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A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection

The discovery of a new physical process in manganese metal is reported. This process will also be present for all manganese-containing materials in condensed matter. The process was discovered by applying our new technique of XR-HERFD (extended-range high-energy-resolution fluorescence detection), w...

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Autores principales: Tran, Nicholas T. T., Sier, Daniel, Kirk, Tony, Tran, Chanh Q., Mosselmans, J. Frederick W., Diaz-Moreno, Sofia, Chantler, Christopher T.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: International Union of Crystallography 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10161895/
https://www.ncbi.nlm.nih.gov/pubmed/37026392
http://dx.doi.org/10.1107/S1600577523002539
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author Tran, Nicholas T. T.
Sier, Daniel
Kirk, Tony
Tran, Chanh Q.
Mosselmans, J. Frederick W.
Diaz-Moreno, Sofia
Chantler, Christopher T.
author_facet Tran, Nicholas T. T.
Sier, Daniel
Kirk, Tony
Tran, Chanh Q.
Mosselmans, J. Frederick W.
Diaz-Moreno, Sofia
Chantler, Christopher T.
author_sort Tran, Nicholas T. T.
collection PubMed
description The discovery of a new physical process in manganese metal is reported. This process will also be present for all manganese-containing materials in condensed matter. The process was discovered by applying our new technique of XR-HERFD (extended-range high-energy-resolution fluorescence detection), which was developed from the popular high-resolution RIXS (resonant inelastic X-ray scattering) and HERFD approaches. The acquired data are accurate to many hundreds of standard deviations beyond what is regarded as the criterion for ‘discovery’. Identification and characterization of many-body processes can shed light on the X-ray absorption fine-structure spectra and inform the scientist on how to interpret them, hence leading to the ability to measure the dynamical nanostructures which are observable using the XR-HERFD method. Although the many-body reduction factor has been used universally in X-ray absorption spectroscopy in analysis over the past 30 years (thousands of papers per year), this experimental result proves that many-body effects are not representable by any constant reduction factor parameter. This paradigm change will provide the foundation for many future studies and X-ray spectroscopy.
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spelling pubmed-101618952023-05-06 A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection Tran, Nicholas T. T. Sier, Daniel Kirk, Tony Tran, Chanh Q. Mosselmans, J. Frederick W. Diaz-Moreno, Sofia Chantler, Christopher T. J Synchrotron Radiat Research Papers The discovery of a new physical process in manganese metal is reported. This process will also be present for all manganese-containing materials in condensed matter. The process was discovered by applying our new technique of XR-HERFD (extended-range high-energy-resolution fluorescence detection), which was developed from the popular high-resolution RIXS (resonant inelastic X-ray scattering) and HERFD approaches. The acquired data are accurate to many hundreds of standard deviations beyond what is regarded as the criterion for ‘discovery’. Identification and characterization of many-body processes can shed light on the X-ray absorption fine-structure spectra and inform the scientist on how to interpret them, hence leading to the ability to measure the dynamical nanostructures which are observable using the XR-HERFD method. Although the many-body reduction factor has been used universally in X-ray absorption spectroscopy in analysis over the past 30 years (thousands of papers per year), this experimental result proves that many-body effects are not representable by any constant reduction factor parameter. This paradigm change will provide the foundation for many future studies and X-ray spectroscopy. International Union of Crystallography 2023-04-07 /pmc/articles/PMC10161895/ /pubmed/37026392 http://dx.doi.org/10.1107/S1600577523002539 Text en © Nicholas T. T. Tran et al. 2023 https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution (CC-BY) Licence, which permits unrestricted use, distribution, and reproduction in any medium, provided the original authors and source are cited.
spellingShingle Research Papers
Tran, Nicholas T. T.
Sier, Daniel
Kirk, Tony
Tran, Chanh Q.
Mosselmans, J. Frederick W.
Diaz-Moreno, Sofia
Chantler, Christopher T.
A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection
title A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection
title_full A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection
title_fullStr A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection
title_full_unstemmed A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection
title_short A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection
title_sort new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection
topic Research Papers
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10161895/
https://www.ncbi.nlm.nih.gov/pubmed/37026392
http://dx.doi.org/10.1107/S1600577523002539
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