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Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES

Combining experimental set up and ab initio molecular dynamics simulations, we were able to follow the time evolution of the X-ray absorption near edge spectrum (XANES) of a dense copper plasma. This provides a deep insight into femtosecond laser interaction with a metallic copper target. This paper...

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Detalles Bibliográficos
Autores principales: Lecherbourg, Ludovic, Recoules, Vanina, Renaudin, Patrick, Dorchies, Fabien
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10315214/
https://www.ncbi.nlm.nih.gov/pubmed/37393940
http://dx.doi.org/10.1098/rsta.2022.0214
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author Lecherbourg, Ludovic
Recoules, Vanina
Renaudin, Patrick
Dorchies, Fabien
author_facet Lecherbourg, Ludovic
Recoules, Vanina
Renaudin, Patrick
Dorchies, Fabien
author_sort Lecherbourg, Ludovic
collection PubMed
description Combining experimental set up and ab initio molecular dynamics simulations, we were able to follow the time evolution of the X-ray absorption near edge spectrum (XANES) of a dense copper plasma. This provides a deep insight into femtosecond laser interaction with a metallic copper target. This paper presents a review of the experimental developments we made to reduce the X-ray probe duration, from approximately 10 ps to fs duration with table-top laser systems. Moreover, we present microscopic scale simulations, performed with Density Functional Theory, as well as macroscopic simulations considering the Two-Temperature Model. These tools allow us to get a complete picture of the evolution of the target at a microscopic level, from the heating process to the melting and expansion stages, with a clear view of the physics involved during these processes. This article is part of the theme issue ‘Dynamic and transient processes in warm dense matter’.
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spelling pubmed-103152142023-07-03 Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES Lecherbourg, Ludovic Recoules, Vanina Renaudin, Patrick Dorchies, Fabien Philos Trans A Math Phys Eng Sci Articles Combining experimental set up and ab initio molecular dynamics simulations, we were able to follow the time evolution of the X-ray absorption near edge spectrum (XANES) of a dense copper plasma. This provides a deep insight into femtosecond laser interaction with a metallic copper target. This paper presents a review of the experimental developments we made to reduce the X-ray probe duration, from approximately 10 ps to fs duration with table-top laser systems. Moreover, we present microscopic scale simulations, performed with Density Functional Theory, as well as macroscopic simulations considering the Two-Temperature Model. These tools allow us to get a complete picture of the evolution of the target at a microscopic level, from the heating process to the melting and expansion stages, with a clear view of the physics involved during these processes. This article is part of the theme issue ‘Dynamic and transient processes in warm dense matter’. The Royal Society 2023-08-21 2023-07-03 /pmc/articles/PMC10315214/ /pubmed/37393940 http://dx.doi.org/10.1098/rsta.2022.0214 Text en © 2023 The Authors. https://creativecommons.org/licenses/by/4.0/Published by the Royal Society under the terms of the Creative Commons Attribution License http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) , which permits unrestricted use, provided the original author and source are credited.
spellingShingle Articles
Lecherbourg, Ludovic
Recoules, Vanina
Renaudin, Patrick
Dorchies, Fabien
Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES
title Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES
title_full Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES
title_fullStr Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES
title_full_unstemmed Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES
title_short Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES
title_sort dynamics of femtosecond heated warm dense copper with time-resolved l3-edge xanes
topic Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10315214/
https://www.ncbi.nlm.nih.gov/pubmed/37393940
http://dx.doi.org/10.1098/rsta.2022.0214
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