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Exploring Material Properties and Device Output Performance of a Miniaturized Flexible Thermoelectric Generator Using Scalable Synthesis of Bi(2)Se(3) Nanoflakes
Environmental heat-to-electric energy conversion presents a promising solution for powering sensors in wearable and portable devices. However, the availability of near-room temperature thermoelectric (TE) materials is highly limited, posing a significant challenge in this field. Bi(2)Se(3), as a roo...
Autores principales: | , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10343555/ https://www.ncbi.nlm.nih.gov/pubmed/37446453 http://dx.doi.org/10.3390/nano13131937 |
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author | Yuan, Zicheng Zhao, Xueke Wang, Canhui Hang, Shuang Li, Mengyao Liu, Yu |
author_facet | Yuan, Zicheng Zhao, Xueke Wang, Canhui Hang, Shuang Li, Mengyao Liu, Yu |
author_sort | Yuan, Zicheng |
collection | PubMed |
description | Environmental heat-to-electric energy conversion presents a promising solution for powering sensors in wearable and portable devices. However, the availability of near-room temperature thermoelectric (TE) materials is highly limited, posing a significant challenge in this field. Bi(2)Se(3), as a room-temperature TE material, has attracted much attention. Here, we demonstrate a large-scale synthesis of Bi(2)Se(3) nanoflakes used for the microflexible TE generator. A high-performance micro-TE generator module, utilizing a flexible printed circuit, has been designed and fabricated through the process of screen printing. The TE generator configuration comprises five pairs of PN TE legs. The p-type TE leg utilizes commercially available Sb(2)Te(3) powder, while the n-type TE leg employs Bi(2)Se(3) nanoflakes synthesized in this study. For comparative purposes, we also incorporate commercially available Bi(2)Se(3) powder as an alternative n-type TE leg. The optimal performance of the single-layer microflexible TE generator, employing Bi(2)Se(3) nanoflakes as the active material, is achieved when operating at a temperature differential of 109.5 K, the open-circuit voltage (V(OC)) is 0.11 V, the short circuit current (I(SC)) is 0.34 mA, and the maximum output power (P(MAX)) is 9.5 μW, much higher than the generator consisting of commercial Bi(2)Se(3) powder, which is expected to provide an energy supply for flexible electronic devices. |
format | Online Article Text |
id | pubmed-10343555 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-103435552023-07-14 Exploring Material Properties and Device Output Performance of a Miniaturized Flexible Thermoelectric Generator Using Scalable Synthesis of Bi(2)Se(3) Nanoflakes Yuan, Zicheng Zhao, Xueke Wang, Canhui Hang, Shuang Li, Mengyao Liu, Yu Nanomaterials (Basel) Article Environmental heat-to-electric energy conversion presents a promising solution for powering sensors in wearable and portable devices. However, the availability of near-room temperature thermoelectric (TE) materials is highly limited, posing a significant challenge in this field. Bi(2)Se(3), as a room-temperature TE material, has attracted much attention. Here, we demonstrate a large-scale synthesis of Bi(2)Se(3) nanoflakes used for the microflexible TE generator. A high-performance micro-TE generator module, utilizing a flexible printed circuit, has been designed and fabricated through the process of screen printing. The TE generator configuration comprises five pairs of PN TE legs. The p-type TE leg utilizes commercially available Sb(2)Te(3) powder, while the n-type TE leg employs Bi(2)Se(3) nanoflakes synthesized in this study. For comparative purposes, we also incorporate commercially available Bi(2)Se(3) powder as an alternative n-type TE leg. The optimal performance of the single-layer microflexible TE generator, employing Bi(2)Se(3) nanoflakes as the active material, is achieved when operating at a temperature differential of 109.5 K, the open-circuit voltage (V(OC)) is 0.11 V, the short circuit current (I(SC)) is 0.34 mA, and the maximum output power (P(MAX)) is 9.5 μW, much higher than the generator consisting of commercial Bi(2)Se(3) powder, which is expected to provide an energy supply for flexible electronic devices. MDPI 2023-06-26 /pmc/articles/PMC10343555/ /pubmed/37446453 http://dx.doi.org/10.3390/nano13131937 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Yuan, Zicheng Zhao, Xueke Wang, Canhui Hang, Shuang Li, Mengyao Liu, Yu Exploring Material Properties and Device Output Performance of a Miniaturized Flexible Thermoelectric Generator Using Scalable Synthesis of Bi(2)Se(3) Nanoflakes |
title | Exploring Material Properties and Device Output Performance of a Miniaturized Flexible Thermoelectric Generator Using Scalable Synthesis of Bi(2)Se(3) Nanoflakes |
title_full | Exploring Material Properties and Device Output Performance of a Miniaturized Flexible Thermoelectric Generator Using Scalable Synthesis of Bi(2)Se(3) Nanoflakes |
title_fullStr | Exploring Material Properties and Device Output Performance of a Miniaturized Flexible Thermoelectric Generator Using Scalable Synthesis of Bi(2)Se(3) Nanoflakes |
title_full_unstemmed | Exploring Material Properties and Device Output Performance of a Miniaturized Flexible Thermoelectric Generator Using Scalable Synthesis of Bi(2)Se(3) Nanoflakes |
title_short | Exploring Material Properties and Device Output Performance of a Miniaturized Flexible Thermoelectric Generator Using Scalable Synthesis of Bi(2)Se(3) Nanoflakes |
title_sort | exploring material properties and device output performance of a miniaturized flexible thermoelectric generator using scalable synthesis of bi(2)se(3) nanoflakes |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10343555/ https://www.ncbi.nlm.nih.gov/pubmed/37446453 http://dx.doi.org/10.3390/nano13131937 |
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