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Generation and control of localized terahertz fields in photoemitted electron plasmas

Dense micron-sized electron plasmas, such as those generated upon irradiation of nanostructured metallic surfaces by intense femtosecond laser pulses, constitute a rich playground to study light–matter interactions, many-body phenomena, and out-of-equilibrium charge dynamics. Besides their fundament...

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Autores principales: Dias, Eduardo J. C., Madan, Ivan, Gargiulo, Simone, Barantani, Francesco, Yannai, Michael, Vanacore, Giovanni Maria, Kaminer, Ido, Carbone, Fabrizio, García de Abajo, F. Javier
Formato: Online Artículo Texto
Lenguaje:English
Publicado: RSC 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10334422/
https://www.ncbi.nlm.nih.gov/pubmed/37441257
http://dx.doi.org/10.1039/d3na00168g
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author Dias, Eduardo J. C.
Madan, Ivan
Gargiulo, Simone
Barantani, Francesco
Yannai, Michael
Vanacore, Giovanni Maria
Kaminer, Ido
Carbone, Fabrizio
García de Abajo, F. Javier
author_facet Dias, Eduardo J. C.
Madan, Ivan
Gargiulo, Simone
Barantani, Francesco
Yannai, Michael
Vanacore, Giovanni Maria
Kaminer, Ido
Carbone, Fabrizio
García de Abajo, F. Javier
author_sort Dias, Eduardo J. C.
collection PubMed
description Dense micron-sized electron plasmas, such as those generated upon irradiation of nanostructured metallic surfaces by intense femtosecond laser pulses, constitute a rich playground to study light–matter interactions, many-body phenomena, and out-of-equilibrium charge dynamics. Besides their fundamental interest, laser-induced plasmas hold great potential for the generation of localized terahertz radiation pulses. However, the underlying mechanisms ruling the formation and evolution of such plasmas are not yet well understood. Here, we develop a comprehensive microscopic theory to predictably describe the spatiotemporal dynamics of laser-pulse-induced plasmas. Through detailed analysis of electron emission, metal screening, and plasma cloud interactions, we investigate the spatial, temporal, and spectral characteristics of the so-generated terahertz fields, which can be extensively controlled through the metal morphology and the illumination conditions. We further describe the interaction with femtosecond electron beams to explain recent ultrafast electron microscopy experiments, whereby the position and temporal dependence of the observed electron acceleration permits assessing the associated terahertz field. Besides its potential application to the design of low-frequency light sources, our work contributes fundamental insight into the generation and dynamics of micron-scale electron plasmas and their interaction with ultrafast electron pulses.
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spelling pubmed-103344222023-07-12 Generation and control of localized terahertz fields in photoemitted electron plasmas Dias, Eduardo J. C. Madan, Ivan Gargiulo, Simone Barantani, Francesco Yannai, Michael Vanacore, Giovanni Maria Kaminer, Ido Carbone, Fabrizio García de Abajo, F. Javier Nanoscale Adv Chemistry Dense micron-sized electron plasmas, such as those generated upon irradiation of nanostructured metallic surfaces by intense femtosecond laser pulses, constitute a rich playground to study light–matter interactions, many-body phenomena, and out-of-equilibrium charge dynamics. Besides their fundamental interest, laser-induced plasmas hold great potential for the generation of localized terahertz radiation pulses. However, the underlying mechanisms ruling the formation and evolution of such plasmas are not yet well understood. Here, we develop a comprehensive microscopic theory to predictably describe the spatiotemporal dynamics of laser-pulse-induced plasmas. Through detailed analysis of electron emission, metal screening, and plasma cloud interactions, we investigate the spatial, temporal, and spectral characteristics of the so-generated terahertz fields, which can be extensively controlled through the metal morphology and the illumination conditions. We further describe the interaction with femtosecond electron beams to explain recent ultrafast electron microscopy experiments, whereby the position and temporal dependence of the observed electron acceleration permits assessing the associated terahertz field. Besides its potential application to the design of low-frequency light sources, our work contributes fundamental insight into the generation and dynamics of micron-scale electron plasmas and their interaction with ultrafast electron pulses. RSC 2023-05-04 /pmc/articles/PMC10334422/ /pubmed/37441257 http://dx.doi.org/10.1039/d3na00168g Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Dias, Eduardo J. C.
Madan, Ivan
Gargiulo, Simone
Barantani, Francesco
Yannai, Michael
Vanacore, Giovanni Maria
Kaminer, Ido
Carbone, Fabrizio
García de Abajo, F. Javier
Generation and control of localized terahertz fields in photoemitted electron plasmas
title Generation and control of localized terahertz fields in photoemitted electron plasmas
title_full Generation and control of localized terahertz fields in photoemitted electron plasmas
title_fullStr Generation and control of localized terahertz fields in photoemitted electron plasmas
title_full_unstemmed Generation and control of localized terahertz fields in photoemitted electron plasmas
title_short Generation and control of localized terahertz fields in photoemitted electron plasmas
title_sort generation and control of localized terahertz fields in photoemitted electron plasmas
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10334422/
https://www.ncbi.nlm.nih.gov/pubmed/37441257
http://dx.doi.org/10.1039/d3na00168g
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