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Room Temperature Exciton–Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum
[Image: see text] We show the first experimental demonstration of room-temperature exciton–polariton (EP) condensation from a bound state in the continuum (BIC). This demonstration is achieved by strongly coupling stable excitons in an organic perylene dye with the extremely long-lived BIC in a diel...
Autores principales: | , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2023
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10311526/ https://www.ncbi.nlm.nih.gov/pubmed/37310271 http://dx.doi.org/10.1021/acs.nanolett.3c01102 |
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author | Berghuis, Anton Matthijs Castellanos, Gabriel W. Murai, Shunsuke Pura, Jose Luis Abujetas, Diego R. van Heijst, Erik Ramezani, Mohammad Sánchez-Gil, José A. Rivas, Jaime Gómez |
author_facet | Berghuis, Anton Matthijs Castellanos, Gabriel W. Murai, Shunsuke Pura, Jose Luis Abujetas, Diego R. van Heijst, Erik Ramezani, Mohammad Sánchez-Gil, José A. Rivas, Jaime Gómez |
author_sort | Berghuis, Anton Matthijs |
collection | PubMed |
description | [Image: see text] We show the first experimental demonstration of room-temperature exciton–polariton (EP) condensation from a bound state in the continuum (BIC). This demonstration is achieved by strongly coupling stable excitons in an organic perylene dye with the extremely long-lived BIC in a dielectric metasurface of silicon nanoparticles. The long lifetime of the BIC, mainly due to the suppression of radiation leakage, allows for EP thermalization to the ground state before decaying. This property results in a condensation threshold of less than 5 μJ cm(–2), 1 order of magnitude lower than the lasing threshold reported in similar systems in the weak coupling limit. |
format | Online Article Text |
id | pubmed-10311526 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-103115262023-07-01 Room Temperature Exciton–Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum Berghuis, Anton Matthijs Castellanos, Gabriel W. Murai, Shunsuke Pura, Jose Luis Abujetas, Diego R. van Heijst, Erik Ramezani, Mohammad Sánchez-Gil, José A. Rivas, Jaime Gómez Nano Lett [Image: see text] We show the first experimental demonstration of room-temperature exciton–polariton (EP) condensation from a bound state in the continuum (BIC). This demonstration is achieved by strongly coupling stable excitons in an organic perylene dye with the extremely long-lived BIC in a dielectric metasurface of silicon nanoparticles. The long lifetime of the BIC, mainly due to the suppression of radiation leakage, allows for EP thermalization to the ground state before decaying. This property results in a condensation threshold of less than 5 μJ cm(–2), 1 order of magnitude lower than the lasing threshold reported in similar systems in the weak coupling limit. American Chemical Society 2023-06-13 /pmc/articles/PMC10311526/ /pubmed/37310271 http://dx.doi.org/10.1021/acs.nanolett.3c01102 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Berghuis, Anton Matthijs Castellanos, Gabriel W. Murai, Shunsuke Pura, Jose Luis Abujetas, Diego R. van Heijst, Erik Ramezani, Mohammad Sánchez-Gil, José A. Rivas, Jaime Gómez Room Temperature Exciton–Polariton Condensation in Silicon Metasurfaces Emerging from Bound States in the Continuum |
title | Room Temperature
Exciton–Polariton Condensation
in Silicon Metasurfaces Emerging from Bound States in the Continuum |
title_full | Room Temperature
Exciton–Polariton Condensation
in Silicon Metasurfaces Emerging from Bound States in the Continuum |
title_fullStr | Room Temperature
Exciton–Polariton Condensation
in Silicon Metasurfaces Emerging from Bound States in the Continuum |
title_full_unstemmed | Room Temperature
Exciton–Polariton Condensation
in Silicon Metasurfaces Emerging from Bound States in the Continuum |
title_short | Room Temperature
Exciton–Polariton Condensation
in Silicon Metasurfaces Emerging from Bound States in the Continuum |
title_sort | room temperature
exciton–polariton condensation
in silicon metasurfaces emerging from bound states in the continuum |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10311526/ https://www.ncbi.nlm.nih.gov/pubmed/37310271 http://dx.doi.org/10.1021/acs.nanolett.3c01102 |
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