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Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES
Combining experimental set up and ab initio molecular dynamics simulations, we were able to follow the time evolution of the X-ray absorption near edge spectrum (XANES) of a dense copper plasma. This provides a deep insight into femtosecond laser interaction with a metallic copper target. This paper...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
The Royal Society
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10315214/ https://www.ncbi.nlm.nih.gov/pubmed/37393940 http://dx.doi.org/10.1098/rsta.2022.0214 |
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author | Lecherbourg, Ludovic Recoules, Vanina Renaudin, Patrick Dorchies, Fabien |
author_facet | Lecherbourg, Ludovic Recoules, Vanina Renaudin, Patrick Dorchies, Fabien |
author_sort | Lecherbourg, Ludovic |
collection | PubMed |
description | Combining experimental set up and ab initio molecular dynamics simulations, we were able to follow the time evolution of the X-ray absorption near edge spectrum (XANES) of a dense copper plasma. This provides a deep insight into femtosecond laser interaction with a metallic copper target. This paper presents a review of the experimental developments we made to reduce the X-ray probe duration, from approximately 10 ps to fs duration with table-top laser systems. Moreover, we present microscopic scale simulations, performed with Density Functional Theory, as well as macroscopic simulations considering the Two-Temperature Model. These tools allow us to get a complete picture of the evolution of the target at a microscopic level, from the heating process to the melting and expansion stages, with a clear view of the physics involved during these processes. This article is part of the theme issue ‘Dynamic and transient processes in warm dense matter’. |
format | Online Article Text |
id | pubmed-10315214 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | The Royal Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-103152142023-07-03 Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES Lecherbourg, Ludovic Recoules, Vanina Renaudin, Patrick Dorchies, Fabien Philos Trans A Math Phys Eng Sci Articles Combining experimental set up and ab initio molecular dynamics simulations, we were able to follow the time evolution of the X-ray absorption near edge spectrum (XANES) of a dense copper plasma. This provides a deep insight into femtosecond laser interaction with a metallic copper target. This paper presents a review of the experimental developments we made to reduce the X-ray probe duration, from approximately 10 ps to fs duration with table-top laser systems. Moreover, we present microscopic scale simulations, performed with Density Functional Theory, as well as macroscopic simulations considering the Two-Temperature Model. These tools allow us to get a complete picture of the evolution of the target at a microscopic level, from the heating process to the melting and expansion stages, with a clear view of the physics involved during these processes. This article is part of the theme issue ‘Dynamic and transient processes in warm dense matter’. The Royal Society 2023-08-21 2023-07-03 /pmc/articles/PMC10315214/ /pubmed/37393940 http://dx.doi.org/10.1098/rsta.2022.0214 Text en © 2023 The Authors. https://creativecommons.org/licenses/by/4.0/Published by the Royal Society under the terms of the Creative Commons Attribution License http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) , which permits unrestricted use, provided the original author and source are credited. |
spellingShingle | Articles Lecherbourg, Ludovic Recoules, Vanina Renaudin, Patrick Dorchies, Fabien Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES |
title | Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES |
title_full | Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES |
title_fullStr | Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES |
title_full_unstemmed | Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES |
title_short | Dynamics of femtosecond heated warm dense copper with time-resolved L3-edge XANES |
title_sort | dynamics of femtosecond heated warm dense copper with time-resolved l3-edge xanes |
topic | Articles |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10315214/ https://www.ncbi.nlm.nih.gov/pubmed/37393940 http://dx.doi.org/10.1098/rsta.2022.0214 |
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