Cargando…
Electrical control of hybrid exciton transport in a van der Waals heterostructure
Interactions between out-of-plane dipoles in bosonic gases enable the long-range propagation of excitons. The lack of direct control over collective dipolar properties has so far limited the degrees of tunability and the microscopic understanding of exciton transport. In this work we modulate the la...
Autores principales: | , , , , , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2023
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10322698/ https://www.ncbi.nlm.nih.gov/pubmed/37426431 http://dx.doi.org/10.1038/s41566-023-01198-w |
_version_ | 1785068815726411776 |
---|---|
author | Tagarelli, Fedele Lopriore, Edoardo Erkensten, Daniel Perea-Causín, Raül Brem, Samuel Hagel, Joakim Sun, Zhe Pasquale, Gabriele Watanabe, Kenji Taniguchi, Takashi Malic, Ermin Kis, Andras |
author_facet | Tagarelli, Fedele Lopriore, Edoardo Erkensten, Daniel Perea-Causín, Raül Brem, Samuel Hagel, Joakim Sun, Zhe Pasquale, Gabriele Watanabe, Kenji Taniguchi, Takashi Malic, Ermin Kis, Andras |
author_sort | Tagarelli, Fedele |
collection | PubMed |
description | Interactions between out-of-plane dipoles in bosonic gases enable the long-range propagation of excitons. The lack of direct control over collective dipolar properties has so far limited the degrees of tunability and the microscopic understanding of exciton transport. In this work we modulate the layer hybridization and interplay between many-body interactions of excitons in a van der Waals heterostructure with an applied vertical electric field. By performing spatiotemporally resolved measurements supported by microscopic theory, we uncover the dipole-dependent properties and transport of excitons with different degrees of hybridization. Moreover, we find constant emission quantum yields of the transporting species as a function of excitation power with radiative decay mechanisms dominating over nonradiative ones, a fundamental requirement for efficient excitonic devices. Our findings provide a complete picture of the many-body effects in the transport of dilute exciton gases, and have crucial implications for studying emerging states of matter such as Bose–Einstein condensation and optoelectronic applications based on exciton propagation. |
format | Online Article Text |
id | pubmed-10322698 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-103226982023-07-07 Electrical control of hybrid exciton transport in a van der Waals heterostructure Tagarelli, Fedele Lopriore, Edoardo Erkensten, Daniel Perea-Causín, Raül Brem, Samuel Hagel, Joakim Sun, Zhe Pasquale, Gabriele Watanabe, Kenji Taniguchi, Takashi Malic, Ermin Kis, Andras Nat Photonics Article Interactions between out-of-plane dipoles in bosonic gases enable the long-range propagation of excitons. The lack of direct control over collective dipolar properties has so far limited the degrees of tunability and the microscopic understanding of exciton transport. In this work we modulate the layer hybridization and interplay between many-body interactions of excitons in a van der Waals heterostructure with an applied vertical electric field. By performing spatiotemporally resolved measurements supported by microscopic theory, we uncover the dipole-dependent properties and transport of excitons with different degrees of hybridization. Moreover, we find constant emission quantum yields of the transporting species as a function of excitation power with radiative decay mechanisms dominating over nonradiative ones, a fundamental requirement for efficient excitonic devices. Our findings provide a complete picture of the many-body effects in the transport of dilute exciton gases, and have crucial implications for studying emerging states of matter such as Bose–Einstein condensation and optoelectronic applications based on exciton propagation. Nature Publishing Group UK 2023-04-20 2023 /pmc/articles/PMC10322698/ /pubmed/37426431 http://dx.doi.org/10.1038/s41566-023-01198-w Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Tagarelli, Fedele Lopriore, Edoardo Erkensten, Daniel Perea-Causín, Raül Brem, Samuel Hagel, Joakim Sun, Zhe Pasquale, Gabriele Watanabe, Kenji Taniguchi, Takashi Malic, Ermin Kis, Andras Electrical control of hybrid exciton transport in a van der Waals heterostructure |
title | Electrical control of hybrid exciton transport in a van der Waals heterostructure |
title_full | Electrical control of hybrid exciton transport in a van der Waals heterostructure |
title_fullStr | Electrical control of hybrid exciton transport in a van der Waals heterostructure |
title_full_unstemmed | Electrical control of hybrid exciton transport in a van der Waals heterostructure |
title_short | Electrical control of hybrid exciton transport in a van der Waals heterostructure |
title_sort | electrical control of hybrid exciton transport in a van der waals heterostructure |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10322698/ https://www.ncbi.nlm.nih.gov/pubmed/37426431 http://dx.doi.org/10.1038/s41566-023-01198-w |
work_keys_str_mv | AT tagarellifedele electricalcontrolofhybridexcitontransportinavanderwaalsheterostructure AT loprioreedoardo electricalcontrolofhybridexcitontransportinavanderwaalsheterostructure AT erkenstendaniel electricalcontrolofhybridexcitontransportinavanderwaalsheterostructure AT pereacausinraul electricalcontrolofhybridexcitontransportinavanderwaalsheterostructure AT bremsamuel electricalcontrolofhybridexcitontransportinavanderwaalsheterostructure AT hageljoakim electricalcontrolofhybridexcitontransportinavanderwaalsheterostructure AT sunzhe electricalcontrolofhybridexcitontransportinavanderwaalsheterostructure AT pasqualegabriele electricalcontrolofhybridexcitontransportinavanderwaalsheterostructure AT watanabekenji electricalcontrolofhybridexcitontransportinavanderwaalsheterostructure AT taniguchitakashi electricalcontrolofhybridexcitontransportinavanderwaalsheterostructure AT malicermin electricalcontrolofhybridexcitontransportinavanderwaalsheterostructure AT kisandras electricalcontrolofhybridexcitontransportinavanderwaalsheterostructure |