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Transient gap generation in BaFe(2)As(2) driven by coherent lattice vibrations

Iron-based superconductors provide a rich platform to investigate the interplay between unconventional superconductivity, nematicity, and magnetism. The electronic structure and the magnetic properties of iron-based superconductors are highly sensitive to the pnictogen height. Coherent excitation of...

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Autores principales: Warshauer, Jacob A, Bustamante Lopez, Daniel Alejandro, Dong, Qingxin, Chen, Genfu, Hu, Wanzheng
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Oxford University Press 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10230283/
https://www.ncbi.nlm.nih.gov/pubmed/37266397
http://dx.doi.org/10.1093/pnasnexus/pgad164
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author Warshauer, Jacob A
Bustamante Lopez, Daniel Alejandro
Dong, Qingxin
Chen, Genfu
Hu, Wanzheng
author_facet Warshauer, Jacob A
Bustamante Lopez, Daniel Alejandro
Dong, Qingxin
Chen, Genfu
Hu, Wanzheng
author_sort Warshauer, Jacob A
collection PubMed
description Iron-based superconductors provide a rich platform to investigate the interplay between unconventional superconductivity, nematicity, and magnetism. The electronic structure and the magnetic properties of iron-based superconductors are highly sensitive to the pnictogen height. Coherent excitation of the [Formula: see text] phonon by femtosecond laser directly modulates the pnictogen height, which has been used to control the physical properties of iron-based superconductors. Previous studies show that the driven [Formula: see text] phonon resulted in a transient increase of the pnictogen height in BaFe [Formula: see text] As [Formula: see text] , favoring an enhanced Fe magnetic moment. However, there are no direct observations on either the enhanced Fe magnetic moments or the enhanced spin-density wave (SDW) gap. Here, we use time-resolved broadband terahertz spectroscopy to investigate the dynamics of BaFe [Formula: see text] As [Formula: see text] in the [Formula: see text] phonon-driven state. Below the SDW transition temperature, we observe a transient gap generation at early-time delays. A similar transient feature is observed in the normal state up to room temperature.
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spelling pubmed-102302832023-06-01 Transient gap generation in BaFe(2)As(2) driven by coherent lattice vibrations Warshauer, Jacob A Bustamante Lopez, Daniel Alejandro Dong, Qingxin Chen, Genfu Hu, Wanzheng PNAS Nexus Physical Sciences and Engineering Iron-based superconductors provide a rich platform to investigate the interplay between unconventional superconductivity, nematicity, and magnetism. The electronic structure and the magnetic properties of iron-based superconductors are highly sensitive to the pnictogen height. Coherent excitation of the [Formula: see text] phonon by femtosecond laser directly modulates the pnictogen height, which has been used to control the physical properties of iron-based superconductors. Previous studies show that the driven [Formula: see text] phonon resulted in a transient increase of the pnictogen height in BaFe [Formula: see text] As [Formula: see text] , favoring an enhanced Fe magnetic moment. However, there are no direct observations on either the enhanced Fe magnetic moments or the enhanced spin-density wave (SDW) gap. Here, we use time-resolved broadband terahertz spectroscopy to investigate the dynamics of BaFe [Formula: see text] As [Formula: see text] in the [Formula: see text] phonon-driven state. Below the SDW transition temperature, we observe a transient gap generation at early-time delays. A similar transient feature is observed in the normal state up to room temperature. Oxford University Press 2023-05-16 /pmc/articles/PMC10230283/ /pubmed/37266397 http://dx.doi.org/10.1093/pnasnexus/pgad164 Text en © The Author(s) 2023. Published by Oxford University Press on behalf of National Academy of Sciences. https://creativecommons.org/licenses/by/4.0/This is an Open Access article distributed under the terms of the Creative Commons Attribution License (https://creativecommons.org/licenses/by/4.0/), which permits unrestricted reuse, distribution, and reproduction in any medium, provided the original work is properly cited.
spellingShingle Physical Sciences and Engineering
Warshauer, Jacob A
Bustamante Lopez, Daniel Alejandro
Dong, Qingxin
Chen, Genfu
Hu, Wanzheng
Transient gap generation in BaFe(2)As(2) driven by coherent lattice vibrations
title Transient gap generation in BaFe(2)As(2) driven by coherent lattice vibrations
title_full Transient gap generation in BaFe(2)As(2) driven by coherent lattice vibrations
title_fullStr Transient gap generation in BaFe(2)As(2) driven by coherent lattice vibrations
title_full_unstemmed Transient gap generation in BaFe(2)As(2) driven by coherent lattice vibrations
title_short Transient gap generation in BaFe(2)As(2) driven by coherent lattice vibrations
title_sort transient gap generation in bafe(2)as(2) driven by coherent lattice vibrations
topic Physical Sciences and Engineering
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10230283/
https://www.ncbi.nlm.nih.gov/pubmed/37266397
http://dx.doi.org/10.1093/pnasnexus/pgad164
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