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Chiral electroluminescence from thin-film perovskite metacavities
Chiral light sources realized in ultracompact device platforms are highly desirable for various applications. Among active media used for thin-film emission devices, lead-halide perovskites have been extensively studied for photoluminescence due to their exceptional properties. However, up to date,...
Autores principales: | , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Association for the Advancement of Science
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10306290/ https://www.ncbi.nlm.nih.gov/pubmed/37379382 http://dx.doi.org/10.1126/sciadv.adh0414 |
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author | Kim, Seongheon An, Soo-Chan Kim, Younggon Shin, Yun Seop Antonov, Alexander A. Seo, In Cheol Woo, Byung Hoon Lim, Yeonsoo Gorkunov, Maxim V. Kivshar, Yuri S. Kim, Jin Young Jun, Young Chul |
author_facet | Kim, Seongheon An, Soo-Chan Kim, Younggon Shin, Yun Seop Antonov, Alexander A. Seo, In Cheol Woo, Byung Hoon Lim, Yeonsoo Gorkunov, Maxim V. Kivshar, Yuri S. Kim, Jin Young Jun, Young Chul |
author_sort | Kim, Seongheon |
collection | PubMed |
description | Chiral light sources realized in ultracompact device platforms are highly desirable for various applications. Among active media used for thin-film emission devices, lead-halide perovskites have been extensively studied for photoluminescence due to their exceptional properties. However, up to date, there have been no demonstrations of chiral electroluminescence with a substantial degree of circular polarization (DCP) based on perovskite materials, being critical for the development of practical devices. Here, we propose a concept of chiral light sources based on a thin-film perovskite metacavity and experimentally demonstrate chiral electroluminescence with a peak DCP approaching 0.38. We design a metacavity created by a metal and a dielectric metasurface supporting photonic eigenstates with a close-to-maximum chiral response. Chiral cavity modes facilitate asymmetric electroluminescence of pairs of left and right circularly polarized waves propagating in the opposite oblique directions. The proposed ultracompact light sources are especially advantageous for many applications requiring chiral light beams of both helicities. |
format | Online Article Text |
id | pubmed-10306290 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | American Association for the Advancement of Science |
record_format | MEDLINE/PubMed |
spelling | pubmed-103062902023-06-29 Chiral electroluminescence from thin-film perovskite metacavities Kim, Seongheon An, Soo-Chan Kim, Younggon Shin, Yun Seop Antonov, Alexander A. Seo, In Cheol Woo, Byung Hoon Lim, Yeonsoo Gorkunov, Maxim V. Kivshar, Yuri S. Kim, Jin Young Jun, Young Chul Sci Adv Physical and Materials Sciences Chiral light sources realized in ultracompact device platforms are highly desirable for various applications. Among active media used for thin-film emission devices, lead-halide perovskites have been extensively studied for photoluminescence due to their exceptional properties. However, up to date, there have been no demonstrations of chiral electroluminescence with a substantial degree of circular polarization (DCP) based on perovskite materials, being critical for the development of practical devices. Here, we propose a concept of chiral light sources based on a thin-film perovskite metacavity and experimentally demonstrate chiral electroluminescence with a peak DCP approaching 0.38. We design a metacavity created by a metal and a dielectric metasurface supporting photonic eigenstates with a close-to-maximum chiral response. Chiral cavity modes facilitate asymmetric electroluminescence of pairs of left and right circularly polarized waves propagating in the opposite oblique directions. The proposed ultracompact light sources are especially advantageous for many applications requiring chiral light beams of both helicities. American Association for the Advancement of Science 2023-06-28 /pmc/articles/PMC10306290/ /pubmed/37379382 http://dx.doi.org/10.1126/sciadv.adh0414 Text en Copyright © 2023 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited. |
spellingShingle | Physical and Materials Sciences Kim, Seongheon An, Soo-Chan Kim, Younggon Shin, Yun Seop Antonov, Alexander A. Seo, In Cheol Woo, Byung Hoon Lim, Yeonsoo Gorkunov, Maxim V. Kivshar, Yuri S. Kim, Jin Young Jun, Young Chul Chiral electroluminescence from thin-film perovskite metacavities |
title | Chiral electroluminescence from thin-film perovskite metacavities |
title_full | Chiral electroluminescence from thin-film perovskite metacavities |
title_fullStr | Chiral electroluminescence from thin-film perovskite metacavities |
title_full_unstemmed | Chiral electroluminescence from thin-film perovskite metacavities |
title_short | Chiral electroluminescence from thin-film perovskite metacavities |
title_sort | chiral electroluminescence from thin-film perovskite metacavities |
topic | Physical and Materials Sciences |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10306290/ https://www.ncbi.nlm.nih.gov/pubmed/37379382 http://dx.doi.org/10.1126/sciadv.adh0414 |
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