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Narrowband, Angle-Tunable, Helicity-Dependent Terahertz Emission from Nanowires of the Topological Dirac Semimetal Cd(3)As(2)

[Image: see text] All-optical control of terahertz pulses is essential for the development of optoelectronic devices for next-generation quantum technologies. Despite substantial research in THz generation methods, polarization control remains difficult. Here, we demonstrate that by exploiting band...

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Autores principales: Boland, Jessica L., Damry, Djamshid A., Xia, Chelsea Q., Schönherr, Piet, Prabhakaran, Dharmalingam, Herz, Laura M., Hesjedal, Thorsten, Johnston, Michael B.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10197169/
https://www.ncbi.nlm.nih.gov/pubmed/37215322
http://dx.doi.org/10.1021/acsphotonics.3c00068
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author Boland, Jessica L.
Damry, Djamshid A.
Xia, Chelsea Q.
Schönherr, Piet
Prabhakaran, Dharmalingam
Herz, Laura M.
Hesjedal, Thorsten
Johnston, Michael B.
author_facet Boland, Jessica L.
Damry, Djamshid A.
Xia, Chelsea Q.
Schönherr, Piet
Prabhakaran, Dharmalingam
Herz, Laura M.
Hesjedal, Thorsten
Johnston, Michael B.
author_sort Boland, Jessica L.
collection PubMed
description [Image: see text] All-optical control of terahertz pulses is essential for the development of optoelectronic devices for next-generation quantum technologies. Despite substantial research in THz generation methods, polarization control remains difficult. Here, we demonstrate that by exploiting band structure topology, both helicity-dependent and helicity-independent THz emission can be generated from nanowires of the topological Dirac semimetal Cd(3)As(2). We show that narrowband THz pulses can be generated at oblique incidence by driving the system with optical (1.55 eV) pulses with circular polarization. Varying the incident angle also provides control of the peak emission frequency, with peak frequencies spanning 0.21–1.40 THz as the angle is tuned from 15 to 45°. We therefore present Cd(3)As(2) nanowires as a promising novel material platform for controllable terahertz emission.
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spelling pubmed-101971692023-05-20 Narrowband, Angle-Tunable, Helicity-Dependent Terahertz Emission from Nanowires of the Topological Dirac Semimetal Cd(3)As(2) Boland, Jessica L. Damry, Djamshid A. Xia, Chelsea Q. Schönherr, Piet Prabhakaran, Dharmalingam Herz, Laura M. Hesjedal, Thorsten Johnston, Michael B. ACS Photonics [Image: see text] All-optical control of terahertz pulses is essential for the development of optoelectronic devices for next-generation quantum technologies. Despite substantial research in THz generation methods, polarization control remains difficult. Here, we demonstrate that by exploiting band structure topology, both helicity-dependent and helicity-independent THz emission can be generated from nanowires of the topological Dirac semimetal Cd(3)As(2). We show that narrowband THz pulses can be generated at oblique incidence by driving the system with optical (1.55 eV) pulses with circular polarization. Varying the incident angle also provides control of the peak emission frequency, with peak frequencies spanning 0.21–1.40 THz as the angle is tuned from 15 to 45°. We therefore present Cd(3)As(2) nanowires as a promising novel material platform for controllable terahertz emission. American Chemical Society 2023-04-03 /pmc/articles/PMC10197169/ /pubmed/37215322 http://dx.doi.org/10.1021/acsphotonics.3c00068 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Boland, Jessica L.
Damry, Djamshid A.
Xia, Chelsea Q.
Schönherr, Piet
Prabhakaran, Dharmalingam
Herz, Laura M.
Hesjedal, Thorsten
Johnston, Michael B.
Narrowband, Angle-Tunable, Helicity-Dependent Terahertz Emission from Nanowires of the Topological Dirac Semimetal Cd(3)As(2)
title Narrowband, Angle-Tunable, Helicity-Dependent Terahertz Emission from Nanowires of the Topological Dirac Semimetal Cd(3)As(2)
title_full Narrowband, Angle-Tunable, Helicity-Dependent Terahertz Emission from Nanowires of the Topological Dirac Semimetal Cd(3)As(2)
title_fullStr Narrowband, Angle-Tunable, Helicity-Dependent Terahertz Emission from Nanowires of the Topological Dirac Semimetal Cd(3)As(2)
title_full_unstemmed Narrowband, Angle-Tunable, Helicity-Dependent Terahertz Emission from Nanowires of the Topological Dirac Semimetal Cd(3)As(2)
title_short Narrowband, Angle-Tunable, Helicity-Dependent Terahertz Emission from Nanowires of the Topological Dirac Semimetal Cd(3)As(2)
title_sort narrowband, angle-tunable, helicity-dependent terahertz emission from nanowires of the topological dirac semimetal cd(3)as(2)
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10197169/
https://www.ncbi.nlm.nih.gov/pubmed/37215322
http://dx.doi.org/10.1021/acsphotonics.3c00068
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