Cargando…

Theoretical Study on the Photoemission Performance of a Transmission Mode In(0.15)Ga(0.85)As Photocathode in the Near-Infrared Region

Benefiting from a high quantum efficiency, low thermal emittance, and large absorption coefficient, In(x)Ga(1−x)As is an excellent group III–V compound for negative electron affinity (NEA) photocathodes. As the emission layer, In(x)Ga(1−x)As, where x = 0.15, has the optimal performance for detection...

Descripción completa

Detalles Bibliográficos
Autores principales: Wang, Huan, Linghu, Jiajun, Zou, Pengfei, Wang, Xuezhi, Shen, Hao, Hai, Bingru
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10343399/
https://www.ncbi.nlm.nih.gov/pubmed/37446922
http://dx.doi.org/10.3390/molecules28135262
_version_ 1785072727944593408
author Wang, Huan
Linghu, Jiajun
Zou, Pengfei
Wang, Xuezhi
Shen, Hao
Hai, Bingru
author_facet Wang, Huan
Linghu, Jiajun
Zou, Pengfei
Wang, Xuezhi
Shen, Hao
Hai, Bingru
author_sort Wang, Huan
collection PubMed
description Benefiting from a high quantum efficiency, low thermal emittance, and large absorption coefficient, In(x)Ga(1−x)As is an excellent group III–V compound for negative electron affinity (NEA) photocathodes. As the emission layer, In(x)Ga(1−x)As, where x = 0.15, has the optimal performance for detection in the near-infrared (NIR) region. Herein, an NEA In(0.15)Ga(0.85)As photocathode with Al(0.63)Ga(0.37)As as the buffer layer is designed in the form of a transmission mode module. The electronic band structures and optical properties of In(0.15)Ga(0.85)As and Al(0.63)Ga(0.37)As are calculated based on density functional theory. The time response characteristics of the In(0.15)Ga(0.85)As photocathode have been fully investigated by changing the photoelectron diffusion coefficient, the interface recombination velocity, and the thickness of the emission layer. Our results demonstrate that the response time of the In(0.15)Ga(0.85)As photocathode can be reduced to 6.1 ps with an incident wavelength of 1064 nm. The quantum efficiency of the In(0.15)Ga(0.85)As photocathode is simulated by taking into account multilayer optical thin film theory. The results indicate that a high quantum efficiency can be obtained by parameter optimization of the emission layer. This paper provides significant theoretical support for the applications of semiconductor photocathodes in the near-infrared region, especially for the study of ultrafast responses in the photoemission process.
format Online
Article
Text
id pubmed-10343399
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher MDPI
record_format MEDLINE/PubMed
spelling pubmed-103433992023-07-14 Theoretical Study on the Photoemission Performance of a Transmission Mode In(0.15)Ga(0.85)As Photocathode in the Near-Infrared Region Wang, Huan Linghu, Jiajun Zou, Pengfei Wang, Xuezhi Shen, Hao Hai, Bingru Molecules Article Benefiting from a high quantum efficiency, low thermal emittance, and large absorption coefficient, In(x)Ga(1−x)As is an excellent group III–V compound for negative electron affinity (NEA) photocathodes. As the emission layer, In(x)Ga(1−x)As, where x = 0.15, has the optimal performance for detection in the near-infrared (NIR) region. Herein, an NEA In(0.15)Ga(0.85)As photocathode with Al(0.63)Ga(0.37)As as the buffer layer is designed in the form of a transmission mode module. The electronic band structures and optical properties of In(0.15)Ga(0.85)As and Al(0.63)Ga(0.37)As are calculated based on density functional theory. The time response characteristics of the In(0.15)Ga(0.85)As photocathode have been fully investigated by changing the photoelectron diffusion coefficient, the interface recombination velocity, and the thickness of the emission layer. Our results demonstrate that the response time of the In(0.15)Ga(0.85)As photocathode can be reduced to 6.1 ps with an incident wavelength of 1064 nm. The quantum efficiency of the In(0.15)Ga(0.85)As photocathode is simulated by taking into account multilayer optical thin film theory. The results indicate that a high quantum efficiency can be obtained by parameter optimization of the emission layer. This paper provides significant theoretical support for the applications of semiconductor photocathodes in the near-infrared region, especially for the study of ultrafast responses in the photoemission process. MDPI 2023-07-07 /pmc/articles/PMC10343399/ /pubmed/37446922 http://dx.doi.org/10.3390/molecules28135262 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Wang, Huan
Linghu, Jiajun
Zou, Pengfei
Wang, Xuezhi
Shen, Hao
Hai, Bingru
Theoretical Study on the Photoemission Performance of a Transmission Mode In(0.15)Ga(0.85)As Photocathode in the Near-Infrared Region
title Theoretical Study on the Photoemission Performance of a Transmission Mode In(0.15)Ga(0.85)As Photocathode in the Near-Infrared Region
title_full Theoretical Study on the Photoemission Performance of a Transmission Mode In(0.15)Ga(0.85)As Photocathode in the Near-Infrared Region
title_fullStr Theoretical Study on the Photoemission Performance of a Transmission Mode In(0.15)Ga(0.85)As Photocathode in the Near-Infrared Region
title_full_unstemmed Theoretical Study on the Photoemission Performance of a Transmission Mode In(0.15)Ga(0.85)As Photocathode in the Near-Infrared Region
title_short Theoretical Study on the Photoemission Performance of a Transmission Mode In(0.15)Ga(0.85)As Photocathode in the Near-Infrared Region
title_sort theoretical study on the photoemission performance of a transmission mode in(0.15)ga(0.85)as photocathode in the near-infrared region
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10343399/
https://www.ncbi.nlm.nih.gov/pubmed/37446922
http://dx.doi.org/10.3390/molecules28135262
work_keys_str_mv AT wanghuan theoreticalstudyonthephotoemissionperformanceofatransmissionmodein015ga085asphotocathodeinthenearinfraredregion
AT linghujiajun theoreticalstudyonthephotoemissionperformanceofatransmissionmodein015ga085asphotocathodeinthenearinfraredregion
AT zoupengfei theoreticalstudyonthephotoemissionperformanceofatransmissionmodein015ga085asphotocathodeinthenearinfraredregion
AT wangxuezhi theoreticalstudyonthephotoemissionperformanceofatransmissionmodein015ga085asphotocathodeinthenearinfraredregion
AT shenhao theoreticalstudyonthephotoemissionperformanceofatransmissionmodein015ga085asphotocathodeinthenearinfraredregion
AT haibingru theoreticalstudyonthephotoemissionperformanceofatransmissionmodein015ga085asphotocathodeinthenearinfraredregion