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Unreported VOC Emissions from Road Transport Including from Electric Vehicles

[Image: see text] There are widespread policy assumptions that the phase-out of gasoline and diesel internal combustion engines will over time lead to much reduced emissions of Volatile Organic Compounds (VOCs) from road transport and related fuels. However, the use of real-world emissions measureme...

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Autores principales: Cliff, Samuel J., Lewis, Alastair C., Shaw, Marvin D., Lee, James D., Flynn, Michael, Andrews, Stephen J., Hopkins, James R., Purvis, Ruth M., Yeoman, Amber M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10233797/
https://www.ncbi.nlm.nih.gov/pubmed/37191998
http://dx.doi.org/10.1021/acs.est.3c00845
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author Cliff, Samuel J.
Lewis, Alastair C.
Shaw, Marvin D.
Lee, James D.
Flynn, Michael
Andrews, Stephen J.
Hopkins, James R.
Purvis, Ruth M.
Yeoman, Amber M.
author_facet Cliff, Samuel J.
Lewis, Alastair C.
Shaw, Marvin D.
Lee, James D.
Flynn, Michael
Andrews, Stephen J.
Hopkins, James R.
Purvis, Ruth M.
Yeoman, Amber M.
author_sort Cliff, Samuel J.
collection PubMed
description [Image: see text] There are widespread policy assumptions that the phase-out of gasoline and diesel internal combustion engines will over time lead to much reduced emissions of Volatile Organic Compounds (VOCs) from road transport and related fuels. However, the use of real-world emissions measurements from a new mobile air quality monitoring station demonstrated a large underestimation of alcohol-based species in road transport emissions inventories. Scaling of industry sales statistics enabled the discrepancy to be attributed to the use of ancillary solvent products such as screenwash and deicer which are not included in internationally applied vehicle emission methodologies. A fleet average nonfuel nonexhaust VOC emission factor of 58 ± 39 mg veh(–1) km(–1) was calculated for the missing source, which is greater than the total of all VOCs emitted from vehicle exhausts and their associated evaporative fuel losses. These emissions are independent of the vehicle energy/propulsion system and therefore applicable to all road vehicle types including those with battery-electric powertrains. In contrast to predictions, vehicle VOC emissions may actually increase given a predicted growth in total vehicle kilometers driven in a future electrified fleet and will undergo a complete VOC respeciation due to the source change.
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spelling pubmed-102337972023-06-02 Unreported VOC Emissions from Road Transport Including from Electric Vehicles Cliff, Samuel J. Lewis, Alastair C. Shaw, Marvin D. Lee, James D. Flynn, Michael Andrews, Stephen J. Hopkins, James R. Purvis, Ruth M. Yeoman, Amber M. Environ Sci Technol [Image: see text] There are widespread policy assumptions that the phase-out of gasoline and diesel internal combustion engines will over time lead to much reduced emissions of Volatile Organic Compounds (VOCs) from road transport and related fuels. However, the use of real-world emissions measurements from a new mobile air quality monitoring station demonstrated a large underestimation of alcohol-based species in road transport emissions inventories. Scaling of industry sales statistics enabled the discrepancy to be attributed to the use of ancillary solvent products such as screenwash and deicer which are not included in internationally applied vehicle emission methodologies. A fleet average nonfuel nonexhaust VOC emission factor of 58 ± 39 mg veh(–1) km(–1) was calculated for the missing source, which is greater than the total of all VOCs emitted from vehicle exhausts and their associated evaporative fuel losses. These emissions are independent of the vehicle energy/propulsion system and therefore applicable to all road vehicle types including those with battery-electric powertrains. In contrast to predictions, vehicle VOC emissions may actually increase given a predicted growth in total vehicle kilometers driven in a future electrified fleet and will undergo a complete VOC respeciation due to the source change. American Chemical Society 2023-05-16 /pmc/articles/PMC10233797/ /pubmed/37191998 http://dx.doi.org/10.1021/acs.est.3c00845 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Cliff, Samuel J.
Lewis, Alastair C.
Shaw, Marvin D.
Lee, James D.
Flynn, Michael
Andrews, Stephen J.
Hopkins, James R.
Purvis, Ruth M.
Yeoman, Amber M.
Unreported VOC Emissions from Road Transport Including from Electric Vehicles
title Unreported VOC Emissions from Road Transport Including from Electric Vehicles
title_full Unreported VOC Emissions from Road Transport Including from Electric Vehicles
title_fullStr Unreported VOC Emissions from Road Transport Including from Electric Vehicles
title_full_unstemmed Unreported VOC Emissions from Road Transport Including from Electric Vehicles
title_short Unreported VOC Emissions from Road Transport Including from Electric Vehicles
title_sort unreported voc emissions from road transport including from electric vehicles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10233797/
https://www.ncbi.nlm.nih.gov/pubmed/37191998
http://dx.doi.org/10.1021/acs.est.3c00845
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