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Enabling Self-Induced Back-Action Trapping of Gold Nanoparticles in Metamaterial Plasmonic Tweezers

[Image: see text] The pursuit for efficient nanoparticle trapping with low powers has led to optical tweezers technology moving from the conventional free-space configuration to advanced plasmonic systems. However, trapping nanoparticles smaller than 10 nm still remains a challenge even for plasmoni...

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Autores principales: Bouloumis, Theodoros D., Kotsifaki, Domna G., Nic Chormaic, Síle
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10273476/
https://www.ncbi.nlm.nih.gov/pubmed/37256850
http://dx.doi.org/10.1021/acs.nanolett.2c04492
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author Bouloumis, Theodoros D.
Kotsifaki, Domna G.
Nic Chormaic, Síle
author_facet Bouloumis, Theodoros D.
Kotsifaki, Domna G.
Nic Chormaic, Síle
author_sort Bouloumis, Theodoros D.
collection PubMed
description [Image: see text] The pursuit for efficient nanoparticle trapping with low powers has led to optical tweezers technology moving from the conventional free-space configuration to advanced plasmonic systems. However, trapping nanoparticles smaller than 10 nm still remains a challenge even for plasmonic tweezers. Proper nanocavity design and excitation has given rise to the self-induced back-action (SIBA) effect offering enhanced trap stiffness with decreased laser power. In this work, we investigate the SIBA effect in metamaterial tweezers and its synergy with the exhibited Fano resonance. We demonstrate stable trapping of 20 nm gold particles with trap stiffnesses as high as 4.18 ± 0.2 (fN/nm)/(mW/μm(2)) and very low excitation intensity. Simulations reveal the existence of two different groups of hotspots on the plasmonic array. The two hotspots exhibit tunable trap stiffnesses, a unique feature that can allow for sorting of particles and biological molecules based on their characteristics.
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spelling pubmed-102734762023-06-17 Enabling Self-Induced Back-Action Trapping of Gold Nanoparticles in Metamaterial Plasmonic Tweezers Bouloumis, Theodoros D. Kotsifaki, Domna G. Nic Chormaic, Síle Nano Lett [Image: see text] The pursuit for efficient nanoparticle trapping with low powers has led to optical tweezers technology moving from the conventional free-space configuration to advanced plasmonic systems. However, trapping nanoparticles smaller than 10 nm still remains a challenge even for plasmonic tweezers. Proper nanocavity design and excitation has given rise to the self-induced back-action (SIBA) effect offering enhanced trap stiffness with decreased laser power. In this work, we investigate the SIBA effect in metamaterial tweezers and its synergy with the exhibited Fano resonance. We demonstrate stable trapping of 20 nm gold particles with trap stiffnesses as high as 4.18 ± 0.2 (fN/nm)/(mW/μm(2)) and very low excitation intensity. Simulations reveal the existence of two different groups of hotspots on the plasmonic array. The two hotspots exhibit tunable trap stiffnesses, a unique feature that can allow for sorting of particles and biological molecules based on their characteristics. American Chemical Society 2023-05-31 /pmc/articles/PMC10273476/ /pubmed/37256850 http://dx.doi.org/10.1021/acs.nanolett.2c04492 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Bouloumis, Theodoros D.
Kotsifaki, Domna G.
Nic Chormaic, Síle
Enabling Self-Induced Back-Action Trapping of Gold Nanoparticles in Metamaterial Plasmonic Tweezers
title Enabling Self-Induced Back-Action Trapping of Gold Nanoparticles in Metamaterial Plasmonic Tweezers
title_full Enabling Self-Induced Back-Action Trapping of Gold Nanoparticles in Metamaterial Plasmonic Tweezers
title_fullStr Enabling Self-Induced Back-Action Trapping of Gold Nanoparticles in Metamaterial Plasmonic Tweezers
title_full_unstemmed Enabling Self-Induced Back-Action Trapping of Gold Nanoparticles in Metamaterial Plasmonic Tweezers
title_short Enabling Self-Induced Back-Action Trapping of Gold Nanoparticles in Metamaterial Plasmonic Tweezers
title_sort enabling self-induced back-action trapping of gold nanoparticles in metamaterial plasmonic tweezers
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10273476/
https://www.ncbi.nlm.nih.gov/pubmed/37256850
http://dx.doi.org/10.1021/acs.nanolett.2c04492
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