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Two-step crystallisation in a 2D active magnetic granular system confined by a parabolic potential

We studied the two-step crystallisation process of a magnetic active 2D-granular system placed on different lens concaveness and under the action of an alternating magnetic field which controls its effective temperature. We have observed that the two-step features of the crystallisation process are...

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Autores principales: Escobar, A., Ledesma-Motolinía, M., Carrillo-Estrada, J. L., Donado, F.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10220085/
https://www.ncbi.nlm.nih.gov/pubmed/37237064
http://dx.doi.org/10.1038/s41598-023-35135-2
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author Escobar, A.
Ledesma-Motolinía, M.
Carrillo-Estrada, J. L.
Donado, F.
author_facet Escobar, A.
Ledesma-Motolinía, M.
Carrillo-Estrada, J. L.
Donado, F.
author_sort Escobar, A.
collection PubMed
description We studied the two-step crystallisation process of a magnetic active 2D-granular system placed on different lens concaveness and under the action of an alternating magnetic field which controls its effective temperature. We have observed that the two-step features of the crystallisation process are more evident as the depth of the parabolic potential increases. At the initial formation of the nucleus, as a first step, in the central region of the lens an amorphous aggregate is formed. In an ulterior second step, this disordered aggregate, due to the effective temperature and the perturbations caused by the impacts of free particles moving in the surrounding region, evolves to an ordered crystalline structure. The nucleus size is larger for deeper concaveness of the parabolic potential. However, if the depth of the parabolic potential exceeds a certain value, the reordering process of the second step does not occur. The crystal growth occurs similarly; small disordered groups of particles join the nucleus, forming an amorphous shell of particles which experiments a rearranging while the aggregate grows. In the explored range of the depths of the parabolic potential, crystallisation generally occurs quicker as the deeper parabolic potential is. Also, aggregates are more clearly round-shaped as parabolic potential depth increases. On the contrary, the structures are more branched for a smaller depth of the parabolic potential. We studied the structural changes and features in the system by using the sixth orientational order parameter and the packing fraction.
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spelling pubmed-102200852023-05-28 Two-step crystallisation in a 2D active magnetic granular system confined by a parabolic potential Escobar, A. Ledesma-Motolinía, M. Carrillo-Estrada, J. L. Donado, F. Sci Rep Article We studied the two-step crystallisation process of a magnetic active 2D-granular system placed on different lens concaveness and under the action of an alternating magnetic field which controls its effective temperature. We have observed that the two-step features of the crystallisation process are more evident as the depth of the parabolic potential increases. At the initial formation of the nucleus, as a first step, in the central region of the lens an amorphous aggregate is formed. In an ulterior second step, this disordered aggregate, due to the effective temperature and the perturbations caused by the impacts of free particles moving in the surrounding region, evolves to an ordered crystalline structure. The nucleus size is larger for deeper concaveness of the parabolic potential. However, if the depth of the parabolic potential exceeds a certain value, the reordering process of the second step does not occur. The crystal growth occurs similarly; small disordered groups of particles join the nucleus, forming an amorphous shell of particles which experiments a rearranging while the aggregate grows. In the explored range of the depths of the parabolic potential, crystallisation generally occurs quicker as the deeper parabolic potential is. Also, aggregates are more clearly round-shaped as parabolic potential depth increases. On the contrary, the structures are more branched for a smaller depth of the parabolic potential. We studied the structural changes and features in the system by using the sixth orientational order parameter and the packing fraction. Nature Publishing Group UK 2023-05-26 /pmc/articles/PMC10220085/ /pubmed/37237064 http://dx.doi.org/10.1038/s41598-023-35135-2 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Escobar, A.
Ledesma-Motolinía, M.
Carrillo-Estrada, J. L.
Donado, F.
Two-step crystallisation in a 2D active magnetic granular system confined by a parabolic potential
title Two-step crystallisation in a 2D active magnetic granular system confined by a parabolic potential
title_full Two-step crystallisation in a 2D active magnetic granular system confined by a parabolic potential
title_fullStr Two-step crystallisation in a 2D active magnetic granular system confined by a parabolic potential
title_full_unstemmed Two-step crystallisation in a 2D active magnetic granular system confined by a parabolic potential
title_short Two-step crystallisation in a 2D active magnetic granular system confined by a parabolic potential
title_sort two-step crystallisation in a 2d active magnetic granular system confined by a parabolic potential
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10220085/
https://www.ncbi.nlm.nih.gov/pubmed/37237064
http://dx.doi.org/10.1038/s41598-023-35135-2
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