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Electrical control of hybrid exciton transport in a van der Waals heterostructure

Interactions between out-of-plane dipoles in bosonic gases enable the long-range propagation of excitons. The lack of direct control over collective dipolar properties has so far limited the degrees of tunability and the microscopic understanding of exciton transport. In this work we modulate the la...

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Autores principales: Tagarelli, Fedele, Lopriore, Edoardo, Erkensten, Daniel, Perea-Causín, Raül, Brem, Samuel, Hagel, Joakim, Sun, Zhe, Pasquale, Gabriele, Watanabe, Kenji, Taniguchi, Takashi, Malic, Ermin, Kis, Andras
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10322698/
https://www.ncbi.nlm.nih.gov/pubmed/37426431
http://dx.doi.org/10.1038/s41566-023-01198-w
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author Tagarelli, Fedele
Lopriore, Edoardo
Erkensten, Daniel
Perea-Causín, Raül
Brem, Samuel
Hagel, Joakim
Sun, Zhe
Pasquale, Gabriele
Watanabe, Kenji
Taniguchi, Takashi
Malic, Ermin
Kis, Andras
author_facet Tagarelli, Fedele
Lopriore, Edoardo
Erkensten, Daniel
Perea-Causín, Raül
Brem, Samuel
Hagel, Joakim
Sun, Zhe
Pasquale, Gabriele
Watanabe, Kenji
Taniguchi, Takashi
Malic, Ermin
Kis, Andras
author_sort Tagarelli, Fedele
collection PubMed
description Interactions between out-of-plane dipoles in bosonic gases enable the long-range propagation of excitons. The lack of direct control over collective dipolar properties has so far limited the degrees of tunability and the microscopic understanding of exciton transport. In this work we modulate the layer hybridization and interplay between many-body interactions of excitons in a van der Waals heterostructure with an applied vertical electric field. By performing spatiotemporally resolved measurements supported by microscopic theory, we uncover the dipole-dependent properties and transport of excitons with different degrees of hybridization. Moreover, we find constant emission quantum yields of the transporting species as a function of excitation power with radiative decay mechanisms dominating over nonradiative ones, a fundamental requirement for efficient excitonic devices. Our findings provide a complete picture of the many-body effects in the transport of dilute exciton gases, and have crucial implications for studying emerging states of matter such as Bose–Einstein condensation and optoelectronic applications based on exciton propagation.
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spelling pubmed-103226982023-07-07 Electrical control of hybrid exciton transport in a van der Waals heterostructure Tagarelli, Fedele Lopriore, Edoardo Erkensten, Daniel Perea-Causín, Raül Brem, Samuel Hagel, Joakim Sun, Zhe Pasquale, Gabriele Watanabe, Kenji Taniguchi, Takashi Malic, Ermin Kis, Andras Nat Photonics Article Interactions between out-of-plane dipoles in bosonic gases enable the long-range propagation of excitons. The lack of direct control over collective dipolar properties has so far limited the degrees of tunability and the microscopic understanding of exciton transport. In this work we modulate the layer hybridization and interplay between many-body interactions of excitons in a van der Waals heterostructure with an applied vertical electric field. By performing spatiotemporally resolved measurements supported by microscopic theory, we uncover the dipole-dependent properties and transport of excitons with different degrees of hybridization. Moreover, we find constant emission quantum yields of the transporting species as a function of excitation power with radiative decay mechanisms dominating over nonradiative ones, a fundamental requirement for efficient excitonic devices. Our findings provide a complete picture of the many-body effects in the transport of dilute exciton gases, and have crucial implications for studying emerging states of matter such as Bose–Einstein condensation and optoelectronic applications based on exciton propagation. Nature Publishing Group UK 2023-04-20 2023 /pmc/articles/PMC10322698/ /pubmed/37426431 http://dx.doi.org/10.1038/s41566-023-01198-w Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Tagarelli, Fedele
Lopriore, Edoardo
Erkensten, Daniel
Perea-Causín, Raül
Brem, Samuel
Hagel, Joakim
Sun, Zhe
Pasquale, Gabriele
Watanabe, Kenji
Taniguchi, Takashi
Malic, Ermin
Kis, Andras
Electrical control of hybrid exciton transport in a van der Waals heterostructure
title Electrical control of hybrid exciton transport in a van der Waals heterostructure
title_full Electrical control of hybrid exciton transport in a van der Waals heterostructure
title_fullStr Electrical control of hybrid exciton transport in a van der Waals heterostructure
title_full_unstemmed Electrical control of hybrid exciton transport in a van der Waals heterostructure
title_short Electrical control of hybrid exciton transport in a van der Waals heterostructure
title_sort electrical control of hybrid exciton transport in a van der waals heterostructure
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10322698/
https://www.ncbi.nlm.nih.gov/pubmed/37426431
http://dx.doi.org/10.1038/s41566-023-01198-w
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