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Structural and Scintillation Properties of Ce(3+):Gd(3)Al(3)Ga(2)O(12) Translucent Ceramics Prepared by One-Step Sintering

Cerium-doped gadolinium aluminum gallium garnet (Ce(3+):Gd(3)Al(3)Ga(2)O(12), Ce(3+):GAGG) ceramic is a promising scintillation material. In this study, Ce(3+):Gd(3)Al(3)Ga(2)O(12) scintillation ceramics were prepared by the one-step sintering of commercially available Gd(2)O(3), Al(2)O(3), Ga(2)O(3...

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Autores principales: You, Qi, Lin, Hui, Hong, Ruijin, Han, Zhaoxia, Zhang, Dawei, Ding, Yuchong
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10179960/
https://www.ncbi.nlm.nih.gov/pubmed/37176253
http://dx.doi.org/10.3390/ma16093373
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author You, Qi
Lin, Hui
Hong, Ruijin
Han, Zhaoxia
Zhang, Dawei
Ding, Yuchong
author_facet You, Qi
Lin, Hui
Hong, Ruijin
Han, Zhaoxia
Zhang, Dawei
Ding, Yuchong
author_sort You, Qi
collection PubMed
description Cerium-doped gadolinium aluminum gallium garnet (Ce(3+):Gd(3)Al(3)Ga(2)O(12), Ce(3+):GAGG) ceramic is a promising scintillation material. In this study, Ce(3+):Gd(3)Al(3)Ga(2)O(12) scintillation ceramics were prepared by the one-step sintering of commercially available Gd(2)O(3), Al(2)O(3), Ga(2)O(3), and CeO(2) powders in a flowing oxygen atmosphere at 1600 °C by solid-phase reaction sintering. For all the Ce(3+):Gd(3)Al(3)Ga(2)O(12) ceramic samples doped with different amounts of Ce(3+) doping, dense ceramics were obtained. The structure, photoluminescence, and scintillation properties of the Ce(3+):Gd(3)Al(3)Ga(2)O(12) ceramics have been investigated. The average grain size of samples sintered at 1600 °C is about 2 μm. The X-ray excitation luminescence peak is around 560 nm, which is consistent with that of Ce(3+):Gd(3)Al(3)Ga(2)O(12) single crystals, matching well with the computed tomography X-ray detector’s response sensitivity. The light yield is higher compared to the standard reference sample—lutetium yttrium orthosilicate single crystal.
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spelling pubmed-101799602023-05-13 Structural and Scintillation Properties of Ce(3+):Gd(3)Al(3)Ga(2)O(12) Translucent Ceramics Prepared by One-Step Sintering You, Qi Lin, Hui Hong, Ruijin Han, Zhaoxia Zhang, Dawei Ding, Yuchong Materials (Basel) Article Cerium-doped gadolinium aluminum gallium garnet (Ce(3+):Gd(3)Al(3)Ga(2)O(12), Ce(3+):GAGG) ceramic is a promising scintillation material. In this study, Ce(3+):Gd(3)Al(3)Ga(2)O(12) scintillation ceramics were prepared by the one-step sintering of commercially available Gd(2)O(3), Al(2)O(3), Ga(2)O(3), and CeO(2) powders in a flowing oxygen atmosphere at 1600 °C by solid-phase reaction sintering. For all the Ce(3+):Gd(3)Al(3)Ga(2)O(12) ceramic samples doped with different amounts of Ce(3+) doping, dense ceramics were obtained. The structure, photoluminescence, and scintillation properties of the Ce(3+):Gd(3)Al(3)Ga(2)O(12) ceramics have been investigated. The average grain size of samples sintered at 1600 °C is about 2 μm. The X-ray excitation luminescence peak is around 560 nm, which is consistent with that of Ce(3+):Gd(3)Al(3)Ga(2)O(12) single crystals, matching well with the computed tomography X-ray detector’s response sensitivity. The light yield is higher compared to the standard reference sample—lutetium yttrium orthosilicate single crystal. MDPI 2023-04-25 /pmc/articles/PMC10179960/ /pubmed/37176253 http://dx.doi.org/10.3390/ma16093373 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
You, Qi
Lin, Hui
Hong, Ruijin
Han, Zhaoxia
Zhang, Dawei
Ding, Yuchong
Structural and Scintillation Properties of Ce(3+):Gd(3)Al(3)Ga(2)O(12) Translucent Ceramics Prepared by One-Step Sintering
title Structural and Scintillation Properties of Ce(3+):Gd(3)Al(3)Ga(2)O(12) Translucent Ceramics Prepared by One-Step Sintering
title_full Structural and Scintillation Properties of Ce(3+):Gd(3)Al(3)Ga(2)O(12) Translucent Ceramics Prepared by One-Step Sintering
title_fullStr Structural and Scintillation Properties of Ce(3+):Gd(3)Al(3)Ga(2)O(12) Translucent Ceramics Prepared by One-Step Sintering
title_full_unstemmed Structural and Scintillation Properties of Ce(3+):Gd(3)Al(3)Ga(2)O(12) Translucent Ceramics Prepared by One-Step Sintering
title_short Structural and Scintillation Properties of Ce(3+):Gd(3)Al(3)Ga(2)O(12) Translucent Ceramics Prepared by One-Step Sintering
title_sort structural and scintillation properties of ce(3+):gd(3)al(3)ga(2)o(12) translucent ceramics prepared by one-step sintering
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10179960/
https://www.ncbi.nlm.nih.gov/pubmed/37176253
http://dx.doi.org/10.3390/ma16093373
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