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Extensive Gaseous Emissions Reduction of Firewood-Fueled Low Power Fireplaces by a Gas Sensor Based Advanced Combustion Airflow Control System and Catalytic Post-Oxidation

In view of the tremendous emissions of toxic gases and particulate matter (PM) by low-power firewood-fueled fireplaces, there is an urgent need for effective measures to lower emissions to keep this renewable and economical source for private home heating available in the future. For this purpose, a...

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Autores principales: Zhang, Xin, Ojha, Binayak, Bichlmaier, Hermann, Hartmann, Ingo, Kohler, Heinz
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10222192/
https://www.ncbi.nlm.nih.gov/pubmed/37430592
http://dx.doi.org/10.3390/s23104679
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author Zhang, Xin
Ojha, Binayak
Bichlmaier, Hermann
Hartmann, Ingo
Kohler, Heinz
author_facet Zhang, Xin
Ojha, Binayak
Bichlmaier, Hermann
Hartmann, Ingo
Kohler, Heinz
author_sort Zhang, Xin
collection PubMed
description In view of the tremendous emissions of toxic gases and particulate matter (PM) by low-power firewood-fueled fireplaces, there is an urgent need for effective measures to lower emissions to keep this renewable and economical source for private home heating available in the future. For this purpose, an advanced combustion air control system was developed and tested on a commercial fireplace (HKD7, Bunner GmbH, Eggenfelden, Germany), complemented with a commercial oxidation catalyst (EmTechEngineering GmbH, Leipzig, Germany) placed in the post-combustion zone. Combustion air stream control of the wood-log charge combustion was realized by five different control algorithms to describe all situations of combustion properly. These control algorithms are based on the signals of commercial sensors representing catalyst temperature (thermocouple), residual oxygen concentration (LSU 4.9, Bosch GmbH, Gerlingen, Germany) and CO/HC-content in the exhaust (LH-sensor, Lamtec Mess- und Regeltechnik für Feuerungen GmbH & Co. KG, Walldorf (Germany)). The actual flows of the combustion air streams, as calculated for the primary and secondary combustion zone, are adjusted by motor-driven shutters and commercial air mass flow sensors (HFM7, Bosch GmbH, Gerlingen, Germany) in separate feedback control loops. For the first time, the residual CO/HC-content (CO, methane, formaldehyde, etc.) in the flue gas is in-situ monitored with a long-term stable AuPt/YSZ/Pt mixed potential high-temperature gas sensor, which allows continuous estimation of the flue gas quality with an accuracy of about ±10%. This parameter is not only an essential input for advanced combustion air stream control but also provides monitoring of the actual combustion quality and logging of this value over a whole heating period. By many firing experiments in the laboratory and by field tests over four months, it could be demonstrated that with this long-term stable and advanced automated firing system, depression of the gaseous emissions by about 90% related to manually operated fireplaces without catalyst could be achieved. In addition, preliminary investigations at a firing appliance complemented by an electrostatic precipitator yielded PM emission depression between 70% and 90%, depending on the firewood load.
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spelling pubmed-102221922023-05-28 Extensive Gaseous Emissions Reduction of Firewood-Fueled Low Power Fireplaces by a Gas Sensor Based Advanced Combustion Airflow Control System and Catalytic Post-Oxidation Zhang, Xin Ojha, Binayak Bichlmaier, Hermann Hartmann, Ingo Kohler, Heinz Sensors (Basel) Article In view of the tremendous emissions of toxic gases and particulate matter (PM) by low-power firewood-fueled fireplaces, there is an urgent need for effective measures to lower emissions to keep this renewable and economical source for private home heating available in the future. For this purpose, an advanced combustion air control system was developed and tested on a commercial fireplace (HKD7, Bunner GmbH, Eggenfelden, Germany), complemented with a commercial oxidation catalyst (EmTechEngineering GmbH, Leipzig, Germany) placed in the post-combustion zone. Combustion air stream control of the wood-log charge combustion was realized by five different control algorithms to describe all situations of combustion properly. These control algorithms are based on the signals of commercial sensors representing catalyst temperature (thermocouple), residual oxygen concentration (LSU 4.9, Bosch GmbH, Gerlingen, Germany) and CO/HC-content in the exhaust (LH-sensor, Lamtec Mess- und Regeltechnik für Feuerungen GmbH & Co. KG, Walldorf (Germany)). The actual flows of the combustion air streams, as calculated for the primary and secondary combustion zone, are adjusted by motor-driven shutters and commercial air mass flow sensors (HFM7, Bosch GmbH, Gerlingen, Germany) in separate feedback control loops. For the first time, the residual CO/HC-content (CO, methane, formaldehyde, etc.) in the flue gas is in-situ monitored with a long-term stable AuPt/YSZ/Pt mixed potential high-temperature gas sensor, which allows continuous estimation of the flue gas quality with an accuracy of about ±10%. This parameter is not only an essential input for advanced combustion air stream control but also provides monitoring of the actual combustion quality and logging of this value over a whole heating period. By many firing experiments in the laboratory and by field tests over four months, it could be demonstrated that with this long-term stable and advanced automated firing system, depression of the gaseous emissions by about 90% related to manually operated fireplaces without catalyst could be achieved. In addition, preliminary investigations at a firing appliance complemented by an electrostatic precipitator yielded PM emission depression between 70% and 90%, depending on the firewood load. MDPI 2023-05-11 /pmc/articles/PMC10222192/ /pubmed/37430592 http://dx.doi.org/10.3390/s23104679 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Zhang, Xin
Ojha, Binayak
Bichlmaier, Hermann
Hartmann, Ingo
Kohler, Heinz
Extensive Gaseous Emissions Reduction of Firewood-Fueled Low Power Fireplaces by a Gas Sensor Based Advanced Combustion Airflow Control System and Catalytic Post-Oxidation
title Extensive Gaseous Emissions Reduction of Firewood-Fueled Low Power Fireplaces by a Gas Sensor Based Advanced Combustion Airflow Control System and Catalytic Post-Oxidation
title_full Extensive Gaseous Emissions Reduction of Firewood-Fueled Low Power Fireplaces by a Gas Sensor Based Advanced Combustion Airflow Control System and Catalytic Post-Oxidation
title_fullStr Extensive Gaseous Emissions Reduction of Firewood-Fueled Low Power Fireplaces by a Gas Sensor Based Advanced Combustion Airflow Control System and Catalytic Post-Oxidation
title_full_unstemmed Extensive Gaseous Emissions Reduction of Firewood-Fueled Low Power Fireplaces by a Gas Sensor Based Advanced Combustion Airflow Control System and Catalytic Post-Oxidation
title_short Extensive Gaseous Emissions Reduction of Firewood-Fueled Low Power Fireplaces by a Gas Sensor Based Advanced Combustion Airflow Control System and Catalytic Post-Oxidation
title_sort extensive gaseous emissions reduction of firewood-fueled low power fireplaces by a gas sensor based advanced combustion airflow control system and catalytic post-oxidation
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10222192/
https://www.ncbi.nlm.nih.gov/pubmed/37430592
http://dx.doi.org/10.3390/s23104679
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