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Chiral electroluminescence from thin-film perovskite metacavities

Chiral light sources realized in ultracompact device platforms are highly desirable for various applications. Among active media used for thin-film emission devices, lead-halide perovskites have been extensively studied for photoluminescence due to their exceptional properties. However, up to date,...

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Autores principales: Kim, Seongheon, An, Soo-Chan, Kim, Younggon, Shin, Yun Seop, Antonov, Alexander A., Seo, In Cheol, Woo, Byung Hoon, Lim, Yeonsoo, Gorkunov, Maxim V., Kivshar, Yuri S., Kim, Jin Young, Jun, Young Chul
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10306290/
https://www.ncbi.nlm.nih.gov/pubmed/37379382
http://dx.doi.org/10.1126/sciadv.adh0414
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author Kim, Seongheon
An, Soo-Chan
Kim, Younggon
Shin, Yun Seop
Antonov, Alexander A.
Seo, In Cheol
Woo, Byung Hoon
Lim, Yeonsoo
Gorkunov, Maxim V.
Kivshar, Yuri S.
Kim, Jin Young
Jun, Young Chul
author_facet Kim, Seongheon
An, Soo-Chan
Kim, Younggon
Shin, Yun Seop
Antonov, Alexander A.
Seo, In Cheol
Woo, Byung Hoon
Lim, Yeonsoo
Gorkunov, Maxim V.
Kivshar, Yuri S.
Kim, Jin Young
Jun, Young Chul
author_sort Kim, Seongheon
collection PubMed
description Chiral light sources realized in ultracompact device platforms are highly desirable for various applications. Among active media used for thin-film emission devices, lead-halide perovskites have been extensively studied for photoluminescence due to their exceptional properties. However, up to date, there have been no demonstrations of chiral electroluminescence with a substantial degree of circular polarization (DCP) based on perovskite materials, being critical for the development of practical devices. Here, we propose a concept of chiral light sources based on a thin-film perovskite metacavity and experimentally demonstrate chiral electroluminescence with a peak DCP approaching 0.38. We design a metacavity created by a metal and a dielectric metasurface supporting photonic eigenstates with a close-to-maximum chiral response. Chiral cavity modes facilitate asymmetric electroluminescence of pairs of left and right circularly polarized waves propagating in the opposite oblique directions. The proposed ultracompact light sources are especially advantageous for many applications requiring chiral light beams of both helicities.
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spelling pubmed-103062902023-06-29 Chiral electroluminescence from thin-film perovskite metacavities Kim, Seongheon An, Soo-Chan Kim, Younggon Shin, Yun Seop Antonov, Alexander A. Seo, In Cheol Woo, Byung Hoon Lim, Yeonsoo Gorkunov, Maxim V. Kivshar, Yuri S. Kim, Jin Young Jun, Young Chul Sci Adv Physical and Materials Sciences Chiral light sources realized in ultracompact device platforms are highly desirable for various applications. Among active media used for thin-film emission devices, lead-halide perovskites have been extensively studied for photoluminescence due to their exceptional properties. However, up to date, there have been no demonstrations of chiral electroluminescence with a substantial degree of circular polarization (DCP) based on perovskite materials, being critical for the development of practical devices. Here, we propose a concept of chiral light sources based on a thin-film perovskite metacavity and experimentally demonstrate chiral electroluminescence with a peak DCP approaching 0.38. We design a metacavity created by a metal and a dielectric metasurface supporting photonic eigenstates with a close-to-maximum chiral response. Chiral cavity modes facilitate asymmetric electroluminescence of pairs of left and right circularly polarized waves propagating in the opposite oblique directions. The proposed ultracompact light sources are especially advantageous for many applications requiring chiral light beams of both helicities. American Association for the Advancement of Science 2023-06-28 /pmc/articles/PMC10306290/ /pubmed/37379382 http://dx.doi.org/10.1126/sciadv.adh0414 Text en Copyright © 2023 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Physical and Materials Sciences
Kim, Seongheon
An, Soo-Chan
Kim, Younggon
Shin, Yun Seop
Antonov, Alexander A.
Seo, In Cheol
Woo, Byung Hoon
Lim, Yeonsoo
Gorkunov, Maxim V.
Kivshar, Yuri S.
Kim, Jin Young
Jun, Young Chul
Chiral electroluminescence from thin-film perovskite metacavities
title Chiral electroluminescence from thin-film perovskite metacavities
title_full Chiral electroluminescence from thin-film perovskite metacavities
title_fullStr Chiral electroluminescence from thin-film perovskite metacavities
title_full_unstemmed Chiral electroluminescence from thin-film perovskite metacavities
title_short Chiral electroluminescence from thin-film perovskite metacavities
title_sort chiral electroluminescence from thin-film perovskite metacavities
topic Physical and Materials Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10306290/
https://www.ncbi.nlm.nih.gov/pubmed/37379382
http://dx.doi.org/10.1126/sciadv.adh0414
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