Cargando…

Direct Measurement of the Local Density of Optical States in the Time Domain

[Image: see text] One of the most fundamental and relevant properties of a photonic system is the local density of optical states (LDOS) as it defines the rate at which an excited emitter dissipates energy by coupling to its surrounding. However, the direct determination of the LDOS is challenging a...

Descripción completa

Detalles Bibliográficos
Autores principales: ter Huurne, Stan E. T., Peeters, Djero B. L., Sánchez-Gil, Jose A., Rivas, Jaime Gómez
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10436706/
https://www.ncbi.nlm.nih.gov/pubmed/37602289
http://dx.doi.org/10.1021/acsphotonics.3c00781
_version_ 1785092391346110464
author ter Huurne, Stan E. T.
Peeters, Djero B. L.
Sánchez-Gil, Jose A.
Rivas, Jaime Gómez
author_facet ter Huurne, Stan E. T.
Peeters, Djero B. L.
Sánchez-Gil, Jose A.
Rivas, Jaime Gómez
author_sort ter Huurne, Stan E. T.
collection PubMed
description [Image: see text] One of the most fundamental and relevant properties of a photonic system is the local density of optical states (LDOS) as it defines the rate at which an excited emitter dissipates energy by coupling to its surrounding. However, the direct determination of the LDOS is challenging as it requires measurements of the complex electric field of a point dipole at its own position. We introduce here a near-field setup which can measure the terahertz electric field amplitude at the position of a point source in the time domain. From the measured amplitude, the frequency-dependent imaginary component of the electric field can be determined and the LDOS can be retrieved. As a proof of concept, this setup has been used to measure the partial LDOS (the LDOS for a defined dipole orientation) as a function of the distance to planar interfaces made of gold, InSb, and quartz. Furthermore, the spatially dependent partial LDOS of a resonant gold rod has been measured as well. These results have been compared with analytical results and simulations. The excellent agreement between measurements and theory demonstrates the applicability of this setup for the quantitative determination of the LDOS in complex photonic systems.
format Online
Article
Text
id pubmed-10436706
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher American Chemical Society
record_format MEDLINE/PubMed
spelling pubmed-104367062023-08-19 Direct Measurement of the Local Density of Optical States in the Time Domain ter Huurne, Stan E. T. Peeters, Djero B. L. Sánchez-Gil, Jose A. Rivas, Jaime Gómez ACS Photonics [Image: see text] One of the most fundamental and relevant properties of a photonic system is the local density of optical states (LDOS) as it defines the rate at which an excited emitter dissipates energy by coupling to its surrounding. However, the direct determination of the LDOS is challenging as it requires measurements of the complex electric field of a point dipole at its own position. We introduce here a near-field setup which can measure the terahertz electric field amplitude at the position of a point source in the time domain. From the measured amplitude, the frequency-dependent imaginary component of the electric field can be determined and the LDOS can be retrieved. As a proof of concept, this setup has been used to measure the partial LDOS (the LDOS for a defined dipole orientation) as a function of the distance to planar interfaces made of gold, InSb, and quartz. Furthermore, the spatially dependent partial LDOS of a resonant gold rod has been measured as well. These results have been compared with analytical results and simulations. The excellent agreement between measurements and theory demonstrates the applicability of this setup for the quantitative determination of the LDOS in complex photonic systems. American Chemical Society 2023-08-01 /pmc/articles/PMC10436706/ /pubmed/37602289 http://dx.doi.org/10.1021/acsphotonics.3c00781 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle ter Huurne, Stan E. T.
Peeters, Djero B. L.
Sánchez-Gil, Jose A.
Rivas, Jaime Gómez
Direct Measurement of the Local Density of Optical States in the Time Domain
title Direct Measurement of the Local Density of Optical States in the Time Domain
title_full Direct Measurement of the Local Density of Optical States in the Time Domain
title_fullStr Direct Measurement of the Local Density of Optical States in the Time Domain
title_full_unstemmed Direct Measurement of the Local Density of Optical States in the Time Domain
title_short Direct Measurement of the Local Density of Optical States in the Time Domain
title_sort direct measurement of the local density of optical states in the time domain
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10436706/
https://www.ncbi.nlm.nih.gov/pubmed/37602289
http://dx.doi.org/10.1021/acsphotonics.3c00781
work_keys_str_mv AT terhuurnestanet directmeasurementofthelocaldensityofopticalstatesinthetimedomain
AT peetersdjerobl directmeasurementofthelocaldensityofopticalstatesinthetimedomain
AT sanchezgiljosea directmeasurementofthelocaldensityofopticalstatesinthetimedomain
AT rivasjaimegomez directmeasurementofthelocaldensityofopticalstatesinthetimedomain