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Ultrafast Coupling of Optical Near Fields to Low-Energy Electrons Probed in a Point-Projection Microscope
[Image: see text] We report the first observation of the coupling of strong optical near fields to wavepackets of free, 100 eV electrons with <50 fs temporal resolution in an ultrafast point-projection microscope. Optical near fields are created by excitation of a thin, nanometer-sized Yagi-Uda a...
Autores principales: | , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2023
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10311584/ https://www.ncbi.nlm.nih.gov/pubmed/37278447 http://dx.doi.org/10.1021/acs.nanolett.3c00738 |
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author | Wöste, Andreas Hergert, Germann Quenzel, Thomas Silies, Martin Wang, Dong Groß, Petra Lienau, Christoph |
author_facet | Wöste, Andreas Hergert, Germann Quenzel, Thomas Silies, Martin Wang, Dong Groß, Petra Lienau, Christoph |
author_sort | Wöste, Andreas |
collection | PubMed |
description | [Image: see text] We report the first observation of the coupling of strong optical near fields to wavepackets of free, 100 eV electrons with <50 fs temporal resolution in an ultrafast point-projection microscope. Optical near fields are created by excitation of a thin, nanometer-sized Yagi-Uda antenna, with 20 fs near-infrared laser pulses. Phase matching between electrons and near fields is achieved due to strong spatial confinement of the antenna near field. Energy-resolved projection images of the antenna are recorded in an optical pump–electron probe scheme. We show that the phase modulation of the electron by transverse-field components results in a transient electron deflection while longitudinal near-field components broaden the kinetic energy distribution. This low-energy electron near-field coupling is used here to characterize the chirp of the ultrafast electron wavepackets, acquired upon propagation from the electron emitter to the sample. Our results bring direct mapping of different vectorial components of highly localized optical near fields into reach. |
format | Online Article Text |
id | pubmed-10311584 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-103115842023-07-01 Ultrafast Coupling of Optical Near Fields to Low-Energy Electrons Probed in a Point-Projection Microscope Wöste, Andreas Hergert, Germann Quenzel, Thomas Silies, Martin Wang, Dong Groß, Petra Lienau, Christoph Nano Lett [Image: see text] We report the first observation of the coupling of strong optical near fields to wavepackets of free, 100 eV electrons with <50 fs temporal resolution in an ultrafast point-projection microscope. Optical near fields are created by excitation of a thin, nanometer-sized Yagi-Uda antenna, with 20 fs near-infrared laser pulses. Phase matching between electrons and near fields is achieved due to strong spatial confinement of the antenna near field. Energy-resolved projection images of the antenna are recorded in an optical pump–electron probe scheme. We show that the phase modulation of the electron by transverse-field components results in a transient electron deflection while longitudinal near-field components broaden the kinetic energy distribution. This low-energy electron near-field coupling is used here to characterize the chirp of the ultrafast electron wavepackets, acquired upon propagation from the electron emitter to the sample. Our results bring direct mapping of different vectorial components of highly localized optical near fields into reach. American Chemical Society 2023-06-06 /pmc/articles/PMC10311584/ /pubmed/37278447 http://dx.doi.org/10.1021/acs.nanolett.3c00738 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Wöste, Andreas Hergert, Germann Quenzel, Thomas Silies, Martin Wang, Dong Groß, Petra Lienau, Christoph Ultrafast Coupling of Optical Near Fields to Low-Energy Electrons Probed in a Point-Projection Microscope |
title | Ultrafast Coupling
of Optical Near Fields to Low-Energy
Electrons Probed in a Point-Projection Microscope |
title_full | Ultrafast Coupling
of Optical Near Fields to Low-Energy
Electrons Probed in a Point-Projection Microscope |
title_fullStr | Ultrafast Coupling
of Optical Near Fields to Low-Energy
Electrons Probed in a Point-Projection Microscope |
title_full_unstemmed | Ultrafast Coupling
of Optical Near Fields to Low-Energy
Electrons Probed in a Point-Projection Microscope |
title_short | Ultrafast Coupling
of Optical Near Fields to Low-Energy
Electrons Probed in a Point-Projection Microscope |
title_sort | ultrafast coupling
of optical near fields to low-energy
electrons probed in a point-projection microscope |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10311584/ https://www.ncbi.nlm.nih.gov/pubmed/37278447 http://dx.doi.org/10.1021/acs.nanolett.3c00738 |
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