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Reusability of Discarded Tubular Ceramic Membranes for CO(2) Removal: A Case Study for Membrane Circularity

[Image: see text] Discarded polymeric or ceramic membranes are currently in need of appropriate and sustainable management. In the present study, the direct reuse of discarded ceramic membranes in membrane contactor (MC) systems for CO(2) removal was investigated for the first time. The hydrophobic...

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Autores principales: Karatas, Elcim, Al-Mutwalli, Sama A., Taher, Mustafa N., Shirazi, Mohammad Mahdi A., Koseoglu-Imer, Derya Y.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10433479/
https://www.ncbi.nlm.nih.gov/pubmed/37599988
http://dx.doi.org/10.1021/acsomega.3c02568
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author Karatas, Elcim
Al-Mutwalli, Sama A.
Taher, Mustafa N.
Shirazi, Mohammad Mahdi A.
Koseoglu-Imer, Derya Y.
author_facet Karatas, Elcim
Al-Mutwalli, Sama A.
Taher, Mustafa N.
Shirazi, Mohammad Mahdi A.
Koseoglu-Imer, Derya Y.
author_sort Karatas, Elcim
collection PubMed
description [Image: see text] Discarded polymeric or ceramic membranes are currently in need of appropriate and sustainable management. In the present study, the direct reuse of discarded ceramic membranes in membrane contactor (MC) systems for CO(2) removal was investigated for the first time. The hydrophobic surface modification of the discarded ceramic membrane was done by using macromolecule additive coating. The influence of operational parameters (absorbent liquid flow rate (Q(L)), feed gas flow rate (Q(g)), and different NaOH concentrations) of the MC on CO(2) removal was investigated to prove the technical feasibility of reused ceramic membranes. The CO(2) absorption flux was 7.9 × 10(–4) mol/m(2) s at optimal conditions of 2 M NaOH, Q(L) (20 mL/min), and Q(g) (300 mL/min) with a removal efficiency of 98%, which lasted for 8 h. This study demonstrates a potential alternative for the reuse of discarded ceramic membranes and avoids their disposal in landfills. The proposed approach will also bring membrane technology into the circular economy and achieve sustainability goals by reducing the amount of waste from discarded ceramic membranes in the future and combating global warming by absorbing CO(2).
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spelling pubmed-104334792023-08-18 Reusability of Discarded Tubular Ceramic Membranes for CO(2) Removal: A Case Study for Membrane Circularity Karatas, Elcim Al-Mutwalli, Sama A. Taher, Mustafa N. Shirazi, Mohammad Mahdi A. Koseoglu-Imer, Derya Y. ACS Omega [Image: see text] Discarded polymeric or ceramic membranes are currently in need of appropriate and sustainable management. In the present study, the direct reuse of discarded ceramic membranes in membrane contactor (MC) systems for CO(2) removal was investigated for the first time. The hydrophobic surface modification of the discarded ceramic membrane was done by using macromolecule additive coating. The influence of operational parameters (absorbent liquid flow rate (Q(L)), feed gas flow rate (Q(g)), and different NaOH concentrations) of the MC on CO(2) removal was investigated to prove the technical feasibility of reused ceramic membranes. The CO(2) absorption flux was 7.9 × 10(–4) mol/m(2) s at optimal conditions of 2 M NaOH, Q(L) (20 mL/min), and Q(g) (300 mL/min) with a removal efficiency of 98%, which lasted for 8 h. This study demonstrates a potential alternative for the reuse of discarded ceramic membranes and avoids their disposal in landfills. The proposed approach will also bring membrane technology into the circular economy and achieve sustainability goals by reducing the amount of waste from discarded ceramic membranes in the future and combating global warming by absorbing CO(2). American Chemical Society 2023-07-31 /pmc/articles/PMC10433479/ /pubmed/37599988 http://dx.doi.org/10.1021/acsomega.3c02568 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Karatas, Elcim
Al-Mutwalli, Sama A.
Taher, Mustafa N.
Shirazi, Mohammad Mahdi A.
Koseoglu-Imer, Derya Y.
Reusability of Discarded Tubular Ceramic Membranes for CO(2) Removal: A Case Study for Membrane Circularity
title Reusability of Discarded Tubular Ceramic Membranes for CO(2) Removal: A Case Study for Membrane Circularity
title_full Reusability of Discarded Tubular Ceramic Membranes for CO(2) Removal: A Case Study for Membrane Circularity
title_fullStr Reusability of Discarded Tubular Ceramic Membranes for CO(2) Removal: A Case Study for Membrane Circularity
title_full_unstemmed Reusability of Discarded Tubular Ceramic Membranes for CO(2) Removal: A Case Study for Membrane Circularity
title_short Reusability of Discarded Tubular Ceramic Membranes for CO(2) Removal: A Case Study for Membrane Circularity
title_sort reusability of discarded tubular ceramic membranes for co(2) removal: a case study for membrane circularity
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10433479/
https://www.ncbi.nlm.nih.gov/pubmed/37599988
http://dx.doi.org/10.1021/acsomega.3c02568
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