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Broadband magnetic resonance spectroscopy in MnSc[Formula: see text] S[Formula: see text]
Recent neutron scattering experiments suggested that frustrated magnetic interactions give rise to antiferromagnetic spiral and fractional skyrmion lattice phases in MnSc[Formula: see text] S[Formula: see text] . Here, to trace the signatures of these modulated phases, we studied the spin excitatio...
Autores principales: | , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10329720/ https://www.ncbi.nlm.nih.gov/pubmed/37422590 http://dx.doi.org/10.1038/s41598-023-37911-6 |
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author | Tóth, Boglárka Amelin, Kirill Rõõm, Toomas Nagel, Urmas Bauernfeind, Anastasia Tsurkan, Vladimir Prodan, Lilian Krug von Nidda, Hans-Albrecht Scheffler, Marc Kézsmárki, István Bordács, Sándor |
author_facet | Tóth, Boglárka Amelin, Kirill Rõõm, Toomas Nagel, Urmas Bauernfeind, Anastasia Tsurkan, Vladimir Prodan, Lilian Krug von Nidda, Hans-Albrecht Scheffler, Marc Kézsmárki, István Bordács, Sándor |
author_sort | Tóth, Boglárka |
collection | PubMed |
description | Recent neutron scattering experiments suggested that frustrated magnetic interactions give rise to antiferromagnetic spiral and fractional skyrmion lattice phases in MnSc[Formula: see text] S[Formula: see text] . Here, to trace the signatures of these modulated phases, we studied the spin excitations of MnSc[Formula: see text] S[Formula: see text] by THz spectroscopy at 300 mK and in magnetic fields up to 12 T and by broadband microwave spectroscopy at various temperatures up to 50 GHz. We found a single magnetic resonance with frequency linearly increasing in field. The small deviation of the Mn[Formula: see text] ion g-factor from 2, g = 1.96, and the absence of other resonances imply very weak anisotropies and negligible contribution of higher harmonics to the spiral state. The significant difference between the dc magnetic susceptibility and the lowest-frequency ac susceptibility in our experiment implies the existence of mode(s) outside of the measured frequency windows. The combination of THz and microwave experiments suggests a spin gap opening below the ordering temperature between 50 GHz and 100 GHz. |
format | Online Article Text |
id | pubmed-10329720 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-103297202023-07-10 Broadband magnetic resonance spectroscopy in MnSc[Formula: see text] S[Formula: see text] Tóth, Boglárka Amelin, Kirill Rõõm, Toomas Nagel, Urmas Bauernfeind, Anastasia Tsurkan, Vladimir Prodan, Lilian Krug von Nidda, Hans-Albrecht Scheffler, Marc Kézsmárki, István Bordács, Sándor Sci Rep Article Recent neutron scattering experiments suggested that frustrated magnetic interactions give rise to antiferromagnetic spiral and fractional skyrmion lattice phases in MnSc[Formula: see text] S[Formula: see text] . Here, to trace the signatures of these modulated phases, we studied the spin excitations of MnSc[Formula: see text] S[Formula: see text] by THz spectroscopy at 300 mK and in magnetic fields up to 12 T and by broadband microwave spectroscopy at various temperatures up to 50 GHz. We found a single magnetic resonance with frequency linearly increasing in field. The small deviation of the Mn[Formula: see text] ion g-factor from 2, g = 1.96, and the absence of other resonances imply very weak anisotropies and negligible contribution of higher harmonics to the spiral state. The significant difference between the dc magnetic susceptibility and the lowest-frequency ac susceptibility in our experiment implies the existence of mode(s) outside of the measured frequency windows. The combination of THz and microwave experiments suggests a spin gap opening below the ordering temperature between 50 GHz and 100 GHz. Nature Publishing Group UK 2023-07-08 /pmc/articles/PMC10329720/ /pubmed/37422590 http://dx.doi.org/10.1038/s41598-023-37911-6 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Tóth, Boglárka Amelin, Kirill Rõõm, Toomas Nagel, Urmas Bauernfeind, Anastasia Tsurkan, Vladimir Prodan, Lilian Krug von Nidda, Hans-Albrecht Scheffler, Marc Kézsmárki, István Bordács, Sándor Broadband magnetic resonance spectroscopy in MnSc[Formula: see text] S[Formula: see text] |
title | Broadband magnetic resonance spectroscopy in MnSc[Formula: see text] S[Formula: see text] |
title_full | Broadband magnetic resonance spectroscopy in MnSc[Formula: see text] S[Formula: see text] |
title_fullStr | Broadband magnetic resonance spectroscopy in MnSc[Formula: see text] S[Formula: see text] |
title_full_unstemmed | Broadband magnetic resonance spectroscopy in MnSc[Formula: see text] S[Formula: see text] |
title_short | Broadband magnetic resonance spectroscopy in MnSc[Formula: see text] S[Formula: see text] |
title_sort | broadband magnetic resonance spectroscopy in mnsc[formula: see text] s[formula: see text] |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10329720/ https://www.ncbi.nlm.nih.gov/pubmed/37422590 http://dx.doi.org/10.1038/s41598-023-37911-6 |
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