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Room Temperature Exciton–Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum

[Image: see text] We show the first experimental demonstration of room-temperature exciton–polariton (EP) condensation from a bound state in the continuum (BIC). This demonstration is achieved by strongly coupling stable excitons in an organic perylene dye with the extremely long-lived BIC in a diel...

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Autores principales: Berghuis, Anton Matthijs, Castellanos, Gabriel W., Murai, Shunsuke, Pura, Jose Luis, Abujetas, Diego R., van Heijst, Erik, Ramezani, Mohammad, Sánchez-Gil, José A., Rivas, Jaime Gómez
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10311526/
https://www.ncbi.nlm.nih.gov/pubmed/37310271
http://dx.doi.org/10.1021/acs.nanolett.3c01102
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author Berghuis, Anton Matthijs
Castellanos, Gabriel W.
Murai, Shunsuke
Pura, Jose Luis
Abujetas, Diego R.
van Heijst, Erik
Ramezani, Mohammad
Sánchez-Gil, José A.
Rivas, Jaime Gómez
author_facet Berghuis, Anton Matthijs
Castellanos, Gabriel W.
Murai, Shunsuke
Pura, Jose Luis
Abujetas, Diego R.
van Heijst, Erik
Ramezani, Mohammad
Sánchez-Gil, José A.
Rivas, Jaime Gómez
author_sort Berghuis, Anton Matthijs
collection PubMed
description [Image: see text] We show the first experimental demonstration of room-temperature exciton–polariton (EP) condensation from a bound state in the continuum (BIC). This demonstration is achieved by strongly coupling stable excitons in an organic perylene dye with the extremely long-lived BIC in a dielectric metasurface of silicon nanoparticles. The long lifetime of the BIC, mainly due to the suppression of radiation leakage, allows for EP thermalization to the ground state before decaying. This property results in a condensation threshold of less than 5 μJ cm(–2), 1 order of magnitude lower than the lasing threshold reported in similar systems in the weak coupling limit.
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spelling pubmed-103115262023-07-01 Room Temperature Exciton–Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum Berghuis, Anton Matthijs Castellanos, Gabriel W. Murai, Shunsuke Pura, Jose Luis Abujetas, Diego R. van Heijst, Erik Ramezani, Mohammad Sánchez-Gil, José A. Rivas, Jaime Gómez Nano Lett [Image: see text] We show the first experimental demonstration of room-temperature exciton–polariton (EP) condensation from a bound state in the continuum (BIC). This demonstration is achieved by strongly coupling stable excitons in an organic perylene dye with the extremely long-lived BIC in a dielectric metasurface of silicon nanoparticles. The long lifetime of the BIC, mainly due to the suppression of radiation leakage, allows for EP thermalization to the ground state before decaying. This property results in a condensation threshold of less than 5 μJ cm(–2), 1 order of magnitude lower than the lasing threshold reported in similar systems in the weak coupling limit. American Chemical Society 2023-06-13 /pmc/articles/PMC10311526/ /pubmed/37310271 http://dx.doi.org/10.1021/acs.nanolett.3c01102 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Berghuis, Anton Matthijs
Castellanos, Gabriel W.
Murai, Shunsuke
Pura, Jose Luis
Abujetas, Diego R.
van Heijst, Erik
Ramezani, Mohammad
Sánchez-Gil, José A.
Rivas, Jaime Gómez
Room Temperature Exciton–Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum
title Room Temperature Exciton–Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum
title_full Room Temperature Exciton–Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum
title_fullStr Room Temperature Exciton–Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum
title_full_unstemmed Room Temperature Exciton–Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum
title_short Room Temperature Exciton–Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum
title_sort room temperature exciton–polariton condensation in silicon metasurfaces emerging from bound states in the continuum
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10311526/
https://www.ncbi.nlm.nih.gov/pubmed/37310271
http://dx.doi.org/10.1021/acs.nanolett.3c01102
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