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Topology of vibrational modes predicts plastic events in glasses

The plastic deformation of crystalline materials can be understood by considering their structural defects such as disclinations and dislocations. Although also glasses are solids, their structure resembles closely the one of a liquid and hence the concept of structural defects becomes ill-defined....

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Autores principales: Wu, Zhen Wei, Chen, Yixiao, Wang, Wei-Hua, Kob, Walter, Xu, Limei
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10209080/
https://www.ncbi.nlm.nih.gov/pubmed/37225717
http://dx.doi.org/10.1038/s41467-023-38547-w
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author Wu, Zhen Wei
Chen, Yixiao
Wang, Wei-Hua
Kob, Walter
Xu, Limei
author_facet Wu, Zhen Wei
Chen, Yixiao
Wang, Wei-Hua
Kob, Walter
Xu, Limei
author_sort Wu, Zhen Wei
collection PubMed
description The plastic deformation of crystalline materials can be understood by considering their structural defects such as disclinations and dislocations. Although also glasses are solids, their structure resembles closely the one of a liquid and hence the concept of structural defects becomes ill-defined. As a consequence it is very challenging to rationalize on a microscopic level the mechanical properties of glasses close to the yielding point and to relate plastic events to structural properties. Here we investigate the topological characteristics of the eigenvector field of the vibrational excitations of a two-dimensional glass model, notably the geometric arrangement of the topological defects as a function of vibrational frequency. We find that if the system is subjected to a quasistatic shear, the location of the resulting plastic events correlate strongly with the topological defects that have a negative charge. Our results provide thus a direct link between the structure of glasses prior their deformation and the plastic events during deformation.
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spelling pubmed-102090802023-05-26 Topology of vibrational modes predicts plastic events in glasses Wu, Zhen Wei Chen, Yixiao Wang, Wei-Hua Kob, Walter Xu, Limei Nat Commun Article The plastic deformation of crystalline materials can be understood by considering their structural defects such as disclinations and dislocations. Although also glasses are solids, their structure resembles closely the one of a liquid and hence the concept of structural defects becomes ill-defined. As a consequence it is very challenging to rationalize on a microscopic level the mechanical properties of glasses close to the yielding point and to relate plastic events to structural properties. Here we investigate the topological characteristics of the eigenvector field of the vibrational excitations of a two-dimensional glass model, notably the geometric arrangement of the topological defects as a function of vibrational frequency. We find that if the system is subjected to a quasistatic shear, the location of the resulting plastic events correlate strongly with the topological defects that have a negative charge. Our results provide thus a direct link between the structure of glasses prior their deformation and the plastic events during deformation. Nature Publishing Group UK 2023-05-24 /pmc/articles/PMC10209080/ /pubmed/37225717 http://dx.doi.org/10.1038/s41467-023-38547-w Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Wu, Zhen Wei
Chen, Yixiao
Wang, Wei-Hua
Kob, Walter
Xu, Limei
Topology of vibrational modes predicts plastic events in glasses
title Topology of vibrational modes predicts plastic events in glasses
title_full Topology of vibrational modes predicts plastic events in glasses
title_fullStr Topology of vibrational modes predicts plastic events in glasses
title_full_unstemmed Topology of vibrational modes predicts plastic events in glasses
title_short Topology of vibrational modes predicts plastic events in glasses
title_sort topology of vibrational modes predicts plastic events in glasses
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10209080/
https://www.ncbi.nlm.nih.gov/pubmed/37225717
http://dx.doi.org/10.1038/s41467-023-38547-w
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