Cargando…

Ultrafast Coupling of Optical Near Fields to Low-Energy Electrons Probed in a Point-Projection Microscope

[Image: see text] We report the first observation of the coupling of strong optical near fields to wavepackets of free, 100 eV electrons with <50 fs temporal resolution in an ultrafast point-projection microscope. Optical near fields are created by excitation of a thin, nanometer-sized Yagi-Uda a...

Descripción completa

Detalles Bibliográficos
Autores principales: Wöste, Andreas, Hergert, Germann, Quenzel, Thomas, Silies, Martin, Wang, Dong, Groß, Petra, Lienau, Christoph
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10311584/
https://www.ncbi.nlm.nih.gov/pubmed/37278447
http://dx.doi.org/10.1021/acs.nanolett.3c00738
_version_ 1785066772498481152
author Wöste, Andreas
Hergert, Germann
Quenzel, Thomas
Silies, Martin
Wang, Dong
Groß, Petra
Lienau, Christoph
author_facet Wöste, Andreas
Hergert, Germann
Quenzel, Thomas
Silies, Martin
Wang, Dong
Groß, Petra
Lienau, Christoph
author_sort Wöste, Andreas
collection PubMed
description [Image: see text] We report the first observation of the coupling of strong optical near fields to wavepackets of free, 100 eV electrons with <50 fs temporal resolution in an ultrafast point-projection microscope. Optical near fields are created by excitation of a thin, nanometer-sized Yagi-Uda antenna, with 20 fs near-infrared laser pulses. Phase matching between electrons and near fields is achieved due to strong spatial confinement of the antenna near field. Energy-resolved projection images of the antenna are recorded in an optical pump–electron probe scheme. We show that the phase modulation of the electron by transverse-field components results in a transient electron deflection while longitudinal near-field components broaden the kinetic energy distribution. This low-energy electron near-field coupling is used here to characterize the chirp of the ultrafast electron wavepackets, acquired upon propagation from the electron emitter to the sample. Our results bring direct mapping of different vectorial components of highly localized optical near fields into reach.
format Online
Article
Text
id pubmed-10311584
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher American Chemical Society
record_format MEDLINE/PubMed
spelling pubmed-103115842023-07-01 Ultrafast Coupling of Optical Near Fields to Low-Energy Electrons Probed in a Point-Projection Microscope Wöste, Andreas Hergert, Germann Quenzel, Thomas Silies, Martin Wang, Dong Groß, Petra Lienau, Christoph Nano Lett [Image: see text] We report the first observation of the coupling of strong optical near fields to wavepackets of free, 100 eV electrons with <50 fs temporal resolution in an ultrafast point-projection microscope. Optical near fields are created by excitation of a thin, nanometer-sized Yagi-Uda antenna, with 20 fs near-infrared laser pulses. Phase matching between electrons and near fields is achieved due to strong spatial confinement of the antenna near field. Energy-resolved projection images of the antenna are recorded in an optical pump–electron probe scheme. We show that the phase modulation of the electron by transverse-field components results in a transient electron deflection while longitudinal near-field components broaden the kinetic energy distribution. This low-energy electron near-field coupling is used here to characterize the chirp of the ultrafast electron wavepackets, acquired upon propagation from the electron emitter to the sample. Our results bring direct mapping of different vectorial components of highly localized optical near fields into reach. American Chemical Society 2023-06-06 /pmc/articles/PMC10311584/ /pubmed/37278447 http://dx.doi.org/10.1021/acs.nanolett.3c00738 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Wöste, Andreas
Hergert, Germann
Quenzel, Thomas
Silies, Martin
Wang, Dong
Groß, Petra
Lienau, Christoph
Ultrafast Coupling of Optical Near Fields to Low-Energy Electrons Probed in a Point-Projection Microscope
title Ultrafast Coupling of Optical Near Fields to Low-Energy Electrons Probed in a Point-Projection Microscope
title_full Ultrafast Coupling of Optical Near Fields to Low-Energy Electrons Probed in a Point-Projection Microscope
title_fullStr Ultrafast Coupling of Optical Near Fields to Low-Energy Electrons Probed in a Point-Projection Microscope
title_full_unstemmed Ultrafast Coupling of Optical Near Fields to Low-Energy Electrons Probed in a Point-Projection Microscope
title_short Ultrafast Coupling of Optical Near Fields to Low-Energy Electrons Probed in a Point-Projection Microscope
title_sort ultrafast coupling of optical near fields to low-energy electrons probed in a point-projection microscope
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10311584/
https://www.ncbi.nlm.nih.gov/pubmed/37278447
http://dx.doi.org/10.1021/acs.nanolett.3c00738
work_keys_str_mv AT wosteandreas ultrafastcouplingofopticalnearfieldstolowenergyelectronsprobedinapointprojectionmicroscope
AT hergertgermann ultrafastcouplingofopticalnearfieldstolowenergyelectronsprobedinapointprojectionmicroscope
AT quenzelthomas ultrafastcouplingofopticalnearfieldstolowenergyelectronsprobedinapointprojectionmicroscope
AT siliesmartin ultrafastcouplingofopticalnearfieldstolowenergyelectronsprobedinapointprojectionmicroscope
AT wangdong ultrafastcouplingofopticalnearfieldstolowenergyelectronsprobedinapointprojectionmicroscope
AT großpetra ultrafastcouplingofopticalnearfieldstolowenergyelectronsprobedinapointprojectionmicroscope
AT lienauchristoph ultrafastcouplingofopticalnearfieldstolowenergyelectronsprobedinapointprojectionmicroscope