Cargando…

Correlated insulator collapse due to quantum avalanche via in-gap ladder states

The significant discrepancy observed between the predicted and experimental switching fields in correlated insulators under a DC electric field far-from-equilibrium necessitates a reevaluation of current microscopic understanding. Here we show that an electron avalanche can occur in the bulk limit o...

Descripción completa

Detalles Bibliográficos
Autores principales: Han, Jong E., Aron, Camille, Chen, Xi, Mansaray, Ishiaka, Han, Jae-Ho, Kim, Ki-Seok, Randle, Michael, Bird, Jonathan P.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10203265/
https://www.ncbi.nlm.nih.gov/pubmed/37217490
http://dx.doi.org/10.1038/s41467-023-38557-8
_version_ 1785045594650181632
author Han, Jong E.
Aron, Camille
Chen, Xi
Mansaray, Ishiaka
Han, Jae-Ho
Kim, Ki-Seok
Randle, Michael
Bird, Jonathan P.
author_facet Han, Jong E.
Aron, Camille
Chen, Xi
Mansaray, Ishiaka
Han, Jae-Ho
Kim, Ki-Seok
Randle, Michael
Bird, Jonathan P.
author_sort Han, Jong E.
collection PubMed
description The significant discrepancy observed between the predicted and experimental switching fields in correlated insulators under a DC electric field far-from-equilibrium necessitates a reevaluation of current microscopic understanding. Here we show that an electron avalanche can occur in the bulk limit of such insulators at arbitrarily small electric field by introducing a generic model of electrons coupled to an inelastic medium of phonons. The quantum avalanche arises by the generation of a ladder of in-gap states, created by a multi-phonon emission process. Hot-phonons in the avalanche trigger a premature and partial collapse of the correlated gap. The phonon spectrum dictates the existence of two-stage versus single-stage switching events which we associate with charge-density-wave and Mott resistive phase transitions, respectively. The behavior of electron and phonon temperatures, as well as the temperature dependence of the threshold fields, demonstrates how a crossover between the thermal and quantum switching scenarios emerges within a unified framework of the quantum avalanche.
format Online
Article
Text
id pubmed-10203265
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-102032652023-05-24 Correlated insulator collapse due to quantum avalanche via in-gap ladder states Han, Jong E. Aron, Camille Chen, Xi Mansaray, Ishiaka Han, Jae-Ho Kim, Ki-Seok Randle, Michael Bird, Jonathan P. Nat Commun Article The significant discrepancy observed between the predicted and experimental switching fields in correlated insulators under a DC electric field far-from-equilibrium necessitates a reevaluation of current microscopic understanding. Here we show that an electron avalanche can occur in the bulk limit of such insulators at arbitrarily small electric field by introducing a generic model of electrons coupled to an inelastic medium of phonons. The quantum avalanche arises by the generation of a ladder of in-gap states, created by a multi-phonon emission process. Hot-phonons in the avalanche trigger a premature and partial collapse of the correlated gap. The phonon spectrum dictates the existence of two-stage versus single-stage switching events which we associate with charge-density-wave and Mott resistive phase transitions, respectively. The behavior of electron and phonon temperatures, as well as the temperature dependence of the threshold fields, demonstrates how a crossover between the thermal and quantum switching scenarios emerges within a unified framework of the quantum avalanche. Nature Publishing Group UK 2023-05-22 /pmc/articles/PMC10203265/ /pubmed/37217490 http://dx.doi.org/10.1038/s41467-023-38557-8 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Han, Jong E.
Aron, Camille
Chen, Xi
Mansaray, Ishiaka
Han, Jae-Ho
Kim, Ki-Seok
Randle, Michael
Bird, Jonathan P.
Correlated insulator collapse due to quantum avalanche via in-gap ladder states
title Correlated insulator collapse due to quantum avalanche via in-gap ladder states
title_full Correlated insulator collapse due to quantum avalanche via in-gap ladder states
title_fullStr Correlated insulator collapse due to quantum avalanche via in-gap ladder states
title_full_unstemmed Correlated insulator collapse due to quantum avalanche via in-gap ladder states
title_short Correlated insulator collapse due to quantum avalanche via in-gap ladder states
title_sort correlated insulator collapse due to quantum avalanche via in-gap ladder states
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10203265/
https://www.ncbi.nlm.nih.gov/pubmed/37217490
http://dx.doi.org/10.1038/s41467-023-38557-8
work_keys_str_mv AT hanjonge correlatedinsulatorcollapseduetoquantumavalancheviaingapladderstates
AT aroncamille correlatedinsulatorcollapseduetoquantumavalancheviaingapladderstates
AT chenxi correlatedinsulatorcollapseduetoquantumavalancheviaingapladderstates
AT mansarayishiaka correlatedinsulatorcollapseduetoquantumavalancheviaingapladderstates
AT hanjaeho correlatedinsulatorcollapseduetoquantumavalancheviaingapladderstates
AT kimkiseok correlatedinsulatorcollapseduetoquantumavalancheviaingapladderstates
AT randlemichael correlatedinsulatorcollapseduetoquantumavalancheviaingapladderstates
AT birdjonathanp correlatedinsulatorcollapseduetoquantumavalancheviaingapladderstates