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Ultrasound-assisted degradation of organophosphorus pesticide methidathion using CuFe(2)O(4)@SiO(2)-GO(COOH) as a magnetic separable sonocatalyst

Water contamination by pesticides is a critical environmental issue, necessitating the development of sustainable and efficient degradation methods. This study focuses on synthesizing and evaluating a novel heterogeneous sonocatalyst for degrading pesticide methidathion. The catalyst consists of gra...

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Autores principales: Maati, Houda, Amadine, Othmane, Essamlali, Younes, Aboulhrouz, Soumia, jioui, Ilham, Dânoun, Karim, Zahouily, Mohamed
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10305793/
https://www.ncbi.nlm.nih.gov/pubmed/37388148
http://dx.doi.org/10.1039/d3ra02773b
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author Maati, Houda
Amadine, Othmane
Essamlali, Younes
Aboulhrouz, Soumia
jioui, Ilham
Dânoun, Karim
Zahouily, Mohamed
author_facet Maati, Houda
Amadine, Othmane
Essamlali, Younes
Aboulhrouz, Soumia
jioui, Ilham
Dânoun, Karim
Zahouily, Mohamed
author_sort Maati, Houda
collection PubMed
description Water contamination by pesticides is a critical environmental issue, necessitating the development of sustainable and efficient degradation methods. This study focuses on synthesizing and evaluating a novel heterogeneous sonocatalyst for degrading pesticide methidathion. The catalyst consists of graphene oxide (GO) decorated CuFe(2)O(4)@SiO(2) nanocomposites. Comprehensive characterization using various techniques confirmed the superior sonocatalytic activity of the CuFe(2)O(4)@SiO(2)-GOCOOH nanocomposite compared to CuFe(2)O(4)@SiO(2) alone. The enhanced performance is attributed to the combined effects of GO and CuFe(2)O(4)@SiO(2), including increased surface area, enhanced adsorption capabilities, and efficient electron transfer pathways. Reaction parameters such as time, temperature, concentration, and pH significantly influenced the degradation efficiency of methidathion. Longer reaction times, higher temperatures, and lower initial pesticide concentrations favored faster degradation and higher efficiency. Optimal pH conditions were identified to ensure effective degradation. Remarkably, the catalyst demonstrated excellent recyclability, indicating its potential for practical implementation in pesticide-contaminated wastewater treatment. This research contributes to the development of sustainable methods for environmental remediation, highlighting the promising potential of the graphene oxide decorated CuFe(2)O(4)@SiO(2) nanocomposite as an effective heterogeneous sonocatalyst for pesticide degradation.
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spelling pubmed-103057932023-06-29 Ultrasound-assisted degradation of organophosphorus pesticide methidathion using CuFe(2)O(4)@SiO(2)-GO(COOH) as a magnetic separable sonocatalyst Maati, Houda Amadine, Othmane Essamlali, Younes Aboulhrouz, Soumia jioui, Ilham Dânoun, Karim Zahouily, Mohamed RSC Adv Chemistry Water contamination by pesticides is a critical environmental issue, necessitating the development of sustainable and efficient degradation methods. This study focuses on synthesizing and evaluating a novel heterogeneous sonocatalyst for degrading pesticide methidathion. The catalyst consists of graphene oxide (GO) decorated CuFe(2)O(4)@SiO(2) nanocomposites. Comprehensive characterization using various techniques confirmed the superior sonocatalytic activity of the CuFe(2)O(4)@SiO(2)-GOCOOH nanocomposite compared to CuFe(2)O(4)@SiO(2) alone. The enhanced performance is attributed to the combined effects of GO and CuFe(2)O(4)@SiO(2), including increased surface area, enhanced adsorption capabilities, and efficient electron transfer pathways. Reaction parameters such as time, temperature, concentration, and pH significantly influenced the degradation efficiency of methidathion. Longer reaction times, higher temperatures, and lower initial pesticide concentrations favored faster degradation and higher efficiency. Optimal pH conditions were identified to ensure effective degradation. Remarkably, the catalyst demonstrated excellent recyclability, indicating its potential for practical implementation in pesticide-contaminated wastewater treatment. This research contributes to the development of sustainable methods for environmental remediation, highlighting the promising potential of the graphene oxide decorated CuFe(2)O(4)@SiO(2) nanocomposite as an effective heterogeneous sonocatalyst for pesticide degradation. The Royal Society of Chemistry 2023-06-28 /pmc/articles/PMC10305793/ /pubmed/37388148 http://dx.doi.org/10.1039/d3ra02773b Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Maati, Houda
Amadine, Othmane
Essamlali, Younes
Aboulhrouz, Soumia
jioui, Ilham
Dânoun, Karim
Zahouily, Mohamed
Ultrasound-assisted degradation of organophosphorus pesticide methidathion using CuFe(2)O(4)@SiO(2)-GO(COOH) as a magnetic separable sonocatalyst
title Ultrasound-assisted degradation of organophosphorus pesticide methidathion using CuFe(2)O(4)@SiO(2)-GO(COOH) as a magnetic separable sonocatalyst
title_full Ultrasound-assisted degradation of organophosphorus pesticide methidathion using CuFe(2)O(4)@SiO(2)-GO(COOH) as a magnetic separable sonocatalyst
title_fullStr Ultrasound-assisted degradation of organophosphorus pesticide methidathion using CuFe(2)O(4)@SiO(2)-GO(COOH) as a magnetic separable sonocatalyst
title_full_unstemmed Ultrasound-assisted degradation of organophosphorus pesticide methidathion using CuFe(2)O(4)@SiO(2)-GO(COOH) as a magnetic separable sonocatalyst
title_short Ultrasound-assisted degradation of organophosphorus pesticide methidathion using CuFe(2)O(4)@SiO(2)-GO(COOH) as a magnetic separable sonocatalyst
title_sort ultrasound-assisted degradation of organophosphorus pesticide methidathion using cufe(2)o(4)@sio(2)-go(cooh) as a magnetic separable sonocatalyst
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10305793/
https://www.ncbi.nlm.nih.gov/pubmed/37388148
http://dx.doi.org/10.1039/d3ra02773b
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