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Exploring the capture and desorption of CO(2) on graphene oxide foams supported by computational calculations

In the last decade, the highest levels of greenhouse gases (GHG) in the atmosphere have been recorded, with carbon dioxide (CO(2)) being one of the GHGs that most concerns mankind due to the rate at which it is generated on the planet. Given its long time of permanence in the atmosphere (between 100...

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Autores principales: Arango Hoyos, Bryan E., Osorio, H. Franco, Valencia Gómez, E. K., Guerrero Sánchez, J., Del Canto Palominos, A. P., Larrain, Felipe A., Prías Barragán, J. J.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10475065/
https://www.ncbi.nlm.nih.gov/pubmed/37660192
http://dx.doi.org/10.1038/s41598-023-41683-4
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author Arango Hoyos, Bryan E.
Osorio, H. Franco
Valencia Gómez, E. K.
Guerrero Sánchez, J.
Del Canto Palominos, A. P.
Larrain, Felipe A.
Prías Barragán, J. J.
author_facet Arango Hoyos, Bryan E.
Osorio, H. Franco
Valencia Gómez, E. K.
Guerrero Sánchez, J.
Del Canto Palominos, A. P.
Larrain, Felipe A.
Prías Barragán, J. J.
author_sort Arango Hoyos, Bryan E.
collection PubMed
description In the last decade, the highest levels of greenhouse gases (GHG) in the atmosphere have been recorded, with carbon dioxide (CO(2)) being one of the GHGs that most concerns mankind due to the rate at which it is generated on the planet. Given its long time of permanence in the atmosphere (between 100 to 150 years); this has deployed research in the scientific field focused on the absorption and desorption of CO(2) in the atmosphere. This work presents the study of CO(2) adsorption employing materials based on graphene oxide (GO), such as GO foams with different oxidation percentages (3.00%, 5.25%, and 9.00%) in their structure, obtained via an environmentally friendly method. The characterization of CO(2) adsorption was carried out in a closed system, within which were placed the GO foams and other CO(2) adsorbent materials (zeolite and silica gel). Through a controlled chemical reaction, production of CO(2) was conducted to obtain CO(2) concentration curves inside the system and calculate from these the efficiency, obtained between 86.28 and 92.20%, yield between 60.10 and 99.50%, and effectiveness of CO(2) adsorption of the materials under study. The results obtained suggest that GO foams are a promising material for carbon capture and the future development of a new clean technology, given their highest CO(2) adsorption efficiency and yield.
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spelling pubmed-104750652023-09-04 Exploring the capture and desorption of CO(2) on graphene oxide foams supported by computational calculations Arango Hoyos, Bryan E. Osorio, H. Franco Valencia Gómez, E. K. Guerrero Sánchez, J. Del Canto Palominos, A. P. Larrain, Felipe A. Prías Barragán, J. J. Sci Rep Article In the last decade, the highest levels of greenhouse gases (GHG) in the atmosphere have been recorded, with carbon dioxide (CO(2)) being one of the GHGs that most concerns mankind due to the rate at which it is generated on the planet. Given its long time of permanence in the atmosphere (between 100 to 150 years); this has deployed research in the scientific field focused on the absorption and desorption of CO(2) in the atmosphere. This work presents the study of CO(2) adsorption employing materials based on graphene oxide (GO), such as GO foams with different oxidation percentages (3.00%, 5.25%, and 9.00%) in their structure, obtained via an environmentally friendly method. The characterization of CO(2) adsorption was carried out in a closed system, within which were placed the GO foams and other CO(2) adsorbent materials (zeolite and silica gel). Through a controlled chemical reaction, production of CO(2) was conducted to obtain CO(2) concentration curves inside the system and calculate from these the efficiency, obtained between 86.28 and 92.20%, yield between 60.10 and 99.50%, and effectiveness of CO(2) adsorption of the materials under study. The results obtained suggest that GO foams are a promising material for carbon capture and the future development of a new clean technology, given their highest CO(2) adsorption efficiency and yield. Nature Publishing Group UK 2023-09-02 /pmc/articles/PMC10475065/ /pubmed/37660192 http://dx.doi.org/10.1038/s41598-023-41683-4 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Arango Hoyos, Bryan E.
Osorio, H. Franco
Valencia Gómez, E. K.
Guerrero Sánchez, J.
Del Canto Palominos, A. P.
Larrain, Felipe A.
Prías Barragán, J. J.
Exploring the capture and desorption of CO(2) on graphene oxide foams supported by computational calculations
title Exploring the capture and desorption of CO(2) on graphene oxide foams supported by computational calculations
title_full Exploring the capture and desorption of CO(2) on graphene oxide foams supported by computational calculations
title_fullStr Exploring the capture and desorption of CO(2) on graphene oxide foams supported by computational calculations
title_full_unstemmed Exploring the capture and desorption of CO(2) on graphene oxide foams supported by computational calculations
title_short Exploring the capture and desorption of CO(2) on graphene oxide foams supported by computational calculations
title_sort exploring the capture and desorption of co(2) on graphene oxide foams supported by computational calculations
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10475065/
https://www.ncbi.nlm.nih.gov/pubmed/37660192
http://dx.doi.org/10.1038/s41598-023-41683-4
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