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Enabling elliptically polarized high harmonic generation with short cross polarized laser pulses

Enabling elliptically polarized high-order harmonics overcomes a historical limitation in the generation of this highly nonlinear process in atomic, molecular and optical physics with applications in other branches. Here, we shed new light on a controversy between experimental observations and theor...

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Autores principales: Ghomashi, B., Walker, S., Becker, A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10409740/
https://www.ncbi.nlm.nih.gov/pubmed/37553388
http://dx.doi.org/10.1038/s41598-023-39814-y
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author Ghomashi, B.
Walker, S.
Becker, A.
author_facet Ghomashi, B.
Walker, S.
Becker, A.
author_sort Ghomashi, B.
collection PubMed
description Enabling elliptically polarized high-order harmonics overcomes a historical limitation in the generation of this highly nonlinear process in atomic, molecular and optical physics with applications in other branches. Here, we shed new light on a controversy between experimental observations and theoretical predictions on the possibility to generate harmonics with large ellipticity using two bichromatic laser pulses which are linearly polarized in orthogonal directions. Results of numerical calculations confirm the previous experimental data that in short laser pulses even harmonics with large ellipticity can be obtained for the interaction of such cross-polarized laser pulses with atoms initially in a s- or p-state, while odd harmonics have low ellipticity. The amount of the ellipticity can be controlled via the relative carrier-envelope phase of the pulses, their intensity ratio and the duration of the pulses.
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spelling pubmed-104097402023-08-10 Enabling elliptically polarized high harmonic generation with short cross polarized laser pulses Ghomashi, B. Walker, S. Becker, A. Sci Rep Article Enabling elliptically polarized high-order harmonics overcomes a historical limitation in the generation of this highly nonlinear process in atomic, molecular and optical physics with applications in other branches. Here, we shed new light on a controversy between experimental observations and theoretical predictions on the possibility to generate harmonics with large ellipticity using two bichromatic laser pulses which are linearly polarized in orthogonal directions. Results of numerical calculations confirm the previous experimental data that in short laser pulses even harmonics with large ellipticity can be obtained for the interaction of such cross-polarized laser pulses with atoms initially in a s- or p-state, while odd harmonics have low ellipticity. The amount of the ellipticity can be controlled via the relative carrier-envelope phase of the pulses, their intensity ratio and the duration of the pulses. Nature Publishing Group UK 2023-08-08 /pmc/articles/PMC10409740/ /pubmed/37553388 http://dx.doi.org/10.1038/s41598-023-39814-y Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Ghomashi, B.
Walker, S.
Becker, A.
Enabling elliptically polarized high harmonic generation with short cross polarized laser pulses
title Enabling elliptically polarized high harmonic generation with short cross polarized laser pulses
title_full Enabling elliptically polarized high harmonic generation with short cross polarized laser pulses
title_fullStr Enabling elliptically polarized high harmonic generation with short cross polarized laser pulses
title_full_unstemmed Enabling elliptically polarized high harmonic generation with short cross polarized laser pulses
title_short Enabling elliptically polarized high harmonic generation with short cross polarized laser pulses
title_sort enabling elliptically polarized high harmonic generation with short cross polarized laser pulses
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10409740/
https://www.ncbi.nlm.nih.gov/pubmed/37553388
http://dx.doi.org/10.1038/s41598-023-39814-y
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