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Direct Observation of Grain-Boundary-Migration-Assisted Radiation Damage Healing in Ultrafine Grained Gold under Mechanical Stress

[Image: see text] Nanostructured metals are a promising class of radiation-tolerant materials. A large volume fraction of grain boundaries (GBs) can provide plenty of sinks for radiation damage, and understanding the underlying healing mechanisms is key to developing more effective radiation toleran...

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Autores principales: Stangebye, Sandra, Ding, Kunqing, Zhang, Yin, Lang, Eric, Hattar, Khalid, Zhu, Ting, Kacher, Josh, Pierron, Olivier
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10141400/
https://www.ncbi.nlm.nih.gov/pubmed/37057989
http://dx.doi.org/10.1021/acs.nanolett.3c00180
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author Stangebye, Sandra
Ding, Kunqing
Zhang, Yin
Lang, Eric
Hattar, Khalid
Zhu, Ting
Kacher, Josh
Pierron, Olivier
author_facet Stangebye, Sandra
Ding, Kunqing
Zhang, Yin
Lang, Eric
Hattar, Khalid
Zhu, Ting
Kacher, Josh
Pierron, Olivier
author_sort Stangebye, Sandra
collection PubMed
description [Image: see text] Nanostructured metals are a promising class of radiation-tolerant materials. A large volume fraction of grain boundaries (GBs) can provide plenty of sinks for radiation damage, and understanding the underlying healing mechanisms is key to developing more effective radiation tolerant materials. Here, we observe radiation damage absorption by stress-assisted GB migration in ultrafine-grained Au thin films using a quantitative in situ transmission electron microscopy nanomechanical testing technique. We show that the GB migration rate is significantly higher in the unirradiated specimens. This behavior is attributed to the presence of smaller grains in the unirradiated specimens that are nearly absent in the irradiated specimens. Our experimental results also suggest that the GB mobility is decreased as a result of irradiation. This work implies that the deleterious effects of irradiation can be reduced by an evolving network of migrating GBs under stress.
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spelling pubmed-101414002023-04-29 Direct Observation of Grain-Boundary-Migration-Assisted Radiation Damage Healing in Ultrafine Grained Gold under Mechanical Stress Stangebye, Sandra Ding, Kunqing Zhang, Yin Lang, Eric Hattar, Khalid Zhu, Ting Kacher, Josh Pierron, Olivier Nano Lett [Image: see text] Nanostructured metals are a promising class of radiation-tolerant materials. A large volume fraction of grain boundaries (GBs) can provide plenty of sinks for radiation damage, and understanding the underlying healing mechanisms is key to developing more effective radiation tolerant materials. Here, we observe radiation damage absorption by stress-assisted GB migration in ultrafine-grained Au thin films using a quantitative in situ transmission electron microscopy nanomechanical testing technique. We show that the GB migration rate is significantly higher in the unirradiated specimens. This behavior is attributed to the presence of smaller grains in the unirradiated specimens that are nearly absent in the irradiated specimens. Our experimental results also suggest that the GB mobility is decreased as a result of irradiation. This work implies that the deleterious effects of irradiation can be reduced by an evolving network of migrating GBs under stress. American Chemical Society 2023-04-14 /pmc/articles/PMC10141400/ /pubmed/37057989 http://dx.doi.org/10.1021/acs.nanolett.3c00180 Text en © 2023 American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Stangebye, Sandra
Ding, Kunqing
Zhang, Yin
Lang, Eric
Hattar, Khalid
Zhu, Ting
Kacher, Josh
Pierron, Olivier
Direct Observation of Grain-Boundary-Migration-Assisted Radiation Damage Healing in Ultrafine Grained Gold under Mechanical Stress
title Direct Observation of Grain-Boundary-Migration-Assisted Radiation Damage Healing in Ultrafine Grained Gold under Mechanical Stress
title_full Direct Observation of Grain-Boundary-Migration-Assisted Radiation Damage Healing in Ultrafine Grained Gold under Mechanical Stress
title_fullStr Direct Observation of Grain-Boundary-Migration-Assisted Radiation Damage Healing in Ultrafine Grained Gold under Mechanical Stress
title_full_unstemmed Direct Observation of Grain-Boundary-Migration-Assisted Radiation Damage Healing in Ultrafine Grained Gold under Mechanical Stress
title_short Direct Observation of Grain-Boundary-Migration-Assisted Radiation Damage Healing in Ultrafine Grained Gold under Mechanical Stress
title_sort direct observation of grain-boundary-migration-assisted radiation damage healing in ultrafine grained gold under mechanical stress
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10141400/
https://www.ncbi.nlm.nih.gov/pubmed/37057989
http://dx.doi.org/10.1021/acs.nanolett.3c00180
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