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Transient gap generation in BaFe(2)As(2) driven by coherent lattice vibrations

Iron-based superconductors provide a rich platform to investigate the interplay between unconventional superconductivity, nematicity, and magnetism. The electronic structure and the magnetic properties of iron-based superconductors are highly sensitive to the pnictogen height. Coherent excitation of...

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Detalles Bibliográficos
Autores principales: Warshauer, Jacob A, Bustamante Lopez, Daniel Alejandro, Dong, Qingxin, Chen, Genfu, Hu, Wanzheng
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Oxford University Press 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10230283/
https://www.ncbi.nlm.nih.gov/pubmed/37266397
http://dx.doi.org/10.1093/pnasnexus/pgad164
Descripción
Sumario:Iron-based superconductors provide a rich platform to investigate the interplay between unconventional superconductivity, nematicity, and magnetism. The electronic structure and the magnetic properties of iron-based superconductors are highly sensitive to the pnictogen height. Coherent excitation of the [Formula: see text] phonon by femtosecond laser directly modulates the pnictogen height, which has been used to control the physical properties of iron-based superconductors. Previous studies show that the driven [Formula: see text] phonon resulted in a transient increase of the pnictogen height in BaFe [Formula: see text] As [Formula: see text] , favoring an enhanced Fe magnetic moment. However, there are no direct observations on either the enhanced Fe magnetic moments or the enhanced spin-density wave (SDW) gap. Here, we use time-resolved broadband terahertz spectroscopy to investigate the dynamics of BaFe [Formula: see text] As [Formula: see text] in the [Formula: see text] phonon-driven state. Below the SDW transition temperature, we observe a transient gap generation at early-time delays. A similar transient feature is observed in the normal state up to room temperature.