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Triboelectric-induced ion mobility for artificial intelligence-enhanced mid-infrared gas spectroscopy

Isopropyl alcohol molecules, as a biomarker for anti-virus diagnosis, play a significant role in the area of environmental safety and healthcare relating volatile organic compounds. However, conventional gas molecule detection exhibits dramatic drawbacks, like the strict working conditions of ion mo...

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Autores principales: Zhu, Jianxiong, Ji, Shanling, Ren, Zhihao, Wu, Wenyu, Zhang, Zhihao, Ni, Zhonghua, Liu, Lei, Zhang, Zhisheng, Song, Aiguo, Lee, Chengkuo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10154418/
https://www.ncbi.nlm.nih.gov/pubmed/37130843
http://dx.doi.org/10.1038/s41467-023-38200-6
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author Zhu, Jianxiong
Ji, Shanling
Ren, Zhihao
Wu, Wenyu
Zhang, Zhihao
Ni, Zhonghua
Liu, Lei
Zhang, Zhisheng
Song, Aiguo
Lee, Chengkuo
author_facet Zhu, Jianxiong
Ji, Shanling
Ren, Zhihao
Wu, Wenyu
Zhang, Zhihao
Ni, Zhonghua
Liu, Lei
Zhang, Zhisheng
Song, Aiguo
Lee, Chengkuo
author_sort Zhu, Jianxiong
collection PubMed
description Isopropyl alcohol molecules, as a biomarker for anti-virus diagnosis, play a significant role in the area of environmental safety and healthcare relating volatile organic compounds. However, conventional gas molecule detection exhibits dramatic drawbacks, like the strict working conditions of ion mobility methodology and weak light-matter interaction of mid-infrared spectroscopy, yielding limited response of targeted molecules. We propose a synergistic methodology of artificial intelligence-enhanced ion mobility and mid-infrared spectroscopy, leveraging the complementary features from the sensing signal in different dimensions to reach superior accuracy for isopropyl alcohol identification. We pull in “cold” plasma discharge from triboelectric generator which improves the mid-infrared spectroscopic response of isopropyl alcohol with good regression prediction. Moreover, this synergistic methodology achieves ~99.08% accuracy for a precise gas concentration prediction, even with interferences of different carbon-based gases. The synergistic methodology of artificial intelligence-enhanced system creates mechanism of accurate gas sensing for mixture and regression prediction in healthcare.
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spelling pubmed-101544182023-05-04 Triboelectric-induced ion mobility for artificial intelligence-enhanced mid-infrared gas spectroscopy Zhu, Jianxiong Ji, Shanling Ren, Zhihao Wu, Wenyu Zhang, Zhihao Ni, Zhonghua Liu, Lei Zhang, Zhisheng Song, Aiguo Lee, Chengkuo Nat Commun Article Isopropyl alcohol molecules, as a biomarker for anti-virus diagnosis, play a significant role in the area of environmental safety and healthcare relating volatile organic compounds. However, conventional gas molecule detection exhibits dramatic drawbacks, like the strict working conditions of ion mobility methodology and weak light-matter interaction of mid-infrared spectroscopy, yielding limited response of targeted molecules. We propose a synergistic methodology of artificial intelligence-enhanced ion mobility and mid-infrared spectroscopy, leveraging the complementary features from the sensing signal in different dimensions to reach superior accuracy for isopropyl alcohol identification. We pull in “cold” plasma discharge from triboelectric generator which improves the mid-infrared spectroscopic response of isopropyl alcohol with good regression prediction. Moreover, this synergistic methodology achieves ~99.08% accuracy for a precise gas concentration prediction, even with interferences of different carbon-based gases. The synergistic methodology of artificial intelligence-enhanced system creates mechanism of accurate gas sensing for mixture and regression prediction in healthcare. Nature Publishing Group UK 2023-05-02 /pmc/articles/PMC10154418/ /pubmed/37130843 http://dx.doi.org/10.1038/s41467-023-38200-6 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Zhu, Jianxiong
Ji, Shanling
Ren, Zhihao
Wu, Wenyu
Zhang, Zhihao
Ni, Zhonghua
Liu, Lei
Zhang, Zhisheng
Song, Aiguo
Lee, Chengkuo
Triboelectric-induced ion mobility for artificial intelligence-enhanced mid-infrared gas spectroscopy
title Triboelectric-induced ion mobility for artificial intelligence-enhanced mid-infrared gas spectroscopy
title_full Triboelectric-induced ion mobility for artificial intelligence-enhanced mid-infrared gas spectroscopy
title_fullStr Triboelectric-induced ion mobility for artificial intelligence-enhanced mid-infrared gas spectroscopy
title_full_unstemmed Triboelectric-induced ion mobility for artificial intelligence-enhanced mid-infrared gas spectroscopy
title_short Triboelectric-induced ion mobility for artificial intelligence-enhanced mid-infrared gas spectroscopy
title_sort triboelectric-induced ion mobility for artificial intelligence-enhanced mid-infrared gas spectroscopy
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10154418/
https://www.ncbi.nlm.nih.gov/pubmed/37130843
http://dx.doi.org/10.1038/s41467-023-38200-6
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