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High Quality Factor in Solution-Processed Inorganic Microcavities Embedding CsPbBr(3) Perovskite Nanocrystals

[Image: see text] Optical microcavities grant manipulation over light–matter interactions and light propagation, enabling the fabrication of foundational optical and optoelectronic components. However, the materials used for high-performing systems, mostly bulk inorganics, are typically costly, and...

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Detalles Bibliográficos
Autores principales: Bertucci, Simone, Escher, Andrea, Cirignano, Matilde, De Franco, Manuela, Locardi, Federico, Patrini, Maddalena, Comoretto, Davide, Lova, Paola, Di Stasio, Francesco
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10391615/
https://www.ncbi.nlm.nih.gov/pubmed/37533664
http://dx.doi.org/10.1021/acsaom.3c00157
Descripción
Sumario:[Image: see text] Optical microcavities grant manipulation over light–matter interactions and light propagation, enabling the fabrication of foundational optical and optoelectronic components. However, the materials used for high-performing systems, mostly bulk inorganics, are typically costly, and their processing is hardly scalable. In this work, we present an alternative way to fabricate planar optical resonators via solely solution processing while approaching the performances of conventional systems. Here, we couple fully solution-processed high dielectric contrast inorganic Bragg mirrors obtained by sol–gel deposition with the remarkable photoluminescence properties of CsPbBr(3) perovskite nanocrystals. The approach yields microcavities with a quality factor of ∼220, which is a record value for solution-processed inorganic structures, and a strong emission redistribution resulting in a 3-fold directional intensity enhancement.