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Unveiling phase diagram of the lightly doped high-T(c) cuprate superconductors with disorder removed

The currently established electronic phase diagram of cuprates is based on a study of single- and double-layered compounds. These CuO(2) planes, however, are directly contacted with dopant layers, thus inevitably disordered with an inhomogeneous electronic state. Here, we solve this issue by investi...

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Autores principales: Kurokawa, Kifu, Isono, Shunsuke, Kohama, Yoshimitsu, Kunisada, So, Sakai, Shiro, Sekine, Ryotaro, Okubo, Makoto, Watson, Matthew D., Kim, Timur K., Cacho, Cephise, Shin, Shik, Tohyama, Takami, Tokiwa, Kazuyasu, Kondo, Takeshi
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10349131/
https://www.ncbi.nlm.nih.gov/pubmed/37452014
http://dx.doi.org/10.1038/s41467-023-39457-7
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author Kurokawa, Kifu
Isono, Shunsuke
Kohama, Yoshimitsu
Kunisada, So
Sakai, Shiro
Sekine, Ryotaro
Okubo, Makoto
Watson, Matthew D.
Kim, Timur K.
Cacho, Cephise
Shin, Shik
Tohyama, Takami
Tokiwa, Kazuyasu
Kondo, Takeshi
author_facet Kurokawa, Kifu
Isono, Shunsuke
Kohama, Yoshimitsu
Kunisada, So
Sakai, Shiro
Sekine, Ryotaro
Okubo, Makoto
Watson, Matthew D.
Kim, Timur K.
Cacho, Cephise
Shin, Shik
Tohyama, Takami
Tokiwa, Kazuyasu
Kondo, Takeshi
author_sort Kurokawa, Kifu
collection PubMed
description The currently established electronic phase diagram of cuprates is based on a study of single- and double-layered compounds. These CuO(2) planes, however, are directly contacted with dopant layers, thus inevitably disordered with an inhomogeneous electronic state. Here, we solve this issue by investigating a 6-layered Ba(2)Ca(5)Cu(6)O(12)(F,O)(2) with inner CuO(2) layers, which are clean with the extremely low disorder, by angle-resolved photoemission spectroscopy (ARPES) and quantum oscillation measurements. We find a tiny Fermi pocket with a doping level less than 1% to exhibit well-defined quasiparticle peaks which surprisingly lack the polaronic feature. This provides the first evidence that the slightest amount of carriers is enough to turn a Mott insulating state into a metallic state with long-lived quasiparticles. By tuning hole carriers, we also find an unexpected phase transition from the superconducting to metallic states at 4%. Our results are distinct from the nodal liquid state with polaronic features proposed as an anomaly of the heavily underdoped cuprates.
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spelling pubmed-103491312023-07-16 Unveiling phase diagram of the lightly doped high-T(c) cuprate superconductors with disorder removed Kurokawa, Kifu Isono, Shunsuke Kohama, Yoshimitsu Kunisada, So Sakai, Shiro Sekine, Ryotaro Okubo, Makoto Watson, Matthew D. Kim, Timur K. Cacho, Cephise Shin, Shik Tohyama, Takami Tokiwa, Kazuyasu Kondo, Takeshi Nat Commun Article The currently established electronic phase diagram of cuprates is based on a study of single- and double-layered compounds. These CuO(2) planes, however, are directly contacted with dopant layers, thus inevitably disordered with an inhomogeneous electronic state. Here, we solve this issue by investigating a 6-layered Ba(2)Ca(5)Cu(6)O(12)(F,O)(2) with inner CuO(2) layers, which are clean with the extremely low disorder, by angle-resolved photoemission spectroscopy (ARPES) and quantum oscillation measurements. We find a tiny Fermi pocket with a doping level less than 1% to exhibit well-defined quasiparticle peaks which surprisingly lack the polaronic feature. This provides the first evidence that the slightest amount of carriers is enough to turn a Mott insulating state into a metallic state with long-lived quasiparticles. By tuning hole carriers, we also find an unexpected phase transition from the superconducting to metallic states at 4%. Our results are distinct from the nodal liquid state with polaronic features proposed as an anomaly of the heavily underdoped cuprates. Nature Publishing Group UK 2023-07-14 /pmc/articles/PMC10349131/ /pubmed/37452014 http://dx.doi.org/10.1038/s41467-023-39457-7 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Kurokawa, Kifu
Isono, Shunsuke
Kohama, Yoshimitsu
Kunisada, So
Sakai, Shiro
Sekine, Ryotaro
Okubo, Makoto
Watson, Matthew D.
Kim, Timur K.
Cacho, Cephise
Shin, Shik
Tohyama, Takami
Tokiwa, Kazuyasu
Kondo, Takeshi
Unveiling phase diagram of the lightly doped high-T(c) cuprate superconductors with disorder removed
title Unveiling phase diagram of the lightly doped high-T(c) cuprate superconductors with disorder removed
title_full Unveiling phase diagram of the lightly doped high-T(c) cuprate superconductors with disorder removed
title_fullStr Unveiling phase diagram of the lightly doped high-T(c) cuprate superconductors with disorder removed
title_full_unstemmed Unveiling phase diagram of the lightly doped high-T(c) cuprate superconductors with disorder removed
title_short Unveiling phase diagram of the lightly doped high-T(c) cuprate superconductors with disorder removed
title_sort unveiling phase diagram of the lightly doped high-t(c) cuprate superconductors with disorder removed
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10349131/
https://www.ncbi.nlm.nih.gov/pubmed/37452014
http://dx.doi.org/10.1038/s41467-023-39457-7
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