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A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection
The discovery of a new physical process in manganese metal is reported. This process will also be present for all manganese-containing materials in condensed matter. The process was discovered by applying our new technique of XR-HERFD (extended-range high-energy-resolution fluorescence detection), w...
Autores principales: | , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
International Union of Crystallography
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10161895/ https://www.ncbi.nlm.nih.gov/pubmed/37026392 http://dx.doi.org/10.1107/S1600577523002539 |
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author | Tran, Nicholas T. T. Sier, Daniel Kirk, Tony Tran, Chanh Q. Mosselmans, J. Frederick W. Diaz-Moreno, Sofia Chantler, Christopher T. |
author_facet | Tran, Nicholas T. T. Sier, Daniel Kirk, Tony Tran, Chanh Q. Mosselmans, J. Frederick W. Diaz-Moreno, Sofia Chantler, Christopher T. |
author_sort | Tran, Nicholas T. T. |
collection | PubMed |
description | The discovery of a new physical process in manganese metal is reported. This process will also be present for all manganese-containing materials in condensed matter. The process was discovered by applying our new technique of XR-HERFD (extended-range high-energy-resolution fluorescence detection), which was developed from the popular high-resolution RIXS (resonant inelastic X-ray scattering) and HERFD approaches. The acquired data are accurate to many hundreds of standard deviations beyond what is regarded as the criterion for ‘discovery’. Identification and characterization of many-body processes can shed light on the X-ray absorption fine-structure spectra and inform the scientist on how to interpret them, hence leading to the ability to measure the dynamical nanostructures which are observable using the XR-HERFD method. Although the many-body reduction factor has been used universally in X-ray absorption spectroscopy in analysis over the past 30 years (thousands of papers per year), this experimental result proves that many-body effects are not representable by any constant reduction factor parameter. This paradigm change will provide the foundation for many future studies and X-ray spectroscopy. |
format | Online Article Text |
id | pubmed-10161895 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | International Union of Crystallography |
record_format | MEDLINE/PubMed |
spelling | pubmed-101618952023-05-06 A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection Tran, Nicholas T. T. Sier, Daniel Kirk, Tony Tran, Chanh Q. Mosselmans, J. Frederick W. Diaz-Moreno, Sofia Chantler, Christopher T. J Synchrotron Radiat Research Papers The discovery of a new physical process in manganese metal is reported. This process will also be present for all manganese-containing materials in condensed matter. The process was discovered by applying our new technique of XR-HERFD (extended-range high-energy-resolution fluorescence detection), which was developed from the popular high-resolution RIXS (resonant inelastic X-ray scattering) and HERFD approaches. The acquired data are accurate to many hundreds of standard deviations beyond what is regarded as the criterion for ‘discovery’. Identification and characterization of many-body processes can shed light on the X-ray absorption fine-structure spectra and inform the scientist on how to interpret them, hence leading to the ability to measure the dynamical nanostructures which are observable using the XR-HERFD method. Although the many-body reduction factor has been used universally in X-ray absorption spectroscopy in analysis over the past 30 years (thousands of papers per year), this experimental result proves that many-body effects are not representable by any constant reduction factor parameter. This paradigm change will provide the foundation for many future studies and X-ray spectroscopy. International Union of Crystallography 2023-04-07 /pmc/articles/PMC10161895/ /pubmed/37026392 http://dx.doi.org/10.1107/S1600577523002539 Text en © Nicholas T. T. Tran et al. 2023 https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution (CC-BY) Licence, which permits unrestricted use, distribution, and reproduction in any medium, provided the original authors and source are cited. |
spellingShingle | Research Papers Tran, Nicholas T. T. Sier, Daniel Kirk, Tony Tran, Chanh Q. Mosselmans, J. Frederick W. Diaz-Moreno, Sofia Chantler, Christopher T. A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection |
title | A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection |
title_full | A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection |
title_fullStr | A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection |
title_full_unstemmed | A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection |
title_short | A new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection |
title_sort | new satellite of manganese revealed by extended-range high-energy-resolution fluorescence detection |
topic | Research Papers |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10161895/ https://www.ncbi.nlm.nih.gov/pubmed/37026392 http://dx.doi.org/10.1107/S1600577523002539 |
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