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Correlated insulator collapse due to quantum avalanche via in-gap ladder states
The significant discrepancy observed between the predicted and experimental switching fields in correlated insulators under a DC electric field far-from-equilibrium necessitates a reevaluation of current microscopic understanding. Here we show that an electron avalanche can occur in the bulk limit o...
Autores principales: | , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10203265/ https://www.ncbi.nlm.nih.gov/pubmed/37217490 http://dx.doi.org/10.1038/s41467-023-38557-8 |
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author | Han, Jong E. Aron, Camille Chen, Xi Mansaray, Ishiaka Han, Jae-Ho Kim, Ki-Seok Randle, Michael Bird, Jonathan P. |
author_facet | Han, Jong E. Aron, Camille Chen, Xi Mansaray, Ishiaka Han, Jae-Ho Kim, Ki-Seok Randle, Michael Bird, Jonathan P. |
author_sort | Han, Jong E. |
collection | PubMed |
description | The significant discrepancy observed between the predicted and experimental switching fields in correlated insulators under a DC electric field far-from-equilibrium necessitates a reevaluation of current microscopic understanding. Here we show that an electron avalanche can occur in the bulk limit of such insulators at arbitrarily small electric field by introducing a generic model of electrons coupled to an inelastic medium of phonons. The quantum avalanche arises by the generation of a ladder of in-gap states, created by a multi-phonon emission process. Hot-phonons in the avalanche trigger a premature and partial collapse of the correlated gap. The phonon spectrum dictates the existence of two-stage versus single-stage switching events which we associate with charge-density-wave and Mott resistive phase transitions, respectively. The behavior of electron and phonon temperatures, as well as the temperature dependence of the threshold fields, demonstrates how a crossover between the thermal and quantum switching scenarios emerges within a unified framework of the quantum avalanche. |
format | Online Article Text |
id | pubmed-10203265 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-102032652023-05-24 Correlated insulator collapse due to quantum avalanche via in-gap ladder states Han, Jong E. Aron, Camille Chen, Xi Mansaray, Ishiaka Han, Jae-Ho Kim, Ki-Seok Randle, Michael Bird, Jonathan P. Nat Commun Article The significant discrepancy observed between the predicted and experimental switching fields in correlated insulators under a DC electric field far-from-equilibrium necessitates a reevaluation of current microscopic understanding. Here we show that an electron avalanche can occur in the bulk limit of such insulators at arbitrarily small electric field by introducing a generic model of electrons coupled to an inelastic medium of phonons. The quantum avalanche arises by the generation of a ladder of in-gap states, created by a multi-phonon emission process. Hot-phonons in the avalanche trigger a premature and partial collapse of the correlated gap. The phonon spectrum dictates the existence of two-stage versus single-stage switching events which we associate with charge-density-wave and Mott resistive phase transitions, respectively. The behavior of electron and phonon temperatures, as well as the temperature dependence of the threshold fields, demonstrates how a crossover between the thermal and quantum switching scenarios emerges within a unified framework of the quantum avalanche. Nature Publishing Group UK 2023-05-22 /pmc/articles/PMC10203265/ /pubmed/37217490 http://dx.doi.org/10.1038/s41467-023-38557-8 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Han, Jong E. Aron, Camille Chen, Xi Mansaray, Ishiaka Han, Jae-Ho Kim, Ki-Seok Randle, Michael Bird, Jonathan P. Correlated insulator collapse due to quantum avalanche via in-gap ladder states |
title | Correlated insulator collapse due to quantum avalanche via in-gap ladder states |
title_full | Correlated insulator collapse due to quantum avalanche via in-gap ladder states |
title_fullStr | Correlated insulator collapse due to quantum avalanche via in-gap ladder states |
title_full_unstemmed | Correlated insulator collapse due to quantum avalanche via in-gap ladder states |
title_short | Correlated insulator collapse due to quantum avalanche via in-gap ladder states |
title_sort | correlated insulator collapse due to quantum avalanche via in-gap ladder states |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10203265/ https://www.ncbi.nlm.nih.gov/pubmed/37217490 http://dx.doi.org/10.1038/s41467-023-38557-8 |
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