh, Abhishek K.
Tiwary, Chandra S.
Spontaneous hydrogen production using gadolinium telluride
title Spontaneous hydrogen production using gadolinium telluride
title_full Spontaneous hydrogen production using gadolinium telluride
title_fullStr Spontaneous hydrogen production using gadolinium telluride
title_full_unstemmed Spontaneous hydrogen production using gadolinium telluride
title_short Spontaneous hydrogen production using gadolinium telluride
title_sort spontaneous hydrogen production using gadolinium telluride
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10130918/
https://www.ncbi.nlm.nih.gov/pubmed/37123242
http://dx.doi.org/10.1016/j.isci.2023.106510
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