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Band Nonlinearity-Enabled Manipulation of Dirac Nodes, Weyl Cones, and Valleytronics with Intense Linearly Polarized Light

[Image: see text] We study low-frequency linearly polarized laser-dressing in materials with valley (graphene and hexagonal-Boron-Nitride) and topological (Dirac- and Weyl-semimetals) properties. In Dirac-like linearly dispersing bands, the laser substantially moves the Dirac nodes away from their o...

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Autores principales: Neufeld, Ofer, Hübener, Hannes, Jotzu, Gregor, De Giovannini, Umberto, Rubio, Angel
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10450813/
https://www.ncbi.nlm.nih.gov/pubmed/37578460
http://dx.doi.org/10.1021/acs.nanolett.3c02139
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author Neufeld, Ofer
Hübener, Hannes
Jotzu, Gregor
De Giovannini, Umberto
Rubio, Angel
author_facet Neufeld, Ofer
Hübener, Hannes
Jotzu, Gregor
De Giovannini, Umberto
Rubio, Angel
author_sort Neufeld, Ofer
collection PubMed
description [Image: see text] We study low-frequency linearly polarized laser-dressing in materials with valley (graphene and hexagonal-Boron-Nitride) and topological (Dirac- and Weyl-semimetals) properties. In Dirac-like linearly dispersing bands, the laser substantially moves the Dirac nodes away from their original position, and the movement direction can be fully controlled by rotating the laser polarization. We prove that this effect originates from band nonlinearities away from the Dirac nodes. We further demonstrate that this physical mechanism is widely applicable and can move the positions of the valley minima in hexagonal materials to tune valley selectivity, split and move Weyl cones in higher-order Weyl semimetals, and merge Dirac nodes in three-dimensional Dirac semimetals. The model results are validated with ab initio calculations. Our results directly affect efforts for exploring light-dressed electronic structure, suggesting that one can benefit from band nonlinearity for tailoring material properties, and highlight the importance of the full band structure in nonlinear optical phenomena in solids.
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spelling pubmed-104508132023-08-26 Band Nonlinearity-Enabled Manipulation of Dirac Nodes, Weyl Cones, and Valleytronics with Intense Linearly Polarized Light Neufeld, Ofer Hübener, Hannes Jotzu, Gregor De Giovannini, Umberto Rubio, Angel Nano Lett [Image: see text] We study low-frequency linearly polarized laser-dressing in materials with valley (graphene and hexagonal-Boron-Nitride) and topological (Dirac- and Weyl-semimetals) properties. In Dirac-like linearly dispersing bands, the laser substantially moves the Dirac nodes away from their original position, and the movement direction can be fully controlled by rotating the laser polarization. We prove that this effect originates from band nonlinearities away from the Dirac nodes. We further demonstrate that this physical mechanism is widely applicable and can move the positions of the valley minima in hexagonal materials to tune valley selectivity, split and move Weyl cones in higher-order Weyl semimetals, and merge Dirac nodes in three-dimensional Dirac semimetals. The model results are validated with ab initio calculations. Our results directly affect efforts for exploring light-dressed electronic structure, suggesting that one can benefit from band nonlinearity for tailoring material properties, and highlight the importance of the full band structure in nonlinear optical phenomena in solids. American Chemical Society 2023-08-14 /pmc/articles/PMC10450813/ /pubmed/37578460 http://dx.doi.org/10.1021/acs.nanolett.3c02139 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Neufeld, Ofer
Hübener, Hannes
Jotzu, Gregor
De Giovannini, Umberto
Rubio, Angel
Band Nonlinearity-Enabled Manipulation of Dirac Nodes, Weyl Cones, and Valleytronics with Intense Linearly Polarized Light
title Band Nonlinearity-Enabled Manipulation of Dirac Nodes, Weyl Cones, and Valleytronics with Intense Linearly Polarized Light
title_full Band Nonlinearity-Enabled Manipulation of Dirac Nodes, Weyl Cones, and Valleytronics with Intense Linearly Polarized Light
title_fullStr Band Nonlinearity-Enabled Manipulation of Dirac Nodes, Weyl Cones, and Valleytronics with Intense Linearly Polarized Light
title_full_unstemmed Band Nonlinearity-Enabled Manipulation of Dirac Nodes, Weyl Cones, and Valleytronics with Intense Linearly Polarized Light
title_short Band Nonlinearity-Enabled Manipulation of Dirac Nodes, Weyl Cones, and Valleytronics with Intense Linearly Polarized Light
title_sort band nonlinearity-enabled manipulation of dirac nodes, weyl cones, and valleytronics with intense linearly polarized light
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10450813/
https://www.ncbi.nlm.nih.gov/pubmed/37578460
http://dx.doi.org/10.1021/acs.nanolett.3c02139
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