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Low-energy quasi-circular electron correlations with charge order wavelength in Bi(2)Sr(2)CaCu(2)O(8+δ)

Most resonant inelastic x-ray scattering (RIXS) studies of dynamic charge order correlations in the cuprates have focused on the high-symmetry directions of the copper oxide plane. However, scattering along other in-plane directions should not be ignored as it may help understand, for example, the o...

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Autores principales: Scott, Kirsty, Kisiel, Elliot, Boyle, Timothy J., Basak, Rourav, Jargot, Gaëtan, Das, Sarmistha, Agrestini, Stefano, Garcia-Fernandez, Mirian, Choi, Jaewon, Pelliciari, Jonathan, Li, Jiemin, Chuang, Yi-De, Zhong, Ruidan, Schneeloch, John A., Gu, Genda, Légaré, François, Kemper, Alexander F., Zhou, Ke-Jin, Bisogni, Valentina, Blanco-Canosa, Santiago, Frano, Alex, Boschini, Fabio, da Silva Neto, Eduardo H.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10355819/
https://www.ncbi.nlm.nih.gov/pubmed/37467326
http://dx.doi.org/10.1126/sciadv.adg3710
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author Scott, Kirsty
Kisiel, Elliot
Boyle, Timothy J.
Basak, Rourav
Jargot, Gaëtan
Das, Sarmistha
Agrestini, Stefano
Garcia-Fernandez, Mirian
Choi, Jaewon
Pelliciari, Jonathan
Li, Jiemin
Chuang, Yi-De
Zhong, Ruidan
Schneeloch, John A.
Gu, Genda
Légaré, François
Kemper, Alexander F.
Zhou, Ke-Jin
Bisogni, Valentina
Blanco-Canosa, Santiago
Frano, Alex
Boschini, Fabio
da Silva Neto, Eduardo H.
author_facet Scott, Kirsty
Kisiel, Elliot
Boyle, Timothy J.
Basak, Rourav
Jargot, Gaëtan
Das, Sarmistha
Agrestini, Stefano
Garcia-Fernandez, Mirian
Choi, Jaewon
Pelliciari, Jonathan
Li, Jiemin
Chuang, Yi-De
Zhong, Ruidan
Schneeloch, John A.
Gu, Genda
Légaré, François
Kemper, Alexander F.
Zhou, Ke-Jin
Bisogni, Valentina
Blanco-Canosa, Santiago
Frano, Alex
Boschini, Fabio
da Silva Neto, Eduardo H.
author_sort Scott, Kirsty
collection PubMed
description Most resonant inelastic x-ray scattering (RIXS) studies of dynamic charge order correlations in the cuprates have focused on the high-symmetry directions of the copper oxide plane. However, scattering along other in-plane directions should not be ignored as it may help understand, for example, the origin of charge order correlations or the isotropic scattering resulting in strange metal behavior. Our RIXS experiments reveal dynamic charge correlations over the q(x)-q(y) scattering plane in underdoped Bi(2)Sr(2)CaCu(2)O(8+δ). Tracking the softening of the RIXS-measured bond-stretching phonon, we show that these dynamic correlations exist at energies below approximately 70 meV and are centered around a quasi-circular manifold in the q(x)-q(y) scattering plane with radius equal to the magnitude of the charge order wave vector, q(CO). This phonon-tracking procedure also allows us to rule out fluctuations of short-range directional charge order (i.e., centered around [q(x) = ±q(CO), q(y) = 0] and [q(x) = 0, q(y) = ±q(CO)]) as the origin of the observed correlations.
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spelling pubmed-103558192023-07-20 Low-energy quasi-circular electron correlations with charge order wavelength in Bi(2)Sr(2)CaCu(2)O(8+δ) Scott, Kirsty Kisiel, Elliot Boyle, Timothy J. Basak, Rourav Jargot, Gaëtan Das, Sarmistha Agrestini, Stefano Garcia-Fernandez, Mirian Choi, Jaewon Pelliciari, Jonathan Li, Jiemin Chuang, Yi-De Zhong, Ruidan Schneeloch, John A. Gu, Genda Légaré, François Kemper, Alexander F. Zhou, Ke-Jin Bisogni, Valentina Blanco-Canosa, Santiago Frano, Alex Boschini, Fabio da Silva Neto, Eduardo H. Sci Adv Physical and Materials Sciences Most resonant inelastic x-ray scattering (RIXS) studies of dynamic charge order correlations in the cuprates have focused on the high-symmetry directions of the copper oxide plane. However, scattering along other in-plane directions should not be ignored as it may help understand, for example, the origin of charge order correlations or the isotropic scattering resulting in strange metal behavior. Our RIXS experiments reveal dynamic charge correlations over the q(x)-q(y) scattering plane in underdoped Bi(2)Sr(2)CaCu(2)O(8+δ). Tracking the softening of the RIXS-measured bond-stretching phonon, we show that these dynamic correlations exist at energies below approximately 70 meV and are centered around a quasi-circular manifold in the q(x)-q(y) scattering plane with radius equal to the magnitude of the charge order wave vector, q(CO). This phonon-tracking procedure also allows us to rule out fluctuations of short-range directional charge order (i.e., centered around [q(x) = ±q(CO), q(y) = 0] and [q(x) = 0, q(y) = ±q(CO)]) as the origin of the observed correlations. American Association for the Advancement of Science 2023-07-19 /pmc/articles/PMC10355819/ /pubmed/37467326 http://dx.doi.org/10.1126/sciadv.adg3710 Text en Copyright © 2023 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Physical and Materials Sciences
Scott, Kirsty
Kisiel, Elliot
Boyle, Timothy J.
Basak, Rourav
Jargot, Gaëtan
Das, Sarmistha
Agrestini, Stefano
Garcia-Fernandez, Mirian
Choi, Jaewon
Pelliciari, Jonathan
Li, Jiemin
Chuang, Yi-De
Zhong, Ruidan
Schneeloch, John A.
Gu, Genda
Légaré, François
Kemper, Alexander F.
Zhou, Ke-Jin
Bisogni, Valentina
Blanco-Canosa, Santiago
Frano, Alex
Boschini, Fabio
da Silva Neto, Eduardo H.
Low-energy quasi-circular electron correlations with charge order wavelength in Bi(2)Sr(2)CaCu(2)O(8+δ)
title Low-energy quasi-circular electron correlations with charge order wavelength in Bi(2)Sr(2)CaCu(2)O(8+δ)
title_full Low-energy quasi-circular electron correlations with charge order wavelength in Bi(2)Sr(2)CaCu(2)O(8+δ)
title_fullStr Low-energy quasi-circular electron correlations with charge order wavelength in Bi(2)Sr(2)CaCu(2)O(8+δ)
title_full_unstemmed Low-energy quasi-circular electron correlations with charge order wavelength in Bi(2)Sr(2)CaCu(2)O(8+δ)
title_short Low-energy quasi-circular electron correlations with charge order wavelength in Bi(2)Sr(2)CaCu(2)O(8+δ)
title_sort low-energy quasi-circular electron correlations with charge order wavelength in bi(2)sr(2)cacu(2)o(8+δ)
topic Physical and Materials Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10355819/
https://www.ncbi.nlm.nih.gov/pubmed/37467326
http://dx.doi.org/10.1126/sciadv.adg3710
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