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Towards High-Efficiency Photon Trapping in Thin-Film Perovskite Solar Cells Using Etched Fractal Metadevices

Reflective loss is one of the main factors contributing to power conversion efficiency limitation in thin-film perovskite solar cells. This issue has been tackled through several approaches, such as anti-reflective coatings, surface texturing, or superficial light-trapping metastructures. We report...

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Autores principales: Bărar, Ana, Maclean, Stephen Akwei, Dănilă, Octavian, Taylor, André D.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10254356/
https://www.ncbi.nlm.nih.gov/pubmed/37297068
http://dx.doi.org/10.3390/ma16113934
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author Bărar, Ana
Maclean, Stephen Akwei
Dănilă, Octavian
Taylor, André D.
author_facet Bărar, Ana
Maclean, Stephen Akwei
Dănilă, Octavian
Taylor, André D.
author_sort Bărar, Ana
collection PubMed
description Reflective loss is one of the main factors contributing to power conversion efficiency limitation in thin-film perovskite solar cells. This issue has been tackled through several approaches, such as anti-reflective coatings, surface texturing, or superficial light-trapping metastructures. We report detailed simulation-based investigations on the photon trapping capabilities of a standard Methylammonium Lead Iodide (MAPbI [Formula: see text]) solar cell, with its top layer conveniently designed as a fractal metadevice, to reach a reflection value [Formula: see text] in the visible domain. Our results show that, under certain architecture configurations, reflection values below 0.1 are obtained throughout the visible domain. This represents a net improvement when compared to the 0.25 reflection yielded by a reference MAPbI [Formula: see text] having a plane surface, under identical simulation conditions. We also present the minimum architectural requirements of the metadevice by comparing it to simpler structures of the same family and performing a comparative study. Furthermore, the designed metadevice presents low power dissipation and exhibits approximately similar behavior regardless of the incident polarization angle. As a result, the proposed system is a viable candidate for being a standard requirement in obtaining high-efficiency perovskite solar cells.
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spelling pubmed-102543562023-06-10 Towards High-Efficiency Photon Trapping in Thin-Film Perovskite Solar Cells Using Etched Fractal Metadevices Bărar, Ana Maclean, Stephen Akwei Dănilă, Octavian Taylor, André D. Materials (Basel) Article Reflective loss is one of the main factors contributing to power conversion efficiency limitation in thin-film perovskite solar cells. This issue has been tackled through several approaches, such as anti-reflective coatings, surface texturing, or superficial light-trapping metastructures. We report detailed simulation-based investigations on the photon trapping capabilities of a standard Methylammonium Lead Iodide (MAPbI [Formula: see text]) solar cell, with its top layer conveniently designed as a fractal metadevice, to reach a reflection value [Formula: see text] in the visible domain. Our results show that, under certain architecture configurations, reflection values below 0.1 are obtained throughout the visible domain. This represents a net improvement when compared to the 0.25 reflection yielded by a reference MAPbI [Formula: see text] having a plane surface, under identical simulation conditions. We also present the minimum architectural requirements of the metadevice by comparing it to simpler structures of the same family and performing a comparative study. Furthermore, the designed metadevice presents low power dissipation and exhibits approximately similar behavior regardless of the incident polarization angle. As a result, the proposed system is a viable candidate for being a standard requirement in obtaining high-efficiency perovskite solar cells. MDPI 2023-05-24 /pmc/articles/PMC10254356/ /pubmed/37297068 http://dx.doi.org/10.3390/ma16113934 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Bărar, Ana
Maclean, Stephen Akwei
Dănilă, Octavian
Taylor, André D.
Towards High-Efficiency Photon Trapping in Thin-Film Perovskite Solar Cells Using Etched Fractal Metadevices
title Towards High-Efficiency Photon Trapping in Thin-Film Perovskite Solar Cells Using Etched Fractal Metadevices
title_full Towards High-Efficiency Photon Trapping in Thin-Film Perovskite Solar Cells Using Etched Fractal Metadevices
title_fullStr Towards High-Efficiency Photon Trapping in Thin-Film Perovskite Solar Cells Using Etched Fractal Metadevices
title_full_unstemmed Towards High-Efficiency Photon Trapping in Thin-Film Perovskite Solar Cells Using Etched Fractal Metadevices
title_short Towards High-Efficiency Photon Trapping in Thin-Film Perovskite Solar Cells Using Etched Fractal Metadevices
title_sort towards high-efficiency photon trapping in thin-film perovskite solar cells using etched fractal metadevices
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10254356/
https://www.ncbi.nlm.nih.gov/pubmed/37297068
http://dx.doi.org/10.3390/ma16113934
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