Cargando…

A study on rapid and stable catalytic reduction of 4-nitrophenol by 2-hydroxyethylamine stabilized Fe(3)O(4)@Pt and its kinetic factors

The successful development of efficient and stable catalysts for 4-NP reduction reactions is beneficial to the environment and ecology. Fe(3)O(4)@Pt exhibits excellent catalytic performance for 4-NP reduction reaction due to the synergistic effect between Fe and Pt. But its structure and catalytic p...

Descripción completa

Detalles Bibliográficos
Autores principales: Xu, Xia, Yang, Liming, Cui, Yanjun, Hu, Bing
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10467567/
https://www.ncbi.nlm.nih.gov/pubmed/37655348
http://dx.doi.org/10.1039/d3ra05298b
_version_ 1785099130584956928
author Xu, Xia
Yang, Liming
Cui, Yanjun
Hu, Bing
author_facet Xu, Xia
Yang, Liming
Cui, Yanjun
Hu, Bing
author_sort Xu, Xia
collection PubMed
description The successful development of efficient and stable catalysts for 4-NP reduction reactions is beneficial to the environment and ecology. Fe(3)O(4)@Pt exhibits excellent catalytic performance for 4-NP reduction reaction due to the synergistic effect between Fe and Pt. But its structure and catalytic performance are extremely unstable. Here, we utilized the small-scale organic compound 2-hydroxyethylamine as surfactant to construct a stable composite nanomaterial. Then investigated the influence of monochromatic light (650 nm, 808 nm and 980 nm) and temperature on the kinetics of 4-NP reduction reaction by 2-hydroxyethylamine stabilized Fe(3)O(4)@Pt. The results indicate that both temperature and monochromatic light radiation can affect kinetic regulation. Increasing temperature can promote the catalytic rate, while monochromatic light radiation can induce agglomeration and inhibit the catalytic rate. This study opens up a new way for developing and regulating catalysts for heterogeneous catalysis reactions.
format Online
Article
Text
id pubmed-10467567
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher The Royal Society of Chemistry
record_format MEDLINE/PubMed
spelling pubmed-104675672023-08-31 A study on rapid and stable catalytic reduction of 4-nitrophenol by 2-hydroxyethylamine stabilized Fe(3)O(4)@Pt and its kinetic factors Xu, Xia Yang, Liming Cui, Yanjun Hu, Bing RSC Adv Chemistry The successful development of efficient and stable catalysts for 4-NP reduction reactions is beneficial to the environment and ecology. Fe(3)O(4)@Pt exhibits excellent catalytic performance for 4-NP reduction reaction due to the synergistic effect between Fe and Pt. But its structure and catalytic performance are extremely unstable. Here, we utilized the small-scale organic compound 2-hydroxyethylamine as surfactant to construct a stable composite nanomaterial. Then investigated the influence of monochromatic light (650 nm, 808 nm and 980 nm) and temperature on the kinetics of 4-NP reduction reaction by 2-hydroxyethylamine stabilized Fe(3)O(4)@Pt. The results indicate that both temperature and monochromatic light radiation can affect kinetic regulation. Increasing temperature can promote the catalytic rate, while monochromatic light radiation can induce agglomeration and inhibit the catalytic rate. This study opens up a new way for developing and regulating catalysts for heterogeneous catalysis reactions. The Royal Society of Chemistry 2023-08-30 /pmc/articles/PMC10467567/ /pubmed/37655348 http://dx.doi.org/10.1039/d3ra05298b Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Xu, Xia
Yang, Liming
Cui, Yanjun
Hu, Bing
A study on rapid and stable catalytic reduction of 4-nitrophenol by 2-hydroxyethylamine stabilized Fe(3)O(4)@Pt and its kinetic factors
title A study on rapid and stable catalytic reduction of 4-nitrophenol by 2-hydroxyethylamine stabilized Fe(3)O(4)@Pt and its kinetic factors
title_full A study on rapid and stable catalytic reduction of 4-nitrophenol by 2-hydroxyethylamine stabilized Fe(3)O(4)@Pt and its kinetic factors
title_fullStr A study on rapid and stable catalytic reduction of 4-nitrophenol by 2-hydroxyethylamine stabilized Fe(3)O(4)@Pt and its kinetic factors
title_full_unstemmed A study on rapid and stable catalytic reduction of 4-nitrophenol by 2-hydroxyethylamine stabilized Fe(3)O(4)@Pt and its kinetic factors
title_short A study on rapid and stable catalytic reduction of 4-nitrophenol by 2-hydroxyethylamine stabilized Fe(3)O(4)@Pt and its kinetic factors
title_sort study on rapid and stable catalytic reduction of 4-nitrophenol by 2-hydroxyethylamine stabilized fe(3)o(4)@pt and its kinetic factors
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10467567/
https://www.ncbi.nlm.nih.gov/pubmed/37655348
http://dx.doi.org/10.1039/d3ra05298b
work_keys_str_mv AT xuxia astudyonrapidandstablecatalyticreductionof4nitrophenolby2hydroxyethylaminestabilizedfe3o4ptanditskineticfactors
AT yangliming astudyonrapidandstablecatalyticreductionof4nitrophenolby2hydroxyethylaminestabilizedfe3o4ptanditskineticfactors
AT cuiyanjun astudyonrapidandstablecatalyticreductionof4nitrophenolby2hydroxyethylaminestabilizedfe3o4ptanditskineticfactors
AT hubing astudyonrapidandstablecatalyticreductionof4nitrophenolby2hydroxyethylaminestabilizedfe3o4ptanditskineticfactors
AT xuxia studyonrapidandstablecatalyticreductionof4nitrophenolby2hydroxyethylaminestabilizedfe3o4ptanditskineticfactors
AT yangliming studyonrapidandstablecatalyticreductionof4nitrophenolby2hydroxyethylaminestabilizedfe3o4ptanditskineticfactors
AT cuiyanjun studyonrapidandstablecatalyticreductionof4nitrophenolby2hydroxyethylaminestabilizedfe3o4ptanditskineticfactors
AT hubing studyonrapidandstablecatalyticreductionof4nitrophenolby2hydroxyethylaminestabilizedfe3o4ptanditskineticfactors